Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes
Identifieur interne : 000955 ( Hal/Curation ); précédent : 000954; suivant : 000956Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes
Auteurs : Chiheb Bahrini [France] ; Olivier Herbinet [France] ; Pierre Alexandre Glaude [France] ; Coralie Schoemaecker [France] ; Christa Fittschen [France] ; Frédérique Battin-Leclerc [France]Source :
- Journal of the American Chemical Society [ 0002-7863 ] ; 2012-07-02.
English descriptors
Abstract
The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.
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DOI: 10.1021/ja305200h
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<front><div type="abstract" xml:lang="en">The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</div>
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<hal api="V3"><titleStmt><title xml:lang="en">Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes</title>
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<funder>This work was supported by the European Commission through the "Clean ICE" Advanced Research Grant of the European Research Council and by the COST Action CM0901</funder>
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