5,6-Bis(tetradecyloxy)-2,1,3-benzoselenadiazole-Based Polymers for Photovoltaic Applications
Identifieur interne : 001235 ( Main/Repository ); précédent : 001234; suivant : 0012365,6-Bis(tetradecyloxy)-2,1,3-benzoselenadiazole-Based Polymers for Photovoltaic Applications
Auteurs : RBID : Pascal:13-0291632Descripteurs français
- Pascal (Inist)
- Polymère conducteur, Polycondensation solution, Copulation Stille, Copulation Suzuki, Thiophène copolymère, Propriété filmogène, Stabilité thermique, Thiophène dérivé copolymère, Carbazole dérivé copolymère, Copolymère hétérocyclique azote, Polymère sélénium, Copolymère aromatique, Copolymère conjugué, Préparation, Propriété électrochimique, Absorption optique, Cellule solaire organique, Etude expérimentale, Propriété thermique, Fluorène dérivé copolymère, Propriété optique, Copolymère sélénium, Fluorénylène(9,9-dioctyl) copolymère, 2,1,3-Benzosélénadiazole dérivé copolymère.
English descriptors
- KwdEn :
- Aromatic copolymer, Carbazole derivative copolymer, Conducting polymers, Conjugated copolymer, Electrochemical properties, Experimental study, Film forming properties, Fluorene derivative copolymer, Nitrogen heterocycle copolymer, Optical absorption, Optical properties, Organic solar cells, Preparation, Selenium containing polymer, Solution polycondensation, Stille coupling, Suzuki coupling, Thermal properties, Thermal stability, Thiophene copolymer, Thiophene derivative copolymer.
Abstract
A series of new 5,6-bis(tetradecyloxy)-2,1,3-benzoselenadiazole-based copolymers (PBDT-DTBSe, PC-DTBSe, and PF-DTBSe) have been first synthesized by Stille or Suzuki coupling polymerization reaction. The synthesized copolymers show good solubility in common organic solvents, such as chloroform, tetrahydrofuran, and chlorobenzene with excellent film-forming properties. The molecular weight was determined by gel permeation chromatography and the thermal properties were investigated by thermogravimetric analysis. All the copolymers exhibited broad absorption from 350 to 700 nm. The preliminary results showed the device based on the structure of indium tin oxide/PEDOT:PSS/PC-DTBSe:PC61BM (1: 2, w/w)/Ca/Al displayed the best photovoltaic performance with a power conversion efficiency of 1.35%, a Voc of 0.87 V, a Jsc of 3.84 mA/cm2 and a fill factor of 40.4%, under illumination of AM 1.5 G (100 mW/cm2).
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Pascal:13-0291632Le document en format XML
<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">5,6-Bis(tetradecyloxy)-2,1,3-benzoselenadiazole-Based Polymers for Photovoltaic Applications</title><author><name>WANJUN TANG</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>College of Chemistry and Chemical Engineering, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>République populaire de Chine</country><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name>XUEWEN CHEN</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>College of Chemistry and Chemical Engineering, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>République populaire de Chine</country><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name>YINGPING ZOU</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>College of Chemistry and Chemical Engineering, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>République populaire de Chine</country><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name>BO LIU</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>State Key Laboratory for Powder Metallurgy, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>4 aut.</sZ></inist:fA14><country>République populaire de Chine</country><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name>HONG ZHONG</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>College of Chemistry and Chemical Engineering, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>République populaire de Chine</country><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author><author><name>CHUNYUE PAN</name><affiliation wicri:level="1"><inist:fA14 i1="01"><s1>College of Chemistry and Chemical Engineering, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></inist:fA14><country>République populaire de Chine</country><wicri:noRegion>Changsha 410083</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="inist">13-0291632</idno><date when="2013">2013</date><idno type="stanalyst">PASCAL 13-0291632 INIST</idno><idno type="RBID">Pascal:13-0291632</idno><idno type="wicri:Area/Main/Corpus">000774</idno><idno type="wicri:Area/Main/Repository">001235</idno></publicationStmt><seriesStmt><idno type="ISSN">0021-8995</idno><title level="j" type="abbreviated">J. appl. polym. sci.</title><title level="j" type="main">Journal of applied polymer science</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Aromatic copolymer</term><term>Carbazole derivative copolymer</term><term>Conducting polymers</term><term>Conjugated copolymer</term><term>Electrochemical properties</term><term>Experimental study</term><term>Film forming properties</term><term>Fluorene derivative copolymer</term><term>Nitrogen heterocycle copolymer</term><term>Optical absorption</term><term>Optical properties</term><term>Organic solar cells</term><term>Preparation</term><term>Selenium containing polymer</term><term>Solution polycondensation</term><term>Stille coupling</term><term>Suzuki coupling</term><term>Thermal properties</term><term>Thermal stability</term><term>Thiophene copolymer</term><term>Thiophene derivative copolymer</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Polymère conducteur</term><term>Polycondensation solution</term><term>Copulation Stille</term><term>Copulation Suzuki</term><term>Thiophène copolymère</term><term>Propriété filmogène</term><term>Stabilité thermique</term><term>Thiophène dérivé copolymère</term><term>Carbazole dérivé copolymère</term><term>Copolymère hétérocyclique azote</term><term>Polymère sélénium</term><term>Copolymère aromatique</term><term>Copolymère conjugué</term><term>Préparation</term><term>Propriété électrochimique</term><term>Absorption optique</term><term>Cellule solaire organique</term><term>Etude expérimentale</term><term>Propriété thermique</term><term>Fluorène dérivé copolymère</term><term>Propriété optique</term><term>Copolymère sélénium</term><term>Fluorénylène(9,9-dioctyl) copolymère</term><term>2,1,3-Benzosélénadiazole dérivé copolymère</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">A series of new 5,6-bis(tetradecyloxy)-2,1,3-benzoselenadiazole-based copolymers (PBDT-DTBSe, PC-DTBSe, and PF-DTBSe) have been first synthesized by Stille or Suzuki coupling polymerization reaction. The synthesized copolymers show good solubility in common organic solvents, such as chloroform, tetrahydrofuran, and chlorobenzene with excellent film-forming properties. The molecular weight was determined by gel permeation chromatography and the thermal properties were investigated by thermogravimetric analysis. All the copolymers exhibited broad absorption from 350 to 700 nm. The preliminary results showed the device based on the structure of indium tin oxide/PEDOT:PSS/PC-DTBSe:PC<sub>61</sub>BM (1: 2, w/w)/Ca/Al displayed the best photovoltaic performance with a power conversion efficiency of 1.35%, a V<sub>oc</sub> of 0.87 V, a J<sub>sc</sub> of 3.84 mA/cm<sup>2</sup> and a fill factor of 40.4%, under illumination of AM 1.5 G (100 mW/cm<sup>2</sup>).</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0021-8995</s0></fA01><fA02 i1="01"><s0>JAPNAB</s0></fA02><fA03 i2="1"><s0>J. appl. polym. sci.</s0></fA03><fA05><s2>128</s2></fA05><fA06><s2>6</s2></fA06><fA08 i1="01" i2="1" l="ENG"><s1>5,6-Bis(tetradecyloxy)-2,1,3-benzoselenadiazole-Based Polymers for Photovoltaic Applications</s1></fA08><fA11 i1="01" i2="1"><s1>WANJUN TANG</s1></fA11><fA11 i1="02" i2="1"><s1>XUEWEN CHEN</s1></fA11><fA11 i1="03" i2="1"><s1>YINGPING ZOU</s1></fA11><fA11 i1="04" i2="1"><s1>BO LIU</s1></fA11><fA11 i1="05" i2="1"><s1>HONG ZHONG</s1></fA11><fA11 i1="06" i2="1"><s1>CHUNYUE PAN</s1></fA11><fA14 i1="01"><s1>College of Chemistry and Chemical Engineering, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ></fA14><fA14 i1="02"><s1>State Key Laboratory for Powder Metallurgy, Central South University</s1><s2>Changsha 410083</s2><s3>CHN</s3><sZ>4 aut.</sZ></fA14><fA20><s1>3678-3686</s1></fA20><fA21><s1>2013</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>1257</s2><s5>354000503742640230</s5></fA43><fA44><s0>0000</s0><s1>© 2013 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>31 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>13-0291632</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Journal of applied polymer science</s0></fA64><fA66 i1="01"><s0>USA</s0></fA66><fC01 i1="01" l="ENG"><s0>A series of new 5,6-bis(tetradecyloxy)-2,1,3-benzoselenadiazole-based copolymers (PBDT-DTBSe, PC-DTBSe, and PF-DTBSe) have been first synthesized by Stille or Suzuki coupling polymerization reaction. The synthesized copolymers show good solubility in common organic solvents, such as chloroform, tetrahydrofuran, and chlorobenzene with excellent film-forming properties. The molecular weight was determined by gel permeation chromatography and the thermal properties were investigated by thermogravimetric analysis. All the copolymers exhibited broad absorption from 350 to 700 nm. The preliminary results showed the device based on the structure of indium tin oxide/PEDOT:PSS/PC-DTBSe:PC<sub>61</sub>BM (1: 2, w/w)/Ca/Al displayed the best photovoltaic performance with a power conversion efficiency of 1.35%, a V<sub>oc</sub> of 0.87 V, a J<sub>sc</sub> of 3.84 mA/cm<sup>2</sup> and a fill factor of 40.4%, under illumination of AM 1.5 G (100 mW/cm<sup>2</sup>).</s0></fC01><fC02 i1="01" i2="X"><s0>001D09D02E</s0></fC02><fC02 i1="02" i2="X"><s0>001D06C02D1</s0></fC02><fC02 i1="03" i2="X"><s0>230</s0></fC02><fC03 i1="01" i2="3" l="FRE"><s0>Polymère conducteur</s0><s5>01</s5></fC03><fC03 i1="01" i2="3" l="ENG"><s0>Conducting polymers</s0><s5>01</s5></fC03><fC03 i1="02" i2="X" l="FRE"><s0>Polycondensation solution</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="ENG"><s0>Solution polycondensation</s0><s5>02</s5></fC03><fC03 i1="02" i2="X" l="SPA"><s0>Policondensación solución</s0><s5>02</s5></fC03><fC03 i1="03" i2="X" l="FRE"><s0>Copulation 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stability</s0><s5>07</s5></fC03><fC03 i1="07" i2="X" l="SPA"><s0>Estabilidad térmica</s0><s5>07</s5></fC03><fC03 i1="08" i2="X" l="FRE"><s0>Thiophène dérivé copolymère</s0><s2>NK</s2><s5>08</s5></fC03><fC03 i1="08" i2="X" l="ENG"><s0>Thiophene derivative copolymer</s0><s2>NK</s2><s5>08</s5></fC03><fC03 i1="08" i2="X" l="SPA"><s0>Tiofeno derivado copolímero</s0><s2>NK</s2><s5>08</s5></fC03><fC03 i1="09" i2="X" l="FRE"><s0>Carbazole dérivé copolymère</s0><s2>NK</s2><s5>09</s5></fC03><fC03 i1="09" i2="X" l="ENG"><s0>Carbazole derivative copolymer</s0><s2>NK</s2><s5>09</s5></fC03><fC03 i1="09" i2="X" l="SPA"><s0>Carbazol derivado copolímero</s0><s2>NK</s2><s5>09</s5></fC03><fC03 i1="10" i2="X" l="FRE"><s0>Copolymère hétérocyclique azote</s0><s2>NK</s2><s5>10</s5></fC03><fC03 i1="10" i2="X" l="ENG"><s0>Nitrogen heterocycle copolymer</s0><s2>NK</s2><s5>10</s5></fC03><fC03 i1="10" i2="X" l="SPA"><s0>Copolímero heterocíclico nitrógeno</s0><s2>NK</s2><s5>10</s5></fC03><fC03 i1="11" i2="X" l="FRE"><s0>Polymère sélénium</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="ENG"><s0>Selenium containing polymer</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="SPA"><s0>Polimero selenio</s0><s5>11</s5></fC03><fC03 i1="12" i2="X" l="FRE"><s0>Copolymère aromatique</s0><s2>NK</s2><s5>12</s5></fC03><fC03 i1="12" i2="X" l="ENG"><s0>Aromatic copolymer</s0><s2>NK</s2><s5>12</s5></fC03><fC03 i1="12" i2="X" l="SPA"><s0>Copolímero aromático</s0><s2>NK</s2><s5>12</s5></fC03><fC03 i1="13" i2="X" l="FRE"><s0>Copolymère conjugué</s0><s2>NK</s2><s5>13</s5></fC03><fC03 i1="13" i2="X" l="ENG"><s0>Conjugated copolymer</s0><s2>NK</s2><s5>13</s5></fC03><fC03 i1="13" i2="X" l="SPA"><s0>Copolímero conjugado</s0><s2>NK</s2><s5>13</s5></fC03><fC03 i1="14" i2="X" l="FRE"><s0>Préparation</s0><s5>14</s5></fC03><fC03 i1="14" i2="X" l="ENG"><s0>Preparation</s0><s5>14</s5></fC03><fC03 i1="14" i2="X" l="SPA"><s0>Preparación</s0><s5>14</s5></fC03><fC03 i1="15" i2="X" l="FRE"><s0>Propriété électrochimique</s0><s5>15</s5></fC03><fC03 i1="15" i2="X" l="ENG"><s0>Electrochemical properties</s0><s5>15</s5></fC03><fC03 i1="15" i2="X" l="SPA"><s0>Propiedad electroquímica</s0><s5>15</s5></fC03><fC03 i1="16" i2="X" l="FRE"><s0>Absorption optique</s0><s5>16</s5></fC03><fC03 i1="16" i2="X" l="ENG"><s0>Optical absorption</s0><s5>16</s5></fC03><fC03 i1="16" i2="X" l="SPA"><s0>Absorción óptica</s0><s5>16</s5></fC03><fC03 i1="17" i2="3" l="FRE"><s0>Cellule solaire organique</s0><s5>17</s5></fC03><fC03 i1="17" i2="3" l="ENG"><s0>Organic solar cells</s0><s5>17</s5></fC03><fC03 i1="18" i2="X" l="FRE"><s0>Etude expérimentale</s0><s5>18</s5></fC03><fC03 i1="18" i2="X" l="ENG"><s0>Experimental study</s0><s5>18</s5></fC03><fC03 i1="18" i2="X" l="SPA"><s0>Estudio experimental</s0><s5>18</s5></fC03><fC03 i1="19" i2="X" l="FRE"><s0>Propriété thermique</s0><s5>31</s5></fC03><fC03 i1="19" i2="X" l="ENG"><s0>Thermal properties</s0><s5>31</s5></fC03><fC03 i1="19" i2="X" l="SPA"><s0>Propiedad térmica</s0><s5>31</s5></fC03><fC03 i1="20" i2="X" l="FRE"><s0>Fluorène dérivé copolymère</s0><s5>32</s5></fC03><fC03 i1="20" i2="X" l="ENG"><s0>Fluorene derivative copolymer</s0><s5>32</s5></fC03><fC03 i1="20" i2="X" l="SPA"><s0>Fluoreno derivado copolímero</s0><s5>32</s5></fC03><fC03 i1="21" i2="X" l="FRE"><s0>Propriété optique</s0><s5>33</s5></fC03><fC03 i1="21" i2="X" l="ENG"><s0>Optical properties</s0><s5>33</s5></fC03><fC03 i1="21" i2="X" l="SPA"><s0>Propiedad óptica</s0><s5>33</s5></fC03><fC03 i1="22" i2="X" l="FRE"><s0>Copolymère sélénium</s0><s2>NK</s2><s4>INC</s4><s5>41</s5></fC03><fC03 i1="23" i2="X" l="FRE"><s0>Fluorénylène(9,9-dioctyl) copolymère</s0><s2>NK</s2><s4>INC</s4><s5>42</s5></fC03><fC03 i1="24" i2="X" l="FRE"><s0>2,1,3-Benzosélénadiazole dérivé copolymère</s0><s2>NK</s2><s4>INC</s4><s5>43</s5></fC03><fN21><s1>273</s1></fN21></pA></standard></inist></record>Pour manipuler ce document sous Unix (Dilib)
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