Linking the thermodynamic temperature to an optical frequency: recent advances in Doppler broadening thermometry
Identifieur interne : 000B15 ( Ncbi/Curation ); précédent : 000B14; suivant : 000B16Linking the thermodynamic temperature to an optical frequency: recent advances in Doppler broadening thermometry
Auteurs : Livio Gianfrani [Italie]Source :
- Philosophical transactions. Series A, Mathematical, physical, and engineering sciences [ 1364-503X ] ; 2016.
Abstract
Laser spectroscopy in the linear regime of radiation–matter interaction is a powerful tool for measuring thermodynamic quantities in a gas at thermodynamic equilibrium. In particular, the Doppler effect can be considered a gift of nature, linking the thermal energy to an optical frequency, namely the line centre frequency of an atomic or molecular spectral line. This is the basis of a relatively new method of primary gas thermometry, known as Doppler broadening thermometry (DBT). This paper reports on the efforts that have been carried out, in the last decade, worldwide, to the end of making DBT competitive with more consolidated and accurate methodologies, such as acoustic gas thermometry and dielectric constant gas thermometry. The main requirements for low-uncertainty DBT, of both theoretical and technical nature, will be discussed, with a special focus on those related to the line shape model and to the frequency scale. A deep comparison among the different molecules that have been selected in successful DBT implementations is also reported. Finally, for the first time, to the best of my knowledge, the influence of refractive index effects is discussed.
Url:
DOI: 10.1098/rsta.2015.0047
PubMed: 26903093
PubMed Central: 4760123
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PMC:4760123Le document en format XML
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<front><div type="abstract" xml:lang="en"><p>Laser spectroscopy in the linear regime of radiation–matter interaction is a powerful tool for measuring thermodynamic quantities in a gas at thermodynamic equilibrium. In particular, the Doppler effect can be considered a gift of nature, linking the thermal energy to an optical frequency, namely the line centre frequency of an atomic or molecular spectral line. This is the basis of a relatively new method of primary gas thermometry, known as Doppler broadening thermometry (DBT). This paper reports on the efforts that have been carried out, in the last decade, worldwide, to the end of making DBT competitive with more consolidated and accurate methodologies, such as acoustic gas thermometry and dielectric constant gas thermometry. The main requirements for low-uncertainty DBT, of both theoretical and technical nature, will be discussed, with a special focus on those related to the line shape model and to the frequency scale. A deep comparison among the different molecules that have been selected in successful DBT implementations is also reported. Finally, for the first time, to the best of my knowledge, the influence of refractive index effects is discussed.</p>
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