Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes
Identifieur interne : 000956 ( Hal/Corpus ); précédent : 000955; suivant : 000957Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes
Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frederique Battin-LeclercSource :
- Journal of the American Chemical Society [ 0002-7863 ] ; 2012.
English descriptors
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Abstract
The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions dose to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.
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DOI: 10.1021/ja305200h
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Hal:hal-00776644Le document en format XML
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<front><div type="abstract" xml:lang="en">The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions dose to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</div>
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