Surface Segregation of Cyclic Chains in Binary Melts of Thin Polymer Films: The Influence of Constituent Concentration
Identifieur interne : 000794 ( Main/Curation ); précédent : 000793; suivant : 000795Surface Segregation of Cyclic Chains in Binary Melts of Thin Polymer Films: The Influence of Constituent Concentration
Auteurs : Francis M. Gaitho ; Mesfin Tsige ; Genene T. Mola ; Giuseppe Pellicane [Afrique du Sud]Source :
- Polymers [ 2073-4360 ] ; 2018.
Abstract
We carry out extensive molecular dynamics simulations of thin films of bead-spring models of binary mixtures composed of cyclic and linear polymer chains. We study the equilibrium behavior of the polymer chains for two very different chain lengths, which resemble short (10-mers) and long (100-mers) chains, at different concentrations of the binary mixture. We clearly show how the concentration variable affects the enrichment of either of the two polymer species at the interface, and also how the chain length influences this process.
Url:
DOI: 10.3390/polym10030324
PubMed: 30966359
PubMed Central: 6414847
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Gaitho</name><affiliation><nlm:aff id="af1-polymers-10-00324">School of Chemistry & Physics, University of KwaZulu-Natal, Pietermaritzburg, Private Bag X01, Scottsville 3209, South Africa;<email>fgaitho@mmust.ac.ke</email> (F.M.G.);<email>mola@ukzn.ac.za</email> (G.T.M.)</nlm:aff></affiliation></author><author><name sortKey="Tsige, Mesfin" sort="Tsige, Mesfin" uniqKey="Tsige M" first="Mesfin" last="Tsige">Mesfin Tsige</name><affiliation><nlm:aff id="af2-polymers-10-00324">Department of Polymer Science, University of Akron, Akron, OH 44325, USA;<email>mtsige@uakron.edu</email></nlm:aff></affiliation></author><author><name sortKey="Mola, Genene T" sort="Mola, Genene T" uniqKey="Mola G" first="Genene T." last="Mola">Genene T. 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Gaitho</name><affiliation><nlm:aff id="af1-polymers-10-00324">School of Chemistry & Physics, University of KwaZulu-Natal, Pietermaritzburg, Private Bag X01, Scottsville 3209, South Africa;<email>fgaitho@mmust.ac.ke</email> (F.M.G.);<email>mola@ukzn.ac.za</email> (G.T.M.)</nlm:aff></affiliation></author><author><name sortKey="Tsige, Mesfin" sort="Tsige, Mesfin" uniqKey="Tsige M" first="Mesfin" last="Tsige">Mesfin Tsige</name><affiliation><nlm:aff id="af2-polymers-10-00324">Department of Polymer Science, University of Akron, Akron, OH 44325, USA;<email>mtsige@uakron.edu</email></nlm:aff></affiliation></author><author><name sortKey="Mola, Genene T" sort="Mola, Genene T" uniqKey="Mola G" first="Genene T." last="Mola">Genene T. Mola</name><affiliation><nlm:aff id="af1-polymers-10-00324">School of Chemistry & Physics, University of KwaZulu-Natal, Pietermaritzburg, Private Bag X01, Scottsville 3209, South Africa;<email>fgaitho@mmust.ac.ke</email> (F.M.G.);<email>mola@ukzn.ac.za</email> (G.T.M.)</nlm:aff></affiliation></author><author><name sortKey="Pellicane, Giuseppe" sort="Pellicane, Giuseppe" uniqKey="Pellicane G" first="Giuseppe" last="Pellicane">Giuseppe Pellicane</name><affiliation><nlm:aff id="af1-polymers-10-00324">School of Chemistry & Physics, University of KwaZulu-Natal, Pietermaritzburg, Private Bag X01, Scottsville 3209, South Africa;<email>fgaitho@mmust.ac.ke</email> (F.M.G.);<email>mola@ukzn.ac.za</email> (G.T.M.)</nlm:aff></affiliation><affiliation wicri:level="1"><nlm:aff id="af3-polymers-10-00324">National Institute of Theoretical Physics (NITheP) KZN Node, Pietermaritzburg, Private Bag X01, Scottsville 3209, South Africa</nlm:aff><country xml:lang="fr">Afrique du Sud</country><wicri:regionArea>National Institute of Theoretical Physics (NITheP) KZN Node, Pietermaritzburg, Private Bag X01, Scottsville 3209</wicri:regionArea><wicri:noRegion>Scottsville 3209</wicri:noRegion></affiliation></author></analytic><series><title level="j">Polymers</title><idno type="eISSN">2073-4360</idno><imprint><date when="2018">2018</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>We carry out extensive molecular dynamics simulations of thin films of bead-spring models of binary mixtures composed of cyclic and linear polymer chains. We study the equilibrium behavior of the polymer chains for two very different chain lengths, which resemble short (10-mers) and long (100-mers) chains, at different concentrations of the binary mixture. We clearly show how the concentration variable affects the enrichment of either of the two polymer species at the interface, and also how the chain length influences this process.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Chen, D" uniqKey="Chen D">D. Chen</name></author><author><name sortKey="Nakahara, A" uniqKey="Nakahara A">A. Nakahara</name></author><author><name sortKey="Wei, D" uniqKey="Wei D">D. Wei</name></author><author><name sortKey="Nordlund, D" uniqKey="Nordlund D">D. Nordlund</name></author><author><name sortKey="Russell, T P" uniqKey="Russell T">T.P. Russell</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Shi, J" uniqKey="Shi J">J. 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