ThuliumV1, Pascal, Curation, bibRecord, 000A54

Optical spectroscopy of Ho3+ and Tm3+ in Ca3Sc2Ge3O12 crystals

Identifieur interne : 000A54 ( Pascal/Curation ); précédent : 000A53; suivant : 000A55

Optical spectroscopy of Ho3+ and Tm3+ in Ca3Sc2Ge3O12 crystals

Auteurs : Enrico Cavalli [Italie] ; Alessandro Belletti [Italie] ; Stefano Bigotta [Italie] ; Alessandra Toncelli [Italie] ; Mauro Tonelli [Italie]

Source :

Journal of alloys and compounds [ 0925-8388 ] ; 2004.

RBID : Pascal:04-0236865

Descripteurs français

Pascal (Inist)
- Photoluminescence, Spectre absorption, Déclin luminescence, Etat excité, Effet Judd Ofelt, Rapport branchement, Durée vie radiative, Impureté, Emission spontanée, Addition holmium, Addition thulium, Monocristal, Grenats, Calcium Germanate, Scandium Germanate, Composé quaternaire, Etude expérimentale, Ca3Sc2Ge3O12:Ho Tm, Ca Ge O Sc, 7855H.

English descriptors

KwdEn :
- Absorption spectra, Branching ratio, Calcium Germanates, Excited states, Experimental study, Garnets, Holmium additions, Impurities, Judd Ofelt effect, Luminescence decay, Monocrystals, Photoluminescence, Quaternary compounds, Radiative lifetimes, Scandium Germanates, Spontaneous emission, Thulium additions.

Abstract

Single crystals of the Ca₃Sc₂Ge₃O₁₂ (CaSGG) garnet activated with Ho³⁺ and Tm³⁺ have been grown by the 'flux growth' technique. The absorption spectra, the visible emission properties and the decay curves of the excited states have been measured at 10 and 298 K. The room temperature absorption spectra have been analyzed in the framework of the Judd-Ofelt theory and the intensity parameters have been evaluated. The spontaneous transition probabilities, the branching ratios and the radiative lifetimes have been determined for the most important emitting states using the calculated intensity parameters, and the results have been compared with the experimental data in order to estimate the efficiency of the non-radiative processes.

A01	`01`	`1`		`@0 0925-8388`
A03		`1`		`@0 J. alloys compd.`
A05				`@2 365`
A08	`01`	`1`	`ENG`	`@1 Optical spectroscopy of Ho³⁺ and Tm³⁺ in Ca₃Sc₂Ge₃O₁₂ crystals`
A11	`01`	`1`		`@1 CAVALLI (Enrico)`
A11	`02`	`1`		`@1 BELLETTI (Alessandro)`
A11	`03`	`1`		`@1 BIGOTTA (Stefano)`
A11	`04`	`1`		`@1 TONCELLI (Alessandra)`
A11	`05`	`1`		`@1 TONELLI (Mauro)`
A14	`01`			`@1 INFM and Dipartimento di Chimica Generale ed Inorganica, Chimica Analitica e Chimica Fisica, Università di Parma, Viale delle Scienze 17/a @2 43100 Parma @3 ITA @Z 1 aut. @Z 2 aut.`
A14	`02`			`@1 INFM-NEST and Dipartimento di Fisica, University di Pisa, Via Buonarroti 2 @2 56127 Pisa @3 ITA @Z 3 aut. @Z 4 aut. @Z 5 aut.`
A20				`@1 1-7`
A21				`@1 2004`
A23	`01`			`@0 ENG`
A43	`01`			`@1 INIST @2 1151 @5 354000119288850030`
A44				`@0 0000 @1 © 2004 INIST-CNRS. All rights reserved.`
A45				`@0 16 ref.`
A47	`01`	`1`		`@0 04-0236865`
A60				`@1 P`
A61				`@0 A`
A64	`01`	`1`		`@0 Journal of alloys and compounds`
A66	`01`			`@0 CHE`
C01	`01`		`ENG`	@0 Single crystals of the Ca₃Sc₂Ge₃O₁₂ (CaSGG) garnet activated with Ho³⁺ and Tm³⁺ have been grown by the 'flux growth' technique. The absorption spectra, the visible emission properties and the decay curves of the excited states have been measured at 10 and 298 K. The room temperature absorption spectra have been analyzed in the framework of the Judd-Ofelt theory and the intensity parameters have been evaluated. The spontaneous transition probabilities, the branching ratios and the radiative lifetimes have been determined for the most important emitting states using the calculated intensity parameters, and the results have been compared with the experimental data in order to estimate the efficiency of the non-radiative processes.
C02	`01`	`3`		`@0 001B70H55H`
C03	`01`	`3`	`FRE`	`@0 Photoluminescence @5 02`
C03	`01`	`3`	`ENG`	`@0 Photoluminescence @5 02`
C03	`02`	`3`	`FRE`	`@0 Spectre absorption @5 03`
C03	`02`	`3`	`ENG`	`@0 Absorption spectra @5 03`
C03	`03`	`X`	`FRE`	`@0 Déclin luminescence @5 05`
C03	`03`	`X`	`ENG`	`@0 Luminescence decay @5 05`
C03	`03`	`X`	`SPA`	`@0 Decadencia luminiscencia @5 05`
C03	`04`	`3`	`FRE`	`@0 Etat excité @5 06`
C03	`04`	`3`	`ENG`	`@0 Excited states @5 06`
C03	`05`	`X`	`FRE`	`@0 Effet Judd Ofelt @5 07`
C03	`05`	`X`	`ENG`	`@0 Judd Ofelt effect @5 07`
C03	`05`	`X`	`SPA`	`@0 Efecto Judd Ofelt @5 07`
C03	`06`	`3`	`FRE`	`@0 Rapport branchement @5 08`
C03	`06`	`3`	`ENG`	`@0 Branching ratio @5 08`
C03	`07`	`3`	`FRE`	`@0 Durée vie radiative @5 09`
C03	`07`	`3`	`ENG`	`@0 Radiative lifetimes @5 09`
C03	`08`	`3`	`FRE`	`@0 Impureté @5 10`
C03	`08`	`3`	`ENG`	`@0 Impurities @5 10`
C03	`09`	`3`	`FRE`	`@0 Emission spontanée @5 11`
C03	`09`	`3`	`ENG`	`@0 Spontaneous emission @5 11`
C03	`10`	`3`	`FRE`	`@0 Addition holmium @5 12`
C03	`10`	`3`	`ENG`	`@0 Holmium additions @5 12`
C03	`11`	`3`	`FRE`	`@0 Addition thulium @5 13`
C03	`11`	`3`	`ENG`	`@0 Thulium additions @5 13`
C03	`12`	`3`	`FRE`	`@0 Monocristal @5 15`
C03	`12`	`3`	`ENG`	`@0 Monocrystals @5 15`
C03	`13`	`3`	`FRE`	`@0 Grenats @5 16`
C03	`13`	`3`	`ENG`	`@0 Garnets @5 16`
C03	`14`	`3`	`FRE`	`@0 Calcium Germanate @2 NC @2 NA @5 17`
C03	`14`	`3`	`ENG`	`@0 Calcium Germanates @2 NC @2 NA @5 17`
C03	`15`	`3`	`FRE`	`@0 Scandium Germanate @2 NC @2 NA @5 18`
C03	`15`	`3`	`ENG`	`@0 Scandium Germanates @2 NC @2 NA @5 18`
C03	`16`	`3`	`FRE`	`@0 Composé quaternaire @5 19`
C03	`16`	`3`	`ENG`	`@0 Quaternary compounds @5 19`
C03	`17`	`3`	`FRE`	`@0 Etude expérimentale @5 20`
C03	`17`	`3`	`ENG`	`@0 Experimental study @5 20`
C03	`18`	`3`	`FRE`	`@0 Ca3Sc2Ge3O12:Ho Tm @4 INC @5 53`
C03	`19`	`3`	`FRE`	`@0 Ca Ge O Sc @4 INC @5 54`
C03	`20`	`3`	`FRE`	`@0 7855H @4 INC @5 56`
C07	`01`	`3`	`FRE`	`@0 Composé minéral @5 48`
C07	`01`	`3`	`ENG`	`@0 Inorganic compounds @5 48`
N21				`@1 152`
N82				`@1 PSI`

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Le document en format XML

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 and Tm<sup>3+</sup>
 in Ca<sub>3</sub>
Sc<sub>2</sub>
Ge<sub>3</sub>
O<sub>12</sub>
 crystals</title>
<author><name sortKey="Cavalli, Enrico" sort="Cavalli, Enrico" uniqKey="Cavalli E" first="Enrico" last="Cavalli">Enrico Cavalli</name>
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<author><name sortKey="Tonelli, Mauro" sort="Tonelli, Mauro" uniqKey="Tonelli M" first="Mauro" last="Tonelli">Mauro Tonelli</name>
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Optical spectroscopy of Ho<sup>3+</sup>
 and Tm<sup>3+</sup>
 in Ca<sub>3</sub>
Sc<sub>2</sub>
Ge<sub>3</sub>
O<sub>12</sub>
 crystals</title>
<author><name sortKey="Cavalli, Enrico" sort="Cavalli, Enrico" uniqKey="Cavalli E" first="Enrico" last="Cavalli">Enrico Cavalli</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>INFM and Dipartimento di Chimica Generale ed Inorganica, Chimica Analitica e Chimica Fisica, Università di Parma, Viale delle Scienze 17/a</s1>
<s2>43100 Parma</s2>
<s3>ITA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
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<country>Italie</country>
</affiliation>
</author>
<author><name sortKey="Belletti, Alessandro" sort="Belletti, Alessandro" uniqKey="Belletti A" first="Alessandro" last="Belletti">Alessandro Belletti</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>INFM and Dipartimento di Chimica Generale ed Inorganica, Chimica Analitica e Chimica Fisica, Università di Parma, Viale delle Scienze 17/a</s1>
<s2>43100 Parma</s2>
<s3>ITA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</inist:fA14>
<country>Italie</country>
</affiliation>
</author>
<author><name sortKey="Bigotta, Stefano" sort="Bigotta, Stefano" uniqKey="Bigotta S" first="Stefano" last="Bigotta">Stefano Bigotta</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>INFM-NEST and Dipartimento di Fisica, University di Pisa, Via Buonarroti 2</s1>
<s2>56127 Pisa</s2>
<s3>ITA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</inist:fA14>
<country>Italie</country>
</affiliation>
</author>
<author><name sortKey="Toncelli, Alessandra" sort="Toncelli, Alessandra" uniqKey="Toncelli A" first="Alessandra" last="Toncelli">Alessandra Toncelli</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>INFM-NEST and Dipartimento di Fisica, University di Pisa, Via Buonarroti 2</s1>
<s2>56127 Pisa</s2>
<s3>ITA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</inist:fA14>
<country>Italie</country>
</affiliation>
</author>
<author><name sortKey="Tonelli, Mauro" sort="Tonelli, Mauro" uniqKey="Tonelli M" first="Mauro" last="Tonelli">Mauro Tonelli</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>INFM-NEST and Dipartimento di Fisica, University di Pisa, Via Buonarroti 2</s1>
<s2>56127 Pisa</s2>
<s3>ITA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</inist:fA14>
<country>Italie</country>
</affiliation>
</author>
</analytic>
<series><title level="j" type="main">Journal of alloys and compounds</title>
<title level="j" type="abbreviated">J. alloys compd.</title>
<idno type="ISSN">0925-8388</idno>
<imprint><date when="2004">2004</date>
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</series>
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<seriesStmt><title level="j" type="main">Journal of alloys and compounds</title>
<title level="j" type="abbreviated">J. alloys compd.</title>
<idno type="ISSN">0925-8388</idno>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Absorption spectra</term>
<term>Branching ratio</term>
<term>Calcium Germanates</term>
<term>Excited states</term>
<term>Experimental study</term>
<term>Garnets</term>
<term>Holmium additions</term>
<term>Impurities</term>
<term>Judd Ofelt effect</term>
<term>Luminescence decay</term>
<term>Monocrystals</term>
<term>Photoluminescence</term>
<term>Quaternary compounds</term>
<term>Radiative lifetimes</term>
<term>Scandium Germanates</term>
<term>Spontaneous emission</term>
<term>Thulium additions</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Photoluminescence</term>
<term>Spectre absorption</term>
<term>Déclin luminescence</term>
<term>Etat excité</term>
<term>Effet Judd Ofelt</term>
<term>Rapport branchement</term>
<term>Durée vie radiative</term>
<term>Impureté</term>
<term>Emission spontanée</term>
<term>Addition holmium</term>
<term>Addition thulium</term>
<term>Monocristal</term>
<term>Grenats</term>
<term>Calcium Germanate</term>
<term>Scandium Germanate</term>
<term>Composé quaternaire</term>
<term>Etude expérimentale</term>
<term>Ca3Sc2Ge3O12:Ho Tm</term>
<term>Ca Ge O Sc</term>
<term>7855H</term>
</keywords>
</textClass>
</profileDesc>
</teiHeader>
<front><div type="abstract" xml:lang="en">Single crystals of the Ca<sub>3</sub>
Sc<sub>2</sub>
Ge<sub>3</sub>
O<sub>12</sub>
 (CaSGG) garnet activated with Ho<sup>3+</sup>
 and Tm<sup>3+</sup>
 have been grown by the 'flux growth' technique. The absorption spectra, the visible emission properties and the decay curves of the excited states have been measured at 10 and 298 K. The room temperature absorption spectra have been analyzed in the framework of the Judd-Ofelt theory and the intensity parameters have been evaluated. The spontaneous transition probabilities, the branching ratios and the radiative lifetimes have been determined for the most important emitting states using the calculated intensity parameters, and the results have been compared with the experimental data in order to estimate the efficiency of the non-radiative processes.</div>
</front>
</TEI>
<inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0925-8388</s0>
</fA01>
<fA03 i2="1"><s0>J. alloys compd.</s0>
</fA03>
<fA05><s2>365</s2>
</fA05>
<fA08 i1="01" i2="1" l="ENG"><s1>Optical spectroscopy of Ho<sup>3+</sup>
 and Tm<sup>3+</sup>
 in Ca<sub>3</sub>
Sc<sub>2</sub>
Ge<sub>3</sub>
O<sub>12</sub>
 crystals</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>CAVALLI (Enrico)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>BELLETTI (Alessandro)</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>BIGOTTA (Stefano)</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>TONCELLI (Alessandra)</s1>
</fA11>
<fA11 i1="05" i2="1"><s1>TONELLI (Mauro)</s1>
</fA11>
<fA14 i1="01"><s1>INFM and Dipartimento di Chimica Generale ed Inorganica, Chimica Analitica e Chimica Fisica, Università di Parma, Viale delle Scienze 17/a</s1>
<s2>43100 Parma</s2>
<s3>ITA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>INFM-NEST and Dipartimento di Fisica, University di Pisa, Via Buonarroti 2</s1>
<s2>56127 Pisa</s2>
<s3>ITA</s3>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</fA14>
<fA20><s1>1-7</s1>
</fA20>
<fA21><s1>2004</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>1151</s2>
<s5>354000119288850030</s5>
</fA43>
<fA44><s0>0000</s0>
<s1>© 2004 INIST-CNRS. All rights reserved.</s1>
</fA44>
<fA45><s0>16 ref.</s0>
</fA45>
<fA47 i1="01" i2="1"><s0>04-0236865</s0>
</fA47>
<fA60><s1>P</s1>
</fA60>
<fA61><s0>A</s0>
</fA61>
<fA64 i1="01" i2="1"><s0>Journal of alloys and compounds</s0>
</fA64>
<fA66 i1="01"><s0>CHE</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>Single crystals of the Ca<sub>3</sub>
Sc<sub>2</sub>
Ge<sub>3</sub>
O<sub>12</sub>
 (CaSGG) garnet activated with Ho<sup>3+</sup>
 and Tm<sup>3+</sup>
 have been grown by the 'flux growth' technique. The absorption spectra, the visible emission properties and the decay curves of the excited states have been measured at 10 and 298 K. The room temperature absorption spectra have been analyzed in the framework of the Judd-Ofelt theory and the intensity parameters have been evaluated. The spontaneous transition probabilities, the branching ratios and the radiative lifetimes have been determined for the most important emitting states using the calculated intensity parameters, and the results have been compared with the experimental data in order to estimate the efficiency of the non-radiative processes.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001B70H55H</s0>
</fC02>
<fC03 i1="01" i2="3" l="FRE"><s0>Photoluminescence</s0>
<s5>02</s5>
</fC03>
<fC03 i1="01" i2="3" l="ENG"><s0>Photoluminescence</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="3" l="FRE"><s0>Spectre absorption</s0>
<s5>03</s5>
</fC03>
<fC03 i1="02" i2="3" l="ENG"><s0>Absorption spectra</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="FRE"><s0>Déclin luminescence</s0>
<s5>05</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Luminescence decay</s0>
<s5>05</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA"><s0>Decadencia luminiscencia</s0>
<s5>05</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Etat excité</s0>
<s5>06</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Excited states</s0>
<s5>06</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE"><s0>Effet Judd Ofelt</s0>
<s5>07</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG"><s0>Judd Ofelt effect</s0>
<s5>07</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA"><s0>Efecto Judd Ofelt</s0>
<s5>07</s5>
</fC03>
<fC03 i1="06" i2="3" l="FRE"><s0>Rapport branchement</s0>
<s5>08</s5>
</fC03>
<fC03 i1="06" i2="3" l="ENG"><s0>Branching ratio</s0>
<s5>08</s5>
</fC03>
<fC03 i1="07" i2="3" l="FRE"><s0>Durée vie radiative</s0>
<s5>09</s5>
</fC03>
<fC03 i1="07" i2="3" l="ENG"><s0>Radiative lifetimes</s0>
<s5>09</s5>
</fC03>
<fC03 i1="08" i2="3" l="FRE"><s0>Impureté</s0>
<s5>10</s5>
</fC03>
<fC03 i1="08" i2="3" l="ENG"><s0>Impurities</s0>
<s5>10</s5>
</fC03>
<fC03 i1="09" i2="3" l="FRE"><s0>Emission spontanée</s0>
<s5>11</s5>
</fC03>
<fC03 i1="09" i2="3" l="ENG"><s0>Spontaneous emission</s0>
<s5>11</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Addition holmium</s0>
<s5>12</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>Holmium additions</s0>
<s5>12</s5>
</fC03>
<fC03 i1="11" i2="3" l="FRE"><s0>Addition thulium</s0>
<s5>13</s5>
</fC03>
<fC03 i1="11" i2="3" l="ENG"><s0>Thulium additions</s0>
<s5>13</s5>
</fC03>
<fC03 i1="12" i2="3" l="FRE"><s0>Monocristal</s0>
<s5>15</s5>
</fC03>
<fC03 i1="12" i2="3" l="ENG"><s0>Monocrystals</s0>
<s5>15</s5>
</fC03>
<fC03 i1="13" i2="3" l="FRE"><s0>Grenats</s0>
<s5>16</s5>
</fC03>
<fC03 i1="13" i2="3" l="ENG"><s0>Garnets</s0>
<s5>16</s5>
</fC03>
<fC03 i1="14" i2="3" l="FRE"><s0>Calcium Germanate</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>17</s5>
</fC03>
<fC03 i1="14" i2="3" l="ENG"><s0>Calcium Germanates</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>17</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>Scandium Germanate</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>18</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>Scandium Germanates</s0>
<s2>NC</s2>
<s2>NA</s2>
<s5>18</s5>
</fC03>
<fC03 i1="16" i2="3" l="FRE"><s0>Composé quaternaire</s0>
<s5>19</s5>
</fC03>
<fC03 i1="16" i2="3" l="ENG"><s0>Quaternary compounds</s0>
<s5>19</s5>
</fC03>
<fC03 i1="17" i2="3" l="FRE"><s0>Etude expérimentale</s0>
<s5>20</s5>
</fC03>
<fC03 i1="17" i2="3" l="ENG"><s0>Experimental study</s0>
<s5>20</s5>
</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>Ca3Sc2Ge3O12:Ho Tm</s0>
<s4>INC</s4>
<s5>53</s5>
</fC03>
<fC03 i1="19" i2="3" l="FRE"><s0>Ca Ge O Sc</s0>
<s4>INC</s4>
<s5>54</s5>
</fC03>
<fC03 i1="20" i2="3" l="FRE"><s0>7855H</s0>
<s4>INC</s4>
<s5>56</s5>
</fC03>
<fC07 i1="01" i2="3" l="FRE"><s0>Composé minéral</s0>
<s5>48</s5>
</fC07>
<fC07 i1="01" i2="3" l="ENG"><s0>Inorganic compounds</s0>
<s5>48</s5>
</fC07>
<fN21><s1>152</s1>
</fN21>
<fN82><s1>PSI</s1>
</fN82>
</pA>
</standard>
</inist>
</record>

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Optical spectroscopy of Ho3+ and Tm3+ in Ca3Sc2Ge3O12 crystals

Optical spectroscopy of Ho3+ and Tm3+ in Ca3Sc2Ge3O12 crystals

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