LrgpV1, Main, Merge, bibRecord, 000947

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Identifieur interne : 000947 ( Main/Merge ); précédent : 000946; suivant : 000948

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Auteurs : Chiheb Bahrini [France] ; Olivier Herbinet [France] ; Pierre-Alexandre Glaude [France] ; Coralie Schoemaecker [France] ; Christa Fittschen [France] ; Frédérique Battin-Leclerc [France]

Source :

Chemical physics letters [ 0009-2614 ] ; 2012.

RBID : PMC:3662210

English descriptors

mix :
- cw-CRDS, formaldehyde, jet-stirred reactor, methane.

Abstract

We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH₄, H₂O and CH₂O) have been quantified through their well structured spectra around 1506 nm, while H₂O₂ and HO₂ radicals could not be detected.

Url:

DOI: 10.1016/j.cplett.2012.03.012
PubMed: 23710075
PubMed Central: 3662210

Links to Exploration step

PMC:3662210

Le document en format XML

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<front><div type="abstract" xml:lang="en"><p id="P1">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH<sub>4</sub>
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<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
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<idno type="DOI">10.1016/j.cplett.2012.03.012</idno>
<series><title level="j">Chemical Physics Letters</title>
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<front><div type="abstract" xml:lang="en">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.</div>
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<PMC><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS</title>
<author><name sortKey="Bahrini, Chiheb" sort="Bahrini, Chiheb" uniqKey="Bahrini C" first="Chiheb" last="Bahrini">Chiheb Bahrini</name>
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<author><name sortKey="Schoemaecker, Coralie" sort="Schoemaecker, Coralie" uniqKey="Schoemaecker C" first="Coralie" last="Schoemaecker">Coralie Schoemaecker</name>
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<author><name sortKey="Fittschen, Christa" sort="Fittschen, Christa" uniqKey="Fittschen C" first="Christa" last="Fittschen">Christa Fittschen</name>
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<country xml:lang="fr">France</country>
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<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a" type="main">Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS</title>
<author><name sortKey="Bahrini, Chiheb" sort="Bahrini, Chiheb" uniqKey="Bahrini C" first="Chiheb" last="Bahrini">Chiheb Bahrini</name>
<affiliation wicri:level="3"><nlm:aff id="A1">KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy, France</nlm:aff>
<country xml:lang="fr">France</country>
<wicri:regionArea>KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy</wicri:regionArea>
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<region type="old region" nuts="2">Lorraine (région)</region>
<settlement type="city">Nancy</settlement>
</placeName>
</affiliation>
</author>
<author><name sortKey="Herbinet, Olivier" sort="Herbinet, Olivier" uniqKey="Herbinet O" first="Olivier" last="Herbinet">Olivier Herbinet</name>
<affiliation wicri:level="3"><nlm:aff id="A1">KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy, France</nlm:aff>
<country xml:lang="fr">France</country>
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</author>
<author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name>
<affiliation wicri:level="3"><nlm:aff id="A1">KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy, France</nlm:aff>
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</author>
<author><name sortKey="Schoemaecker, Coralie" sort="Schoemaecker, Coralie" uniqKey="Schoemaecker C" first="Coralie" last="Schoemaecker">Coralie Schoemaecker</name>
<affiliation wicri:level="3"><nlm:aff id="A2">PhysicoChimie des Processus de Combustion et de l’Atmosphère PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France</nlm:aff>
<country xml:lang="fr">France</country>
<wicri:regionArea>PhysicoChimie des Processus de Combustion et de l’Atmosphère PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq</wicri:regionArea>
<placeName><region type="region" nuts="2">Hauts-de-France</region>
<region type="old region" nuts="2">Nord-Pas-de-Calais</region>
<settlement type="city">Villeneuve d’Ascq</settlement>
</placeName>
</affiliation>
</author>
<author><name sortKey="Fittschen, Christa" sort="Fittschen, Christa" uniqKey="Fittschen C" first="Christa" last="Fittschen">Christa Fittschen</name>
<affiliation wicri:level="3"><nlm:aff id="A2">PhysicoChimie des Processus de Combustion et de l’Atmosphère PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France</nlm:aff>
<country xml:lang="fr">France</country>
<wicri:regionArea>PhysicoChimie des Processus de Combustion et de l’Atmosphère PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq</wicri:regionArea>
<placeName><region type="region" nuts="2">Hauts-de-France</region>
<region type="old region" nuts="2">Nord-Pas-de-Calais</region>
<settlement type="city">Villeneuve d’Ascq</settlement>
</placeName>
</affiliation>
</author>
<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
<affiliation wicri:level="3"><nlm:aff id="A1">KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy, France</nlm:aff>
<country xml:lang="fr">France</country>
<wicri:regionArea>KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy</wicri:regionArea>
<placeName><region type="region" nuts="2">Grand Est</region>
<region type="old region" nuts="2">Lorraine (région)</region>
<settlement type="city">Nancy</settlement>
</placeName>
<placeName><settlement type="city">Nancy</settlement>
<region type="region" nuts="2">Grand Est</region>
<region type="region" nuts="2">Lorraine (région)</region>
</placeName>
<orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName>
<orgName type="university">Université de Lorraine</orgName>
<orgName type="institution">Centre national de la recherche scientifique</orgName>
</affiliation>
</author>
</analytic>
<series><title level="j">Chemical physics letters</title>
<idno type="ISSN">0009-2614</idno>
<imprint><date when="2012">2012</date>
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<front><div type="abstract" xml:lang="en"><p id="P1">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH<sub>4</sub>
, H<sub>2</sub>
O and CH<sub>2</sub>
O) have been quantified through their well structured spectra around 1506 nm, while H<sub>2</sub>
O<sub>2</sub>
 and HO<sub>2</sub>
 radicals could not be detected.</p>
</div>
</front>
</TEI>
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Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

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