Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS.
Identifieur interne : 000074 ( PubMed/Corpus ); précédent : 000073; suivant : 000075Detection of some stable species during the oxidation of methane by coupling a jet-stirred reactor (JSR) to cw-CRDS.
Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-LeclercSource :
- Chemical physics letters [ 0009-2614 ] ; 2012.
Abstract
We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.
DOI: 10.1016/j.cplett.2012.03.012
PubMed: 23710075
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pubmed:23710075Le document en format XML
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<author><name sortKey="Herbinet, Olivier" sort="Herbinet, Olivier" uniqKey="Herbinet O" first="Olivier" last="Herbinet">Olivier Herbinet</name>
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<author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name>
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<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
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<front><div type="abstract" xml:lang="en">We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.</div>
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<Abstract><AbstractText>We present the coupling of a jet-stirred reactor to detection by cw-CRDS in the near infrared and first results obtained during the oxidation of methane. The mixture is rapidly expanded from the jet-stirred reactor into a 80 cm-long cw-CRDS cell maintained at a the pressure around 1.33 kPa, thus freezing the reaction and decreasing pressure broadening of the absorption lines. Some stable species (CH4, H2O and CH2O) have been quantified through their well structured spectra around 1506 nm, while H2O2 and HO2 radicals could not be detected.</AbstractText>
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