LrgpV1, Hal, Corpus, bibRecord, 000957

Quantification of OH and HO2 radicals during the low-temperature oxidation of hydrocarbons by Fluorescence Assay by Gas Expansion technique

Identifieur interne : 000957 ( Hal/Corpus ); précédent : 000956; suivant : 000958

Quantification of OH and HO2 radicals during the low-temperature oxidation of hydrocarbons by Fluorescence Assay by Gas Expansion technique

Auteurs : Marion Blocquet ; Coralie Schoemaecker ; Damien Amedro ; Olivier Herbinet ; Frédérique Battin-Leclerc ; Christa Fittschen

Source :

RBID : Hal:hal-00923973

Descripteurs français

mix :
- HOx radicals, autoignition.

Abstract

OH and *HO2 radicals are known to be the key species in the development of ignition. A direct measurement of these radicals under low-temperature oxidation conditions (T = 550 - 1000 K) has been achieved by coupling a technique named fluorescence assay by gas expansion, an experimental technique designed for the quantification of these radicals in the free atmosphere, to a jet-stirred reactor, an experimental device designed for the study of low-temperature combustion chemistry. Calibration allows conversion of relative fluorescence signals to absolute mole fractions. Such radical mole fraction profiles will serve as a benchmark for testing chemical models developed to improve the understanding of combustion processes.

Url:

https://hal.archives-ouvertes.fr/hal-00923973

DOI: 10.1073/pnas.1314968110

Links to Exploration step

Hal:hal-00923973

Le document en format XML

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<front><div type="abstract" xml:lang="en">OH and *HO2 radicals are known to be the key species in the development of ignition. A direct measurement of these radicals under low-temperature oxidation conditions (T = 550 - 1000 K) has been achieved by coupling a technique named fluorescence assay by gas expansion, an experimental technique designed for the quantification of these radicals in the free atmosphere, to a jet-stirred reactor, an experimental device designed for the study of low-temperature combustion chemistry. Calibration allows conversion of relative fluorescence signals to absolute mole fractions. Such radical mole fraction profiles will serve as a benchmark for testing chemical models developed to improve the understanding of combustion processes.</div>
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<funder>PhysicoChimie des Processus de Combustion et de l'Atmosphère participates in the Institut de Recherche en Environnement Industriel financed by the Région Nord Pas-de-Calais, the Ministère de l'Enseignement Supérieur et de la Recherche, the Centre National de la Recherche Scientifique, and the European Regional Development Fund. This project was supported by the French Agence Nationale de la Recherche under Contract ANR-11-LabEx-0005-01 "Chemical and Physical Properties of the Atmosphere," by the European Commission through the "Clean ICE" Advanced Research Grant of the European Research Council, and by European Cooperation in Science and Technology Action CM0901.</funder>
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<abstract xml:lang="en">OH and *HO2 radicals are known to be the key species in the development of ignition. A direct measurement of these radicals under low-temperature oxidation conditions (T = 550 - 1000 K) has been achieved by coupling a technique named fluorescence assay by gas expansion, an experimental technique designed for the quantification of these radicals in the free atmosphere, to a jet-stirred reactor, an experimental device designed for the study of low-temperature combustion chemistry. Calibration allows conversion of relative fluorescence signals to absolute mole fractions. Such radical mole fraction profiles will serve as a benchmark for testing chemical models developed to improve the understanding of combustion processes.</abstract>
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Quantification of OH and HO2 radicals during the low-temperature oxidation of hydrocarbons by Fluorescence Assay by Gas Expansion technique

Quantification of OH and HO2 radicals during the low-temperature oxidation of hydrocarbons by Fluorescence Assay by Gas Expansion technique

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