Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.
Identifieur interne : 002412 ( Ncbi/Curation ); précédent : 002411; suivant : 002413Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.
Auteurs : Vânia T. Freitas [Portugal] ; Lianshe Fu [Portugal] ; Ana M. Cojocariu [France] ; Xavier Cattoën [France] ; John R. Bartlett ; Rozenn Le Parc [France] ; Jean-Louis Bantignies [France] ; Michel Wong Chi Man [France] ; Paulo S. André [Portugal] ; Rute A S. Ferreira [Portugal] ; Luís D. Carlos [Portugal]Source :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2015.
Abstract
The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).
DOI: 10.1021/acsami.5b01281
PubMed: 25835303
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John R. Bartlett<affiliation><nlm:affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</nlm:affiliation><wicri:noCountry code="subField">QLD 4558 Australia</wicri:noCountry></affiliation>Le document en format XML
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Freitas</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Fu, Lianshe" sort="Fu, Lianshe" uniqKey="Fu L" first="Lianshe" last="Fu">Lianshe Fu</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Cojocariu, Ana M" sort="Cojocariu, Ana M" uniqKey="Cojocariu A" first="Ana M" last="Cojocariu">Ana M. 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André</name><affiliation wicri:level="1"><nlm:affiliation>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa</wicri:regionArea><wicri:noRegion>Lisboa</wicri:noRegion></affiliation></author><author><name sortKey="Ferreira, Rute A S" sort="Ferreira, Rute A S" uniqKey="Ferreira R" first="Rute A S" last="Ferreira">Rute A S. 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Carlos</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2015">2015</date><idno type="RBID">pubmed:25835303</idno><idno type="pmid">25835303</idno><idno type="doi">10.1021/acsami.5b01281</idno><idno type="wicri:Area/PubMed/Corpus">002E38</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">002E38</idno><idno type="wicri:Area/PubMed/Curation">002D62</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Curation">002D62</idno><idno type="wicri:Area/PubMed/Checkpoint">002D62</idno><idno type="wicri:explorRef" wicri:stream="Checkpoint" wicri:step="PubMed">002D62</idno><idno type="wicri:Area/Ncbi/Merge">002412</idno><idno type="wicri:Area/Ncbi/Curation">002412</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.</title><author><name sortKey="Freitas, Vania T" sort="Freitas, Vania T" uniqKey="Freitas V" first="Vânia T" last="Freitas">Vânia T. Freitas</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Fu, Lianshe" sort="Fu, Lianshe" uniqKey="Fu L" first="Lianshe" last="Fu">Lianshe Fu</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Cojocariu, Ana M" sort="Cojocariu, Ana M" uniqKey="Cojocariu A" first="Ana M" last="Cojocariu">Ana M. Cojocariu</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea><wicri:noRegion>34296 Montpellier</wicri:noRegion><placeName><settlement type="city">Montpellier</settlement><region type="region" nuts="2">Occitanie (région administrative)</region><region type="old region" nuts="2">Languedoc-Roussillon</region></placeName></affiliation></author><author><name sortKey="Cattoen, Xavier" sort="Cattoen, Xavier" uniqKey="Cattoen X" first="Xavier" last="Cattoën">Xavier Cattoën</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea><wicri:noRegion>34296 Montpellier</wicri:noRegion><placeName><settlement type="city">Montpellier</settlement><region type="region" nuts="2">Occitanie (région administrative)</region><region type="old region" nuts="2">Languedoc-Roussillon</region></placeName></affiliation></author><author><name sortKey="Bartlett, John R" sort="Bartlett, John R" uniqKey="Bartlett J" first="John R" last="Bartlett">John R. Bartlett</name><affiliation><nlm:affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</nlm:affiliation><wicri:noCountry code="subField">QLD 4558 Australia</wicri:noCountry></affiliation></author><author><name sortKey="Le Parc, Rozenn" sort="Le Parc, Rozenn" uniqKey="Le Parc R" first="Rozenn" last="Le Parc">Rozenn Le Parc</name><affiliation wicri:level="1"><nlm:affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier</wicri:regionArea><wicri:noRegion>34095 Montpellier</wicri:noRegion><placeName><settlement type="city">Montpellier</settlement><region type="region" nuts="2">Occitanie (région administrative)</region><region type="old region" nuts="2">Languedoc-Roussillon</region></placeName></affiliation></author><author><name sortKey="Bantignies, Jean Louis" sort="Bantignies, Jean Louis" uniqKey="Bantignies J" first="Jean-Louis" last="Bantignies">Jean-Louis Bantignies</name><affiliation wicri:level="1"><nlm:affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier</wicri:regionArea><wicri:noRegion>34095 Montpellier</wicri:noRegion><placeName><settlement type="city">Montpellier</settlement><region type="region" nuts="2">Occitanie (région administrative)</region><region type="old region" nuts="2">Languedoc-Roussillon</region></placeName></affiliation></author><author><name sortKey="Man, Michel Wong Chi" sort="Man, Michel Wong Chi" uniqKey="Man M" first="Michel Wong Chi" last="Man">Michel Wong Chi Man</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea><wicri:noRegion>34296 Montpellier</wicri:noRegion><placeName><settlement type="city">Montpellier</settlement><region type="region" nuts="2">Occitanie (région administrative)</region><region type="old region" nuts="2">Languedoc-Roussillon</region></placeName></affiliation></author><author><name sortKey="Andre, Paulo S" sort="Andre, Paulo S" uniqKey="Andre P" first="Paulo S" last="André">Paulo S. André</name><affiliation wicri:level="1"><nlm:affiliation>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa</wicri:regionArea><wicri:noRegion>Lisboa</wicri:noRegion></affiliation></author><author><name sortKey="Ferreira, Rute A S" sort="Ferreira, Rute A S" uniqKey="Ferreira R" first="Rute A S" last="Ferreira">Rute A S. Ferreira</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author><author><name sortKey="Carlos, Luis D" sort="Carlos, Luis D" uniqKey="Carlos L" first="Luís D" last="Carlos">Luís D. Carlos</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea><wicri:noRegion>3810-193 Aveiro</wicri:noRegion></affiliation></author></analytic><series><title level="j">ACS applied materials & interfaces</title><idno type="eISSN">1944-8252</idno><imprint><date when="2015" type="published">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).</div></front></TEI></record>Pour manipuler ce document sous Unix (Dilib)
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