Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.
Identifieur interne : 002412 ( Ncbi/Merge ); précédent : 002411; suivant : 002413Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.
Auteurs : Vânia T. Freitas [Portugal] ; Lianshe Fu [Portugal] ; Ana M. Cojocariu [France] ; Xavier Cattoën [France] ; John R. Bartlett ; Rozenn Le Parc [France] ; Jean-Louis Bantignies [France] ; Michel Wong Chi Man [France] ; Paulo S. André [Portugal] ; Rute A S. Ferreira [Portugal] ; Luís D. Carlos [Portugal]Source :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2015.
Abstract
The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).
DOI: 10.1021/acsami.5b01281
PubMed: 25835303
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<wicri:regionArea>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa</wicri:regionArea>
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<front><div type="abstract" xml:lang="en">The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).</div>
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<ArticleTitle>Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.</ArticleTitle>
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<Abstract><AbstractText>The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).</AbstractText>
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<AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Freitas</LastName>
<ForeName>Vânia T</ForeName>
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<AffiliationInfo><Affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</Affiliation>
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<AffiliationInfo><Affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</Affiliation>
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<ForeName>Lianshe</ForeName>
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<AffiliationInfo><Affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</Affiliation>
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<AffiliationInfo><Affiliation>#Institut NEEL, CNRS, Université Grenoble-Alpes, 38042 Grenoble, France.</Affiliation>
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<Initials>R</Initials>
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<Author ValidYN="Y"><LastName>Bantignies</LastName>
<ForeName>Jean-Louis</ForeName>
<Initials>JL</Initials>
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<Author ValidYN="Y"><LastName>Man</LastName>
<ForeName>Michel Wong Chi</ForeName>
<Initials>MW</Initials>
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<Author ValidYN="Y"><LastName>André</LastName>
<ForeName>Paulo S</ForeName>
<Initials>PS</Initials>
<AffiliationInfo><Affiliation>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa, Portugal.</Affiliation>
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<ForeName>Rute A S</ForeName>
<Initials>RA</Initials>
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<ForeName>Luís D</ForeName>
<Initials>LD</Initials>
<AffiliationInfo><Affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</Affiliation>
</AffiliationInfo>
</Author>
</AuthorList>
<Language>eng</Language>
<PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType>
<PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType>
</PublicationTypeList>
<ArticleDate DateType="Electronic"><Year>2015</Year>
<Month>04</Month>
<Day>14</Day>
</ArticleDate>
</Article>
<MedlineJournalInfo><Country>United States</Country>
<MedlineTA>ACS Appl Mater Interfaces</MedlineTA>
<NlmUniqueID>101504991</NlmUniqueID>
<ISSNLinking>1944-8244</ISSNLinking>
</MedlineJournalInfo>
<KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">lanthanide complex</Keyword>
<Keyword MajorTopicYN="N">luminescent solar concentrator</Keyword>
<Keyword MajorTopicYN="N">organic−inorganic hybrids</Keyword>
<Keyword MajorTopicYN="N">sol−gel</Keyword>
<Keyword MajorTopicYN="N">thin films</Keyword>
</KeywordList>
</MedlineCitation>
<PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2015</Year>
<Month>4</Month>
<Day>4</Day>
<Hour>6</Hour>
<Minute>0</Minute>
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<PubMedPubDate PubStatus="pubmed"><Year>2015</Year>
<Month>4</Month>
<Day>4</Day>
<Hour>6</Hour>
<Minute>0</Minute>
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<PubMedPubDate PubStatus="medline"><Year>2015</Year>
<Month>4</Month>
<Day>4</Day>
<Hour>6</Hour>
<Minute>1</Minute>
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</History>
<PublicationStatus>ppublish</PublicationStatus>
<ArticleIdList><ArticleId IdType="pubmed">25835303</ArticleId>
<ArticleId IdType="doi">10.1021/acsami.5b01281</ArticleId>
</ArticleIdList>
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<affiliations><list><country><li>France</li>
<li>Portugal</li>
</country>
<region><li>Languedoc-Roussillon</li>
<li>Occitanie (région administrative)</li>
</region>
<settlement><li>Montpellier</li>
</settlement>
</list>
<tree><noCountry><name sortKey="Bartlett, John R" sort="Bartlett, John R" uniqKey="Bartlett J" first="John R" last="Bartlett">John R. Bartlett</name>
</noCountry>
<country name="Portugal"><noRegion><name sortKey="Freitas, Vania T" sort="Freitas, Vania T" uniqKey="Freitas V" first="Vânia T" last="Freitas">Vânia T. Freitas</name>
</noRegion>
<name sortKey="Andre, Paulo S" sort="Andre, Paulo S" uniqKey="Andre P" first="Paulo S" last="André">Paulo S. André</name>
<name sortKey="Carlos, Luis D" sort="Carlos, Luis D" uniqKey="Carlos L" first="Luís D" last="Carlos">Luís D. Carlos</name>
<name sortKey="Ferreira, Rute A S" sort="Ferreira, Rute A S" uniqKey="Ferreira R" first="Rute A S" last="Ferreira">Rute A S. Ferreira</name>
<name sortKey="Fu, Lianshe" sort="Fu, Lianshe" uniqKey="Fu L" first="Lianshe" last="Fu">Lianshe Fu</name>
</country>
<country name="France"><region name="Occitanie (région administrative)"><name sortKey="Cojocariu, Ana M" sort="Cojocariu, Ana M" uniqKey="Cojocariu A" first="Ana M" last="Cojocariu">Ana M. Cojocariu</name>
</region>
<name sortKey="Bantignies, Jean Louis" sort="Bantignies, Jean Louis" uniqKey="Bantignies J" first="Jean-Louis" last="Bantignies">Jean-Louis Bantignies</name>
<name sortKey="Cattoen, Xavier" sort="Cattoen, Xavier" uniqKey="Cattoen X" first="Xavier" last="Cattoën">Xavier Cattoën</name>
<name sortKey="Le Parc, Rozenn" sort="Le Parc, Rozenn" uniqKey="Le Parc R" first="Rozenn" last="Le Parc">Rozenn Le Parc</name>
<name sortKey="Man, Michel Wong Chi" sort="Man, Michel Wong Chi" uniqKey="Man M" first="Michel Wong Chi" last="Man">Michel Wong Chi Man</name>
</country>
</tree>
</affiliations>
</record>
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