Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.
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Auteurs : Vânia T. Freitas [Portugal] ; Lianshe Fu [Portugal] ; Ana M. Cojocariu [France] ; Xavier Cattoën [France] ; John R. Bartlett ; Rozenn Le Parc [France] ; Jean-Louis Bantignies [France] ; Michel Wong Chi Man [France] ; Paulo S. André [Portugal] ; Rute A S. Ferreira [Portugal] ; Luís D. Carlos [Portugal]Source :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2015.
Abstract
The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).
DOI: 10.1021/acsami.5b01281
PubMed: 25835303
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John R. Bartlett<affiliation><nlm:affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</nlm:affiliation><wicri:noCountry code="subField">QLD 4558 Australia</wicri:noCountry></affiliation>Le document en format XML
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Bartlett</name><affiliation><nlm:affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</nlm:affiliation><wicri:noCountry code="subField">QLD 4558 Australia</wicri:noCountry></affiliation></author><author><name sortKey="Le Parc, Rozenn" sort="Le Parc, Rozenn" uniqKey="Le Parc R" first="Rozenn" last="Le Parc">Rozenn Le Parc</name><affiliation wicri:level="1"><nlm:affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Bantignies, Jean Louis" sort="Bantignies, Jean Louis" uniqKey="Bantignies J" first="Jean-Louis" last="Bantignies">Jean-Louis Bantignies</name><affiliation wicri:level="1"><nlm:affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Man, Michel Wong Chi" sort="Man, Michel Wong Chi" uniqKey="Man M" first="Michel Wong Chi" last="Man">Michel Wong Chi Man</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Andre, Paulo S" sort="Andre, Paulo S" uniqKey="Andre P" first="Paulo S" last="André">Paulo S. André</name><affiliation wicri:level="1"><nlm:affiliation>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa</wicri:regionArea></affiliation></author><author><name sortKey="Ferreira, Rute A S" sort="Ferreira, Rute A S" uniqKey="Ferreira R" first="Rute A S" last="Ferreira">Rute A S. 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Carlos</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PubMed</idno><date when="2015">2015</date><idno type="RBID">pubmed:25835303</idno><idno type="pmid">25835303</idno><idno type="doi">10.1021/acsami.5b01281</idno><idno type="wicri:Area/PubMed/Corpus">002E38</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">002E38</idno><idno type="wicri:Area/PubMed/Curation">002D62</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Curation">002D62</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.</title><author><name sortKey="Freitas, Vania T" sort="Freitas, Vania T" uniqKey="Freitas V" first="Vânia T" last="Freitas">Vânia T. Freitas</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea></affiliation></author><author><name sortKey="Fu, Lianshe" sort="Fu, Lianshe" uniqKey="Fu L" first="Lianshe" last="Fu">Lianshe Fu</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea></affiliation></author><author><name sortKey="Cojocariu, Ana M" sort="Cojocariu, Ana M" uniqKey="Cojocariu A" first="Ana M" last="Cojocariu">Ana M. Cojocariu</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Cattoen, Xavier" sort="Cattoen, Xavier" uniqKey="Cattoen X" first="Xavier" last="Cattoën">Xavier Cattoën</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Bartlett, John R" sort="Bartlett, John R" uniqKey="Bartlett J" first="John R" last="Bartlett">John R. Bartlett</name><affiliation><nlm:affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</nlm:affiliation><wicri:noCountry code="subField">QLD 4558 Australia</wicri:noCountry></affiliation></author><author><name sortKey="Le Parc, Rozenn" sort="Le Parc, Rozenn" uniqKey="Le Parc R" first="Rozenn" last="Le Parc">Rozenn Le Parc</name><affiliation wicri:level="1"><nlm:affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Bantignies, Jean Louis" sort="Bantignies, Jean Louis" uniqKey="Bantignies J" first="Jean-Louis" last="Bantignies">Jean-Louis Bantignies</name><affiliation wicri:level="1"><nlm:affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Man, Michel Wong Chi" sort="Man, Michel Wong Chi" uniqKey="Man M" first="Michel Wong Chi" last="Man">Michel Wong Chi Man</name><affiliation wicri:level="1"><nlm:affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier</wicri:regionArea></affiliation></author><author><name sortKey="Andre, Paulo S" sort="Andre, Paulo S" uniqKey="Andre P" first="Paulo S" last="André">Paulo S. André</name><affiliation wicri:level="1"><nlm:affiliation>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa</wicri:regionArea></affiliation></author><author><name sortKey="Ferreira, Rute A S" sort="Ferreira, Rute A S" uniqKey="Ferreira R" first="Rute A S" last="Ferreira">Rute A S. Ferreira</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea></affiliation></author><author><name sortKey="Carlos, Luis D" sort="Carlos, Luis D" uniqKey="Carlos L" first="Luís D" last="Carlos">Luís D. Carlos</name><affiliation wicri:level="1"><nlm:affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</nlm:affiliation><country xml:lang="fr">Portugal</country><wicri:regionArea>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro</wicri:regionArea></affiliation></author></analytic><series><title level="j">ACS applied materials & interfaces</title><idno type="eISSN">1944-8252</idno><imprint><date when="2015" type="published">2015</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">25835303</PMID><DateCreated><Year>2015</Year><Month>04</Month><Day>29</Day></DateCreated><DateCompleted><Year>2015</Year><Month>08</Month><Day>12</Day></DateCompleted><DateRevised><Year>2015</Year><Month>04</Month><Day>29</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1944-8252</ISSN><JournalIssue CitedMedium="Internet"><Volume>7</Volume><Issue>16</Issue><PubDate><Year>2015</Year><Month>Apr</Month><Day>29</Day></PubDate></JournalIssue><Title>ACS applied materials & interfaces</Title><ISOAbbreviation>ACS Appl Mater Interfaces</ISOAbbreviation></Journal><ArticleTitle>Eu³⁺-based bridged silsesquioxanes for transparent luminescent solar concentrators.</ArticleTitle><Pagination><MedlinePgn>8770-8</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/acsami.5b01281</ELocationID><Abstract><AbstractText>The sol-gel preparation of a bridged silsesquioxane containing europium(III) salts and 2-thenoyltrifluoroacetone has been achieved from a new ethane tetracarboxamide-based organosilane. Free-standing films with thicknesses up to 440 μm and maximum absolute quantum yield (q) of 0.34 ± 0.03 (excitation at 320 nm) were prepared by the drop cast method, while thin films (∼200-400 nm) spin-coated on glass substrates led to highly luminescent coatings with q = 0.60 ± 0.02 (excitation at 345 nm). The thin films were tested as planar luminescent solar concentrators and the optimized device displays an optical conversion efficiency of 12.3% in the absorbing spectral region of the active layer (300-380 nm).</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Freitas</LastName><ForeName>Vânia T</ForeName><Initials>VT</Initials><AffiliationInfo><Affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Fu</LastName><ForeName>Lianshe</ForeName><Initials>L</Initials><AffiliationInfo><Affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Cojocariu</LastName><ForeName>Ana M</ForeName><Initials>AM</Initials><AffiliationInfo><Affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Cattoën</LastName><ForeName>Xavier</ForeName><Initials>X</Initials><AffiliationInfo><Affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>#Institut NEEL, CNRS, Université Grenoble-Alpes, 38042 Grenoble, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Bartlett</LastName><ForeName>John R</ForeName><Initials>JR</Initials><AffiliationInfo><Affiliation>⊥Faculty of Science, Health, Education and Engineering, University of the Sunshine Coast, Maroochydore DC, QLD 4558 Australia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Le Parc</LastName><ForeName>Rozenn</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Bantignies</LastName><ForeName>Jean-Louis</ForeName><Initials>JL</Initials><AffiliationInfo><Affiliation>‡Laboratoire Charles Coulomb (L2C), UMR 5521 CNRS-Université de Montpellier, 34095 Montpellier, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Man</LastName><ForeName>Michel Wong Chi</ForeName><Initials>MW</Initials><AffiliationInfo><Affiliation>§Institut Charles Gerhardt Montpellier, UMR 5253 CNRS-UM2-ENSCM-UM1, 34296 Montpellier, France.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>André</LastName><ForeName>Paulo S</ForeName><Initials>PS</Initials><AffiliationInfo><Affiliation>|| Department of Electric and Computer Engineering and Instituto de Telecomunicações, Instituto Superior Técnico, Universidade de Lisboa, Lisboa, Portugal.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Ferreira</LastName><ForeName>Rute A S</ForeName><Initials>RA</Initials><AffiliationInfo><Affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Carlos</LastName><ForeName>Luís D</ForeName><Initials>LD</Initials><AffiliationInfo><Affiliation>†Physics Department and CICECO Aveiro Institute of Materials, University of Aveiro, 3810-193 Aveiro, Portugal.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2015</Year><Month>04</Month><Day>14</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Appl Mater Interfaces</MedlineTA><NlmUniqueID>101504991</NlmUniqueID><ISSNLinking>1944-8244</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">lanthanide complex</Keyword><Keyword MajorTopicYN="N">luminescent solar concentrator</Keyword><Keyword MajorTopicYN="N">organic−inorganic hybrids</Keyword><Keyword MajorTopicYN="N">sol−gel</Keyword><Keyword MajorTopicYN="N">thin films</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2015</Year><Month>4</Month><Day>4</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate 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