ThuliumV1, Pascal, Curation, bibRecord, 000F55

Thulium-doped Ca4GdO(BO3)3 crystals. An investigation of radiative and non-radiative processes

Identifieur interne : 000F55 ( Pascal/Curation ); précédent : 000F54; suivant : 000F56

Thulium-doped Ca4GdO(BO3)3 crystals. An investigation of radiative and non-radiative processes

Auteurs : G. Dominiak-Dzik [Pologne] ; W. Ryba-Romanowski [Pologne] ; S. Gołab [Pologne] ; A. Pajaczkowska [Pologne]

Source :

Journal of physics. Condensed matter : (Print) [ 0953-8984 ] ; 2000.

RBID : Pascal:00-0356364

Descripteurs français

Pascal (Inist)
- Etude expérimentale, Spectre absorption, Photoluminescence, Dépendance température, Champ cristallin, Fluorescence, Déclin luminescence, Effet Judd Ofelt, Processus n phonons, Matériau dopé, Addition thulium, Calcium composé, Gadolinium composé, Borate, Oxyde, Composé quaternaire, Ca4GdO(BO3)3:Tm, B Ca Gd O, 7820C, 7855H.
Wicri :
- topic : Oxyde.

English descriptors

KwdEn :
- Absorption spectra, Borates, Calcium compounds, Crystal field, Doped materials, Experimental study, Fluorescence, Gadolinium compounds, Judd Ofelt effect, Luminescence decay, Multi-phonon processes, Oxides, Photoluminescence, Quaternary compounds, Temperature dependence, Thulium additions.

Abstract

An extensive investigation of optical properties was carried out for Tm³⁺-doped Ca₄GdO(BO₃)₃ crystals in the 5-300 K temperature range. Based on absorption and emission spectra at 5 K, crystal field levels of active ions have been located. Non-equivalent sites for Tm³⁺ in the Ca₄GdO(BO₃)₃ matrix have been demonstrated. Lifetimes and the fluorescence dynamics were studied as a function of temperature and concentration of thulium ions. The Judd-Ofelt analysis of absorption spectra and the Inokuti-Hirayama model for energy transfer between activator ions provided information on radiative processes and non-radiative relaxation of excited states. Additionally, multiphonon emission was taken into account to explain a very strong quenching of the ³H₄ and the ³F₄ fluorescence.

A01	`01`	`1`		`@0 0953-8984`
A02	`01`			`@0 JCOMEL`
A03		`1`		`@0 J. phys., Condens. matter : (Print)`
A05				`@2 12`
A06				`@2 25`
A08	`01`	`1`	`ENG`	`@1 Thulium-doped Ca₄GdO(BO₃)₃ crystals. An investigation of radiative and non-radiative processes`
A11	`01`	`1`		`@1 DOMINIAK-DZIK (G.)`
A11	`02`	`1`		`@1 RYBA-ROMANOWSKI (W.)`
A11	`03`	`1`		`@1 GOŁAB (S.)`
A11	`04`	`1`		`@1 PAJACZKOWSKA (A.)`
A14	`01`			`@1 Institute of Low Temperature and Structure Research, Polish Academy of Sciences, 2 Okólna Street @2 50-950 Wrocław @3 POL @Z 1 aut. @Z 2 aut. @Z 3 aut.`
A14	`02`			`@1 Institute of Electronic Materials Technology, 133 Wólczyńska Street @2 01-919 Warsaw @3 POL @Z 4 aut.`
A20				`@1 5495-5505`
A21				`@1 2000`
A23	`01`			`@0 ENG`
A43	`01`			`@1 INIST @2 577E2 @5 354000088843560200`
A44				`@0 0000 @1 © 2000 INIST-CNRS. All rights reserved.`
A45				`@0 21 ref.`
A47	`01`	`1`		`@0 00-0356364`
A60				`@1 P`
A61				`@0 A`
A64	`01`	`1`		`@0 Journal of physics. Condensed matter : (Print)`
A66	`01`			`@0 GBR`
C01	`01`		`ENG`	@0 An extensive investigation of optical properties was carried out for Tm³⁺-doped Ca₄GdO(BO₃)₃ crystals in the 5-300 K temperature range. Based on absorption and emission spectra at 5 K, crystal field levels of active ions have been located. Non-equivalent sites for Tm³⁺ in the Ca₄GdO(BO₃)₃ matrix have been demonstrated. Lifetimes and the fluorescence dynamics were studied as a function of temperature and concentration of thulium ions. The Judd-Ofelt analysis of absorption spectra and the Inokuti-Hirayama model for energy transfer between activator ions provided information on radiative processes and non-radiative relaxation of excited states. Additionally, multiphonon emission was taken into account to explain a very strong quenching of the ³H₄ and the ³F₄ fluorescence.
C02	`01`	`3`		`@0 001B70H20C`
C02	`02`	`3`		`@0 001B70H55H`
C03	`01`	`3`	`FRE`	`@0 Etude expérimentale @5 01`
C03	`01`	`3`	`ENG`	`@0 Experimental study @5 01`
C03	`02`	`3`	`FRE`	`@0 Spectre absorption @5 02`
C03	`02`	`3`	`ENG`	`@0 Absorption spectra @5 02`
C03	`03`	`3`	`FRE`	`@0 Photoluminescence @5 03`
C03	`03`	`3`	`ENG`	`@0 Photoluminescence @5 03`
C03	`04`	`3`	`FRE`	`@0 Dépendance température @5 04`
C03	`04`	`3`	`ENG`	`@0 Temperature dependence @5 04`
C03	`05`	`3`	`FRE`	`@0 Champ cristallin @5 05`
C03	`05`	`3`	`ENG`	`@0 Crystal field @5 05`
C03	`06`	`3`	`FRE`	`@0 Fluorescence @5 06`
C03	`06`	`3`	`ENG`	`@0 Fluorescence @5 06`
C03	`07`	`X`	`FRE`	`@0 Déclin luminescence @5 07`
C03	`07`	`X`	`ENG`	`@0 Luminescence decay @5 07`
C03	`07`	`X`	`SPA`	`@0 Decadencia luminiscencia @5 07`
C03	`08`	`X`	`FRE`	`@0 Effet Judd Ofelt @5 08`
C03	`08`	`X`	`ENG`	`@0 Judd Ofelt effect @5 08`
C03	`08`	`X`	`SPA`	`@0 Efecto Judd Ofelt @5 08`
C03	`09`	`3`	`FRE`	`@0 Processus n phonons @5 09`
C03	`09`	`3`	`ENG`	`@0 Multi-phonon processes @5 09`
C03	`10`	`3`	`FRE`	`@0 Matériau dopé @5 11`
C03	`10`	`3`	`ENG`	`@0 Doped materials @5 11`
C03	`11`	`3`	`FRE`	`@0 Addition thulium @5 12`
C03	`11`	`3`	`ENG`	`@0 Thulium additions @5 12`
C03	`12`	`3`	`FRE`	`@0 Calcium composé @5 13`
C03	`12`	`3`	`ENG`	`@0 Calcium compounds @5 13`
C03	`13`	`3`	`FRE`	`@0 Gadolinium composé @5 14`
C03	`13`	`3`	`ENG`	`@0 Gadolinium compounds @5 14`
C03	`14`	`3`	`FRE`	`@0 Borate @2 NA @5 15`
C03	`14`	`3`	`ENG`	`@0 Borates @2 NA @5 15`
C03	`15`	`3`	`FRE`	`@0 Oxyde @5 16`
C03	`15`	`3`	`ENG`	`@0 Oxides @5 16`
C03	`16`	`3`	`FRE`	`@0 Composé quaternaire @5 17`
C03	`16`	`3`	`ENG`	`@0 Quaternary compounds @5 17`
C03	`17`	`3`	`FRE`	`@0 Ca4GdO(BO3)3:Tm @4 INC @5 52`
C03	`18`	`3`	`FRE`	`@0 B Ca Gd O @4 INC @5 53`
C03	`19`	`3`	`FRE`	`@0 7820C @2 PAC @4 INC @5 56`
C03	`20`	`3`	`FRE`	`@0 7855H @2 PAC @4 INC @5 57`
C07	`01`	`3`	`FRE`	`@0 Composé minéral @5 48`
C07	`01`	`3`	`ENG`	`@0 Inorganic compounds @5 48`
C07	`02`	`3`	`FRE`	`@0 Lanthanide composé @5 49`
C07	`02`	`3`	`ENG`	`@0 Rare earth compounds @5 49`
N21				`@1 248`

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Le document en format XML

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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Thulium-doped Ca<sub>4</sub>
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<author><name sortKey="Ryba Romanowski, W" sort="Ryba Romanowski, W" uniqKey="Ryba Romanowski W" first="W." last="Ryba-Romanowski">W. Ryba-Romanowski</name>
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<author><name sortKey="Golab, S" sort="Golab, S" uniqKey="Golab S" first="S." last="Gołab">S. Gołab</name>
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<term>Doped materials</term>
<term>Experimental study</term>
<term>Fluorescence</term>
<term>Gadolinium compounds</term>
<term>Judd Ofelt effect</term>
<term>Luminescence decay</term>
<term>Multi-phonon processes</term>
<term>Oxides</term>
<term>Photoluminescence</term>
<term>Quaternary compounds</term>
<term>Temperature dependence</term>
<term>Thulium additions</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Etude expérimentale</term>
<term>Spectre absorption</term>
<term>Photoluminescence</term>
<term>Dépendance température</term>
<term>Champ cristallin</term>
<term>Fluorescence</term>
<term>Déclin luminescence</term>
<term>Effet Judd Ofelt</term>
<term>Processus n phonons</term>
<term>Matériau dopé</term>
<term>Addition thulium</term>
<term>Calcium composé</term>
<term>Gadolinium composé</term>
<term>Borate</term>
<term>Oxyde</term>
<term>Composé quaternaire</term>
<term>Ca4GdO(BO3)3:Tm</term>
<term>B Ca Gd O</term>
<term>7820C</term>
<term>7855H</term>
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<front><div type="abstract" xml:lang="en">An extensive investigation of optical properties was carried out for Tm<sup>3+</sup>
-doped Ca<sub>4</sub>
GdO(BO<sub>3</sub>
)<sub>3</sub>
 crystals in the 5-300 K temperature range. Based on absorption and emission spectra at 5 K, crystal field levels of active ions have been located. Non-equivalent sites for Tm<sup>3+</sup>
 in the Ca<sub>4</sub>
GdO(BO<sub>3</sub>
)<sub>3</sub>
 matrix have been demonstrated. Lifetimes and the fluorescence dynamics were studied as a function of temperature and concentration of thulium ions. The Judd-Ofelt analysis of absorption spectra and the Inokuti-Hirayama model for energy transfer between activator ions provided information on radiative processes and non-radiative relaxation of excited states. Additionally, multiphonon emission was taken into account to explain a very strong quenching of the <sup>3</sup>
H<sub>4</sub>
 and the <sup>3</sup>
F<sub>4</sub>
 fluorescence.</div>
</front>
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 crystals. An investigation of radiative and non-radiative processes</s1>
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<fA11 i1="01" i2="1"><s1>DOMINIAK-DZIK (G.)</s1>
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</fA11>
<fA14 i1="01"><s1>Institute of Low Temperature and Structure Research, Polish Academy of Sciences, 2 Okólna Street</s1>
<s2>50-950 Wrocław</s2>
<s3>POL</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
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<fC01 i1="01" l="ENG"><s0>An extensive investigation of optical properties was carried out for Tm<sup>3+</sup>
-doped Ca<sub>4</sub>
GdO(BO<sub>3</sub>
)<sub>3</sub>
 crystals in the 5-300 K temperature range. Based on absorption and emission spectra at 5 K, crystal field levels of active ions have been located. Non-equivalent sites for Tm<sup>3+</sup>
 in the Ca<sub>4</sub>
GdO(BO<sub>3</sub>
)<sub>3</sub>
 matrix have been demonstrated. Lifetimes and the fluorescence dynamics were studied as a function of temperature and concentration of thulium ions. The Judd-Ofelt analysis of absorption spectra and the Inokuti-Hirayama model for energy transfer between activator ions provided information on radiative processes and non-radiative relaxation of excited states. Additionally, multiphonon emission was taken into account to explain a very strong quenching of the <sup>3</sup>
H<sub>4</sub>
 and the <sup>3</sup>
F<sub>4</sub>
 fluorescence.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001B70H20C</s0>
</fC02>
<fC02 i1="02" i2="3"><s0>001B70H55H</s0>
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<s5>01</s5>
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<fC03 i1="01" i2="3" l="ENG"><s0>Experimental study</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="3" l="FRE"><s0>Spectre absorption</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="3" l="ENG"><s0>Absorption spectra</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="3" l="FRE"><s0>Photoluminescence</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="3" l="ENG"><s0>Photoluminescence</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Dépendance température</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Temperature dependence</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="3" l="FRE"><s0>Champ cristallin</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="3" l="ENG"><s0>Crystal field</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="3" l="FRE"><s0>Fluorescence</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="3" l="ENG"><s0>Fluorescence</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Déclin luminescence</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Luminescence decay</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Decadencia luminiscencia</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Effet Judd Ofelt</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Judd Ofelt effect</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Efecto Judd Ofelt</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="3" l="FRE"><s0>Processus n phonons</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="3" l="ENG"><s0>Multi-phonon processes</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Matériau dopé</s0>
<s5>11</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>Doped materials</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="3" l="FRE"><s0>Addition thulium</s0>
<s5>12</s5>
</fC03>
<fC03 i1="11" i2="3" l="ENG"><s0>Thulium additions</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="3" l="FRE"><s0>Calcium composé</s0>
<s5>13</s5>
</fC03>
<fC03 i1="12" i2="3" l="ENG"><s0>Calcium compounds</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="3" l="FRE"><s0>Gadolinium composé</s0>
<s5>14</s5>
</fC03>
<fC03 i1="13" i2="3" l="ENG"><s0>Gadolinium compounds</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="3" l="FRE"><s0>Borate</s0>
<s2>NA</s2>
<s5>15</s5>
</fC03>
<fC03 i1="14" i2="3" l="ENG"><s0>Borates</s0>
<s2>NA</s2>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>Oxyde</s0>
<s5>16</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>Oxides</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="3" l="FRE"><s0>Composé quaternaire</s0>
<s5>17</s5>
</fC03>
<fC03 i1="16" i2="3" l="ENG"><s0>Quaternary compounds</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="3" l="FRE"><s0>Ca4GdO(BO3)3:Tm</s0>
<s4>INC</s4>
<s5>52</s5>
</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>B Ca Gd O</s0>
<s4>INC</s4>
<s5>53</s5>
</fC03>
<fC03 i1="19" i2="3" l="FRE"><s0>7820C</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>56</s5>
</fC03>
<fC03 i1="20" i2="3" l="FRE"><s0>7855H</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>57</s5>
</fC03>
<fC07 i1="01" i2="3" l="FRE"><s0>Composé minéral</s0>
<s5>48</s5>
</fC07>
<fC07 i1="01" i2="3" l="ENG"><s0>Inorganic compounds</s0>
<s5>48</s5>
</fC07>
<fC07 i1="02" i2="3" l="FRE"><s0>Lanthanide composé</s0>
<s5>49</s5>
</fC07>
<fC07 i1="02" i2="3" l="ENG"><s0>Rare earth compounds</s0>
<s5>49</s5>
</fC07>
<fN21><s1>248</s1>
</fN21>
</pA>
</standard>
</inist>
</record>

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Thulium-doped Ca4GdO(BO3)3 crystals. An investigation of radiative and non-radiative processes

Thulium-doped Ca4GdO(BO3)3 crystals. An investigation of radiative and non-radiative processes

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