Validation of a new apparatus using the dynamic method for determining the critical properties of binary mixtures containing CO2 and a n-alkane
Identifieur interne : 000729 ( Hal/Checkpoint ); précédent : 000728; suivant : 000730Validation of a new apparatus using the dynamic method for determining the critical properties of binary mixtures containing CO2 and a n-alkane
Auteurs : Niramol Juntarachat [France] ; Salma Bello [France] ; Romain Privat [France] ; Jean-Noël Jaubert [France]Source :
- Fluid Phase Equilibria [ 0378-3812 ] ; 2012-07-15.
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Abstract
In this paper the experimental setup of a new apparatus able to provide the critical properties of binary mixtures with known overall composition using a dynamic method is described. Critical temperatures (T-c) and critical pressures (P-c) of binary mixtures composed of carbon dioxide and n-alkanes (CO2 + n-pentane, CO2 + n-heptane and CO2 + n-decane) are measured. The critical points are visually determined by observing the critical opalescence and the simultaneous disappearance and reappearance of the meniscus in the middle of the view cell which withstands operations up to 673 K and 20 MPa. The experimental critical data are compared with success to literature database and with their prediction from the PPR78 thermodynamic model.
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DOI: 10.1016/j.fluid.2012.04.010
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<front><div type="abstract" xml:lang="en">In this paper the experimental setup of a new apparatus able to provide the critical properties of binary mixtures with known overall composition using a dynamic method is described. Critical temperatures (T-c) and critical pressures (P-c) of binary mixtures composed of carbon dioxide and n-alkanes (CO2 + n-pentane, CO2 + n-heptane and CO2 + n-decane) are measured. The critical points are visually determined by observing the critical opalescence and the simultaneous disappearance and reappearance of the meniscus in the middle of the view cell which withstands operations up to 673 K and 20 MPa. The experimental critical data are compared with success to literature database and with their prediction from the PPR78 thermodynamic model.</div>
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<hal api="V3"><titleStmt><title xml:lang="en">Validation of a new apparatus using the dynamic method for determining the critical properties of binary mixtures containing CO2 and a n-alkane</title>
<author role="aut"><persName><forename type="first">Niramol</forename>
<surname>Juntarachat</surname>
</persName>
<email></email>
<idno type="halauthor">806363</idno>
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<author role="aut"><persName><forename type="first">Salma</forename>
<surname>Bello</surname>
</persName>
<email></email>
<idno type="halauthor">806365</idno>
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<author role="aut"><persName><forename type="first">Romain</forename>
<surname>Privat</surname>
</persName>
<email>romain.privat@univ-lorraine.fr</email>
<idno type="halauthor">806338</idno>
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<author role="crp"><persName><forename type="first">Jean-Noël</forename>
<surname>Jaubert</surname>
</persName>
<email>jean-noel.jaubert@univ-lorraine.fr</email>
<idno type="halauthor">806339</idno>
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<editor role="depositor"><persName><forename>Gabriel</forename>
<surname>Wild</surname>
</persName>
<email>gabriel.wild@univ-lorraine.fr</email>
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<editionStmt><edition n="v1" type="current"><date type="whenSubmitted">2013-01-16 14:50:26</date>
<date type="whenWritten">2012</date>
<date type="whenModified">2016-05-11 01:05:31</date>
<date type="whenReleased">2013-01-16 14:50:26</date>
<date type="whenProduced">2012-07-15</date>
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<name key="179637"><persName><forename>Gabriel</forename>
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<idno type="halRefHtml">Fluid Phase Equilibria, Elsevier, 2012, 325, pp.66-70. <10.1016/j.fluid.2012.04.010></idno>
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<sourceDesc><biblStruct><analytic><title xml:lang="en">Validation of a new apparatus using the dynamic method for determining the critical properties of binary mixtures containing CO2 and a n-alkane</title>
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<author role="aut"><persName><forename type="first">Salma</forename>
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<author role="aut"><persName><forename type="first">Romain</forename>
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<author role="crp"><persName><forename type="first">Jean-Noël</forename>
<surname>Jaubert</surname>
</persName>
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<idno type="halAuthorId">806339</idno>
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<title level="j">Fluid Phase Equilibria</title>
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<biblScope unit="volume">325</biblScope>
<biblScope unit="pp">66-70</biblScope>
<date type="datePub">2012-07-15</date>
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<textClass><keywords scheme="author"><term xml:lang="en">Experimental methods</term>
<term xml:lang="en">Critical point</term>
<term xml:lang="en">Critical opalescence</term>
<term xml:lang="en">Critical loci</term>
<term xml:lang="en">Dynamic method</term>
<term xml:lang="en">MODEL PREDICTIVE 1978</term>
<term xml:lang="en">PENG-ROBINSON EOS</term>
<term xml:lang="en">EQUATION-OF-STATE</term>
<term xml:lang="en">EQUILIBRIUM PHASE PROPERTIES</term>
<term xml:lang="en">VAPOR-LIQUID-EQUILIBRIUM</term>
<term xml:lang="en">PPR78 MODEL</term>
<term xml:lang="en">CARBON-DIOXIDE</term>
<term xml:lang="en">CRITICAL-POINTS</term>
<term xml:lang="en">SYSTEMS</term>
<term xml:lang="en">K(IJ)</term>
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<classCode scheme="halDomain" n="phys.phys.phys-chem-ph">Physics [physics]/Physics [physics]/Chemical Physics [physics.chem-ph]</classCode>
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<abstract xml:lang="en">In this paper the experimental setup of a new apparatus able to provide the critical properties of binary mixtures with known overall composition using a dynamic method is described. Critical temperatures (T-c) and critical pressures (P-c) of binary mixtures composed of carbon dioxide and n-alkanes (CO2 + n-pentane, CO2 + n-heptane and CO2 + n-decane) are measured. The critical points are visually determined by observing the critical opalescence and the simultaneous disappearance and reappearance of the meniscus in the middle of the view cell which withstands operations up to 673 K and 20 MPa. The experimental critical data are compared with success to literature database and with their prediction from the PPR78 thermodynamic model.</abstract>
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