LrgpV1, Pmc, Corpus, bibRecord, 000161

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Identifieur interne : 000161 ( Pmc/Corpus ); précédent : 000160; suivant : 000162

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-Leclerc

Source :

Chemical physics letters [ 0009-2614 ] ; 2012.

RBID : PMC:3662210

Abstract

We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH₄, H₂O and CH₂O) have been quantified through their well structured spectra around 1506 nm, while H₂O₂ and HO₂ radicals could not be detected.

Url:

http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3662210

DOI: 10.1016/j.cplett.2012.03.012
PubMed: 23710075
PubMed Central: 3662210

Links to Exploration step

PMC:3662210

Le document en format XML

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<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
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<author><name sortKey="Fittschen, Christa" sort="Fittschen, Christa" uniqKey="Fittschen C" first="Christa" last="Fittschen">Christa Fittschen</name>
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<front><div type="abstract" xml:lang="en"><p id="P1">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH<sub>4</sub>
, H<sub>2</sub>
O and CH<sub>2</sub>
O) have been quantified through their well structured spectra around 1506 nm, while H<sub>2</sub>
O<sub>2</sub>
 and HO<sub>2</sub>
 radicals could not be detected.</p>
</div>
</front>
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<article-categories><subj-group subj-group-type="heading"><subject>Article</subject>
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<title-group><article-title>Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS</article-title>
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<contrib-group><contrib contrib-type="author"><name><surname>Bahrini</surname>
<given-names>Chiheb</given-names>
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<contrib contrib-type="author"><name><surname>Herbinet</surname>
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<contrib contrib-type="author"><name><surname>Glaude</surname>
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<aff id="A1"><label>a</label>
KINCOM ‘Kinetics of Combustion’, CNRS – LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy, France</aff>
<aff id="A2"><label>b</label>
PhysicoChimie des Processus de Combustion et de l’Atmosphère PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France</aff>
<author-notes><corresp id="CR1"><bold>Corresponding author</bold>
: Christa Fittschen, PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France, <email>christa.fittschen@univ-lille1.fr</email>
, Tel : + 33 (0)3 20 33 72 66, Fax : + 33 (0)3 20 43 69 77</corresp>
</author-notes>
<pub-date pub-type="nihms-submitted"><day>16</day>
<month>5</month>
<year>2013</year>
</pub-date>
<pub-date pub-type="ppub"><day>1</day>
<month>5</month>
<year>2012</year>
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<pub-date pub-type="pmc-release"><day>23</day>
<month>5</month>
<year>2013</year>
</pub-date>
<volume>534</volume>
<fpage>1</fpage>
<lpage>7</lpage>
<self-uri xlink:href="http://www.sciencedirect.com/science/article/pii/S0009261412003077"></self-uri>
<abstract><p id="P1">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH<sub>4</sub>
, H<sub>2</sub>
O and CH<sub>2</sub>
O) have been quantified through their well structured spectra around 1506 nm, while H<sub>2</sub>
O<sub>2</sub>
 and HO<sub>2</sub>
 radicals could not be detected.</p>
</abstract>
<funding-group><award-group><funding-source country="International">European Research Council : </funding-source>
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</award-group>
</funding-group>
</article-meta>
</front>
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Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Source :

Abstract

Links to Exploration step

Le document en format XML

Pour manipuler ce document sous Unix (Dilib)

Pour mettre un lien sur cette page dans le réseau Wicri

Pour générer des pages wiki