LrgpV1, Hal, Corpus, bibRecord, 000315

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Identifieur interne : 000315 ( Hal/Corpus ); précédent : 000314; suivant : 000316

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-Leclerc

Source :

Chemical Physics Letters [ 0009-2614 ] ; 2012-05-01.

RBID : Hal:hal-00726381

English descriptors

mix :
- cw-CRDS, formaldehyde, jet-stirred reactor, methane.

Abstract

We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.

Url:

https://hal.archives-ouvertes.fr/hal-00726381

DOI: 10.1016/j.cplett.2012.03.012

Links to Exploration step

Hal:hal-00726381

Le document en format XML

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<front><div type="abstract" xml:lang="en">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.</div>
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<funder>This work was supported by the European Commission ('Clean ICE' ERC Advanced Research Grant) and the COST Action CM0901 (EU).</funder>
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Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

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