Spectroscopic investigation of Tm3+:TeO2-WO3 glass
Identifieur interne : 000621 ( Pascal/Curation ); précédent : 000620; suivant : 000622Spectroscopic investigation of Tm3+:TeO2-WO3 glass
Auteurs : Hamit Kalaycioglu [Turquie] ; Huseyin Cankaya [Turquie] ; M. Natali Cizmeciyan [Turquie] ; Alphan Sennaroglu [Turquie] ; Gonul Ozen [Turquie]Source :
- Journal of luminescence [ 0022-2313 ] ; 2008.
Descripteurs français
- Pascal (Inist)
- Wicri :
- topic : Dopage.
English descriptors
- KwdEn :
Abstract
We studied the spectroscopic characteristics of telluride glass with the host composition (0.85)Te02-(0.15)W03, containing 0.25 and 1.0mol% thulium oxide (Tm2O3). By analyzing the absorption spectra with the Judd-Ofelt theory, the average radiative lifetimes of 305±7.5 μs and 1.95±0.02ms were determined for the 3F4 and 3H4 levels, respectively. Measured fluorescence lifetime of the 3F4 level decreased from 218 to 51 μs for the 0.25 and 1.0 mol% Tm2O3 doped samples, respectively, indicating the effect of boosted non-radiative decay at higher doping concentrations. A similar trend was observed for the 3H4 level, where the fluorescence lifetime decreased from 1.86ms to 350 μs at these concentrations. The quenching of the 1460nm (3F4→3H4) emission in favor of the 1800nm (3H4→3H6) emission due to cross relaxation was further evident in the fluorescence spectra of the samples. The calculated stimulated emission cross sections (3.73±0.1 x 10-21cm2 at 1460nm and 6.57±0.07 x 10-21cm2 at 1808nm) reveal the potential importance of the Tm3+:(0.85)TeO2-(0.15)WO3 glass for applications in fiber-optic amplifiers and fiber lasers.
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Spectroscopic investigation of Tm<sup>3+</sup>
:TeO<sub>2</sub>
-WO<sub>3</sub>
glass</title>
<author><name sortKey="Kalaycioglu, Hamit" sort="Kalaycioglu, Hamit" uniqKey="Kalaycioglu H" first="Hamit" last="Kalaycioglu">Hamit Kalaycioglu</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
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<country>Turquie</country>
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<author><name sortKey="Cankaya, Huseyin" sort="Cankaya, Huseyin" uniqKey="Cankaya H" first="Huseyin" last="Cankaya">Huseyin Cankaya</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
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<author><name sortKey="Cizmeciyan, M Natali" sort="Cizmeciyan, M Natali" uniqKey="Cizmeciyan M" first="M. Natali" last="Cizmeciyan">M. Natali Cizmeciyan</name>
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<s2>Sariyer, 34450 Istanbul</s2>
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<author><name sortKey="Sennaroglu, Alphan" sort="Sennaroglu, Alphan" uniqKey="Sennaroglu A" first="Alphan" last="Sennaroglu">Alphan Sennaroglu</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
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<author><name sortKey="Ozen, Gonul" sort="Ozen, Gonul" uniqKey="Ozen G" first="Gonul" last="Ozen">Gonul Ozen</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Physics, Istanbul Technical University</s1>
<s2>Maslak, 34469 Istanbul</s2>
<s3>TUR</s3>
<sZ>5 aut.</sZ>
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<country>Turquie</country>
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Spectroscopic investigation of Tm<sup>3+</sup>
:TeO<sub>2</sub>
-WO<sub>3</sub>
glass</title>
<author><name sortKey="Kalaycioglu, Hamit" sort="Kalaycioglu, Hamit" uniqKey="Kalaycioglu H" first="Hamit" last="Kalaycioglu">Hamit Kalaycioglu</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>Turquie</country>
</affiliation>
</author>
<author><name sortKey="Cankaya, Huseyin" sort="Cankaya, Huseyin" uniqKey="Cankaya H" first="Huseyin" last="Cankaya">Huseyin Cankaya</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>Turquie</country>
</affiliation>
</author>
<author><name sortKey="Cizmeciyan, M Natali" sort="Cizmeciyan, M Natali" uniqKey="Cizmeciyan M" first="M. Natali" last="Cizmeciyan">M. Natali Cizmeciyan</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>Turquie</country>
</affiliation>
</author>
<author><name sortKey="Sennaroglu, Alphan" sort="Sennaroglu, Alphan" uniqKey="Sennaroglu A" first="Alphan" last="Sennaroglu">Alphan Sennaroglu</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</inist:fA14>
<country>Turquie</country>
</affiliation>
</author>
<author><name sortKey="Ozen, Gonul" sort="Ozen, Gonul" uniqKey="Ozen G" first="Gonul" last="Ozen">Gonul Ozen</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Physics, Istanbul Technical University</s1>
<s2>Maslak, 34469 Istanbul</s2>
<s3>TUR</s3>
<sZ>5 aut.</sZ>
</inist:fA14>
<country>Turquie</country>
</affiliation>
</author>
</analytic>
<series><title level="j" type="main">Journal of luminescence</title>
<title level="j" type="abbreviated">J. lumin.</title>
<idno type="ISSN">0022-2313</idno>
<imprint><date when="2008">2008</date>
</imprint>
</series>
</biblStruct>
</sourceDesc>
<seriesStmt><title level="j" type="main">Journal of luminescence</title>
<title level="j" type="abbreviated">J. lumin.</title>
<idno type="ISSN">0022-2313</idno>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Absorption spectra</term>
<term>Binary systems</term>
<term>Chalcogenide glasses</term>
<term>Cross relaxation</term>
<term>Doping</term>
<term>Energy-level transitions</term>
<term>Fluorescence</term>
<term>Impurity density</term>
<term>Judd-Ofelt theory</term>
<term>Radiative lifetimes</term>
<term>Stimulated emission</term>
<term>Thulium additions</term>
<term>Tungstates</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Spectre absorption</term>
<term>Théorie Judd Ofelt</term>
<term>Durée vie radiative</term>
<term>Fluorescence</term>
<term>Addition thulium</term>
<term>Dopage</term>
<term>Concentration impureté</term>
<term>Transition niveau énergie</term>
<term>Relaxation croisée</term>
<term>Emission stimulée</term>
<term>Tungstate</term>
<term>Système binaire</term>
<term>Verre chalcogénure</term>
<term>Verre de tellurite</term>
</keywords>
<keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Dopage</term>
</keywords>
</textClass>
</profileDesc>
</teiHeader>
<front><div type="abstract" xml:lang="en">We studied the spectroscopic characteristics of telluride glass with the host composition (0.85)Te02-(0.15)W03, containing 0.25 and 1.0mol% thulium oxide (Tm<sub>2</sub>
O<sub>3</sub>
). By analyzing the absorption spectra with the Judd-Ofelt theory, the average radiative lifetimes of 305±7.5 μs and 1.95±0.02ms were determined for the <sup>3</sup>
F<sub>4</sub>
and <sup>3</sup>
H<sub>4</sub>
levels, respectively. Measured fluorescence lifetime of the <sup>3</sup>
F<sub>4</sub>
level decreased from 218 to 51 μs for the 0.25 and 1.0 mol% Tm<sub>2</sub>
O<sub>3</sub>
doped samples, respectively, indicating the effect of boosted non-radiative decay at higher doping concentrations. A similar trend was observed for the <sup>3</sup>
H<sub>4</sub>
level, where the fluorescence lifetime decreased from 1.86ms to 350 μs at these concentrations. The quenching of the 1460nm (<sup>3</sup>
F<sub>4</sub>
→<sup>3</sup>
H<sub>4</sub>
) emission in favor of the 1800nm (<sup>3</sup>
H<sub>4</sub>
→<sup>3</sup>
H<sub>6</sub>
) emission due to cross relaxation was further evident in the fluorescence spectra of the samples. The calculated stimulated emission cross sections (3.73±0.1 x 10<sup>-21</sup>
cm<sup>2</sup>
at 1460nm and 6.57±0.07 x 10<sup>-21</sup>
cm<sup>2</sup>
at 1808nm) reveal the potential importance of the Tm<sup>3+</sup>
:(0.85)TeO<sub>2</sub>
-(0.15)WO<sub>3</sub>
glass for applications in fiber-optic amplifiers and fiber lasers.</div>
</front>
</TEI>
<inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0022-2313</s0>
</fA01>
<fA02 i1="01"><s0>JLUMA8</s0>
</fA02>
<fA03 i2="1"><s0>J. lumin.</s0>
</fA03>
<fA05><s2>128</s2>
</fA05>
<fA06><s2>9</s2>
</fA06>
<fA08 i1="01" i2="1" l="ENG"><s1>Spectroscopic investigation of Tm<sup>3+</sup>
:TeO<sub>2</sub>
-WO<sub>3</sub>
glass</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>KALAYCIOGLU (Hamit)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>CANKAYA (Huseyin)</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>CIZMECIYAN (M. Natali)</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>SENNAROGLU (Alphan)</s1>
</fA11>
<fA11 i1="05" i2="1"><s1>OZEN (Gonul)</s1>
</fA11>
<fA14 i1="01"><s1>Laser Research Laboratory, Department of Physics, Koç University, Rumelifeneri Yolu</s1>
<s2>Sariyer, 34450 Istanbul</s2>
<s3>TUR</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>Department of Physics, Istanbul Technical University</s1>
<s2>Maslak, 34469 Istanbul</s2>
<s3>TUR</s3>
<sZ>5 aut.</sZ>
</fA14>
<fA20><s1>1501-1506</s1>
</fA20>
<fA21><s1>2008</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>14666</s2>
<s5>354000196028620200</s5>
</fA43>
<fA44><s0>0000</s0>
<s1>© 2008 INIST-CNRS. All rights reserved.</s1>
</fA44>
<fA45><s0>25 ref.</s0>
</fA45>
<fA47 i1="01" i2="1"><s0>08-0383061</s0>
</fA47>
<fA60><s1>P</s1>
</fA60>
<fA61><s0>A</s0>
</fA61>
<fA64 i1="01" i2="1"><s0>Journal of luminescence</s0>
</fA64>
<fA66 i1="01"><s0>NLD</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>We studied the spectroscopic characteristics of telluride glass with the host composition (0.85)Te02-(0.15)W03, containing 0.25 and 1.0mol% thulium oxide (Tm<sub>2</sub>
O<sub>3</sub>
). By analyzing the absorption spectra with the Judd-Ofelt theory, the average radiative lifetimes of 305±7.5 μs and 1.95±0.02ms were determined for the <sup>3</sup>
F<sub>4</sub>
and <sup>3</sup>
H<sub>4</sub>
levels, respectively. Measured fluorescence lifetime of the <sup>3</sup>
F<sub>4</sub>
level decreased from 218 to 51 μs for the 0.25 and 1.0 mol% Tm<sub>2</sub>
O<sub>3</sub>
doped samples, respectively, indicating the effect of boosted non-radiative decay at higher doping concentrations. A similar trend was observed for the <sup>3</sup>
H<sub>4</sub>
level, where the fluorescence lifetime decreased from 1.86ms to 350 μs at these concentrations. The quenching of the 1460nm (<sup>3</sup>
F<sub>4</sub>
→<sup>3</sup>
H<sub>4</sub>
) emission in favor of the 1800nm (<sup>3</sup>
H<sub>4</sub>
→<sup>3</sup>
H<sub>6</sub>
) emission due to cross relaxation was further evident in the fluorescence spectra of the samples. The calculated stimulated emission cross sections (3.73±0.1 x 10<sup>-21</sup>
cm<sup>2</sup>
at 1460nm and 6.57±0.07 x 10<sup>-21</sup>
cm<sup>2</sup>
at 1808nm) reveal the potential importance of the Tm<sup>3+</sup>
:(0.85)TeO<sub>2</sub>
-(0.15)WO<sub>3</sub>
glass for applications in fiber-optic amplifiers and fiber lasers.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001B70H55Q</s0>
</fC02>
<fC03 i1="01" i2="3" l="FRE"><s0>Spectre absorption</s0>
<s5>02</s5>
</fC03>
<fC03 i1="01" i2="3" l="ENG"><s0>Absorption spectra</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="3" l="FRE"><s0>Théorie Judd Ofelt</s0>
<s5>03</s5>
</fC03>
<fC03 i1="02" i2="3" l="ENG"><s0>Judd-Ofelt theory</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="3" l="FRE"><s0>Durée vie radiative</s0>
<s5>04</s5>
</fC03>
<fC03 i1="03" i2="3" l="ENG"><s0>Radiative lifetimes</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Fluorescence</s0>
<s5>05</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Fluorescence</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="3" l="FRE"><s0>Addition thulium</s0>
<s5>06</s5>
</fC03>
<fC03 i1="05" i2="3" l="ENG"><s0>Thulium additions</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE"><s0>Dopage</s0>
<s5>07</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Doping</s0>
<s5>07</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Doping</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Concentration impureté</s0>
<s5>08</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Impurity density</s0>
<s5>08</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Concentración impureza</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="3" l="FRE"><s0>Transition niveau énergie</s0>
<s5>09</s5>
</fC03>
<fC03 i1="08" i2="3" l="ENG"><s0>Energy-level transitions</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Relaxation croisée</s0>
<s5>10</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Cross relaxation</s0>
<s5>10</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Relajación cruzada</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Emission stimulée</s0>
<s5>11</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>Stimulated emission</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="3" l="FRE"><s0>Tungstate</s0>
<s2>NA</s2>
<s5>15</s5>
</fC03>
<fC03 i1="11" i2="3" l="ENG"><s0>Tungstates</s0>
<s2>NA</s2>
<s5>15</s5>
</fC03>
<fC03 i1="12" i2="3" l="FRE"><s0>Système binaire</s0>
<s5>16</s5>
</fC03>
<fC03 i1="12" i2="3" l="ENG"><s0>Binary systems</s0>
<s5>16</s5>
</fC03>
<fC03 i1="13" i2="3" l="FRE"><s0>Verre chalcogénure</s0>
<s5>17</s5>
</fC03>
<fC03 i1="13" i2="3" l="ENG"><s0>Chalcogenide glasses</s0>
<s5>17</s5>
</fC03>
<fC03 i1="14" i2="3" l="FRE"><s0>Verre de tellurite</s0>
<s4>INC</s4>
<s5>63</s5>
</fC03>
<fN21><s1>245</s1>
</fN21>
</pA>
</standard>
</inist>
</record>
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