LrgpV1, Pmc, Checkpoint, bibRecord, 000057

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Identifieur interne : 000057 ( Pmc/Checkpoint ); précédent : 000056; suivant : 000058

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Auteurs : Chiheb Bahrini [France] ; Olivier Herbinet [France] ; Pierre-Alexandre Glaude [France] ; Coralie Schoemaecker [France] ; Christa Fittschen [France] ; Frédérique Battin-Leclerc [France]

Source :

Chemical physics letters [ 0009-2614 ] ; 2012.

RBID : PMC:3662210

Abstract

We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH₄, H₂O and CH₂O) have been quantified through their well structured spectra around 1506 nm, while H₂O₂ and HO₂ radicals could not be detected.

Url:

http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3662210

DOI: 10.1016/j.cplett.2012.03.012
PubMed: 23710075
PubMed Central: 3662210

Affiliations:

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PMC:3662210

Le document en format XML

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<front><div type="abstract" xml:lang="en"><p id="P1">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH<sub>4</sub>
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: Christa Fittschen, PC2A, University Lille 1, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France, <email>christa.fittschen@univ-lille1.fr</email>
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<abstract><p id="P1">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH<sub>4</sub>
, H<sub>2</sub>
O and CH<sub>2</sub>
O) have been quantified through their well structured spectra around 1506 nm, while H<sub>2</sub>
O<sub>2</sub>
 and HO<sub>2</sub>
 radicals could not be detected.</p>
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<funding-group><award-group><funding-source country="International">European Research Council : </funding-source>
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Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS

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Abstract

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