LrgpV1, Hal, Checkpoint, bibRecord, 000730

Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

Identifieur interne : 000730 ( Hal/Checkpoint ); précédent : 000729; suivant : 000731

Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

Auteurs : Chiheb Bahrini [France] ; Olivier Herbinet [France] ; Pierre Alexandre Glaude [France] ; Coralie Schoemaecker [France] ; Christa Fittschen [France] ; Frédérique Battin-Leclerc [France]

Source :

Journal of the American Chemical Society [ 0002-7863 ] ; 2012-07-02.

RBID : Hal:hal-00726379

English descriptors

mix :
- combustion, hydrogen peroxide, jet-stirred reactor, low-temperature oxidation.

Abstract

The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.

Url:

https://hal.archives-ouvertes.fr/hal-00726379

DOI: 10.1021/ja305200h

Links toward previous steps (curation, corpus...)

to stream Hal, to step Corpus: 000955
to stream Hal, to step Curation: 000955

Links to Exploration step

Hal:hal-00726379

Le document en format XML

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<front><div type="abstract" xml:lang="en">The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</div>
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<funder>This work was supported by the European Commission through the "Clean ICE" Advanced Research Grant of the European Research Council and by the COST Action CM0901</funder>
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<abstract xml:lang="en">The first reliable quantification of hydrogen peroxide (H2O2) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</abstract>
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Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

Quantification of Hydrogen Peroxide during the Low-Temperature Oxidation of Alkanes

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