LrgpV1, Hal, Curation, bibRecord, 000956

Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

Identifieur interne : 000956 ( Hal/Curation ); précédent : 000955; suivant : 000957

Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

Auteurs : Chiheb Bahrini [France] ; Olivier Herbinet [France] ; Pierre-Alexandre Glaude [France] ; Coralie Schoemaecker [France] ; Christa Fittschen [France] ; Frederique Battin-Leclerc [France]

Source :

Journal of the American Chemical Society [ 0002-7863 ] ; 2012.

RBID : Hal:hal-00776644

English descriptors

mix :
- AUTOIGNITION, CHEMICAL KINETIC-MODELS, COMBUSTION, CW-CRDS, DECOMPOSITION, HO2 RADICALS, IGNITION, SPECTROSCOPY.

Abstract

The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions dose to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.

Url:

https://hal.archives-ouvertes.fr/hal-00776644

DOI: 10.1021/ja305200h

Links toward previous steps (curation, corpus...)

to stream Hal, to step Corpus: Pour aller vers cette notice dans l'étape Curation :000956

Links to Exploration step

Hal:hal-00776644

Le document en format XML

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<front><div type="abstract" xml:lang="en">The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions dose to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</div>
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Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

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