Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS.
Identifieur interne : 000074 ( PubMed/Curation ); précédent : 000073; suivant : 000075Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS.
Auteurs : Chiheb Bahrini [France] ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-LeclercSource :
- Chemical physics letters [ 0009-2614 ] ; 2012.
Abstract
We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.
DOI: 10.1016/j.cplett.2012.03.012
PubMed: 23710075
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The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.</div></front></TEI><pubmed><MedlineCitation Status="Publisher" Owner="NLM"><PMID Version="1">23710075</PMID><DateCreated><Year>2013</Year><Month>5</Month><Day>27</Day></DateCreated><Article PubModel="Print"><Journal><ISSN IssnType="Print">0009-2614</ISSN><JournalIssue CitedMedium="Print"><Volume>534</Volume><PubDate><Year>2012</Year><Month>May</Month><Day>1</Day></PubDate></JournalIssue><Title>Chemical physics letters</Title><ISOAbbreviation>Chem Phys Lett</ISOAbbreviation></Journal><ArticleTitle>Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS.</ArticleTitle><Pagination><MedlinePgn>1-7</MedlinePgn></Pagination><Abstract><AbstractText>We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.</AbstractText></Abstract><AuthorList><Author><LastName>Bahrini</LastName><ForeName>Chiheb</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>KINCOM 'Kinetics of Combustion', CNRS - LRGP ENSIC, 1, rue Grandville, BP 20451, 54001 Nancy, France.</Affiliation></AffiliationInfo></Author><Author><LastName>Herbinet</LastName><ForeName>Olivier</ForeName><Initials>O</Initials></Author><Author><LastName>Glaude</LastName><ForeName>Pierre-Alexandre</ForeName><Initials>PA</Initials></Author><Author><LastName>Schoemaecker</LastName><ForeName>Coralie</ForeName><Initials>C</Initials></Author><Author><LastName>Fittschen</LastName><ForeName>Christa</ForeName><Initials>C</Initials></Author><Author><LastName>Battin-Leclerc</LastName><ForeName>Frédérique</ForeName><Initials>F</Initials></Author></AuthorList><Language>ENG</Language><GrantList><Grant><GrantID>227669</GrantID><Agency>European Research Council</Agency><Country>International</Country></Grant></GrantList><PublicationTypeList><PublicationType UI="">JOURNAL ARTICLE</PublicationType></PublicationTypeList></Article><MedlineJournalInfo><MedlineTA>Chem Phys Lett</MedlineTA><NlmUniqueID>9882685</NlmUniqueID><ISSNLinking>0009-2614</ISSNLinking></MedlineJournalInfo></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2013</Year><Month>5</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2013</Year><Month>5</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2013</Year><Month>5</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="doi">10.1016/j.cplett.2012.03.012</ArticleId><ArticleId IdType="pubmed">23710075</ArticleId><ArticleId IdType="pmc">PMC3662210</ArticleId><ArticleId IdType="mid">EMS53327</ArticleId></ArticleIdList><pmc-dir>nihms</pmc-dir>
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