Use of thulium-sensitized rare earth-doped low phonon energy crystalline hosts for IR sources
Identifieur interne : 000759 ( Ncbi/Curation ); précédent : 000758; suivant : 000760Use of thulium-sensitized rare earth-doped low phonon energy crystalline hosts for IR sources
Auteurs : Joseph Ganem [États-Unis] ; Steven R. Bowman [États-Unis]Source :
- Nanoscale Research Letters [ 1931-7573 ] ; 2013.
Abstract
Crystalline hosts with low phonon energies enable novel energy transfer processes when doped with rare earth ions. Two applications of energy transfer for rare earth ions in thulium-sensitized low phonon energy crystals that result in infrared luminescence are discussed. One application is an endothermic, phonon-assisted cross-relaxation process in thulium-doped yttrium chloride that converts lattice phonons to infrared emission, which raises the possibility of a fundamentally new method for achieving solid-state optical cooling. The other application is an optically pumped mid-IR phosphor using thulium-praseodymium-doped potassium lead chloride that converts 805-nm diode light to broadband emission from 4,000 to 5,500 nm. These two applications in chloride crystals are discussed in terms of critical radii calculated from Forster-Dexter energy transfer theory. It is found that the critical radii for electric dipole-dipole interactions in low phonon energy chloride crystals are comparable to those in conventional oxide and fluoride crystals. It is the reduction in multi-phonon relaxation rates in chloride crystals that enable these additional energy transfer processes and infrared luminescence.
Url:
DOI: 10.1186/1556-276X-8-455
PubMed: 24180684
PubMed Central: 4228387
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Charles Street, Baltimore, MD 21210, USA</nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea>Department of Physics, Loyola University Maryland, 4501 N. Charles Street, Baltimore, MD 21210</wicri:regionArea><placeName><region type="state">Maryland</region></placeName></affiliation></author><author><name sortKey="Bowman, Steven R" sort="Bowman, Steven R" uniqKey="Bowman S" first="Steven R" last="Bowman">Steven R. Bowman</name><affiliation wicri:level="2"><nlm:aff id="I2">Optical Sciences Division, Naval Research Laboratory, 4555 Overlook Avenue SW, Washington, DC 20375, USA</nlm:aff><country xml:lang="fr">États-Unis</country><wicri:regionArea>Optical Sciences Division, Naval Research Laboratory, 4555 Overlook Avenue SW, Washington, DC 20375</wicri:regionArea><placeName><region type="state">District de Columbia</region></placeName></affiliation></author></analytic><series><title level="j">Nanoscale Research Letters</title><idno type="ISSN">1931-7573</idno><idno type="eISSN">1556-276X</idno><imprint><date when="2013">2013</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>Crystalline hosts with low phonon energies enable novel energy transfer processes when doped with rare earth ions. Two applications of energy transfer for rare earth ions in thulium-sensitized low phonon energy crystals that result in infrared luminescence are discussed. One application is an endothermic, phonon-assisted cross-relaxation process in thulium-doped yttrium chloride that converts lattice phonons to infrared emission, which raises the possibility of a fundamentally new method for achieving solid-state optical cooling. The other application is an optically pumped mid-IR phosphor using thulium-praseodymium-doped potassium lead chloride that converts 805-nm diode light to broadband emission from 4,000 to 5,500 nm. These two applications in chloride crystals are discussed in terms of critical radii calculated from Forster-Dexter energy transfer theory. It is found that the critical radii for electric dipole-dipole interactions in low phonon energy chloride crystals are comparable to those in conventional oxide and fluoride crystals. It is the reduction in multi-phonon relaxation rates in chloride crystals that enable these additional energy transfer processes and infrared luminescence.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Kosterev, A" uniqKey="Kosterev A">A Kosterev</name></author><author><name sortKey="Wysocki, G" uniqKey="Wysocki G">G Wysocki</name></author><author><name sortKey="Bakhirkin, Y" uniqKey="Bakhirkin Y">Y Bakhirkin</name></author><author><name sortKey="So, S" uniqKey="So S">S So</name></author><author><name sortKey="Lewicki, R" uniqKey="Lewicki R">R Lewicki</name></author><author><name sortKey="Fraser, M" uniqKey="Fraser M">M Fraser</name></author><author><name sortKey="Tittel, F" uniqKey="Tittel F">F Tittel</name></author><author><name sortKey="Curl, Rf" uniqKey="Curl R">RF Curl</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Aidaraliev, M" uniqKey="Aidaraliev M">M 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A">AJ Gareia</name></author><author><name sortKey="Balda, R" uniqKey="Balda R">R Balda</name></author><author><name sortKey="Adam, Jl" uniqKey="Adam J">JL Adam</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Bluiett, Ag" uniqKey="Bluiett A">AG Bluiett</name></author><author><name sortKey="Condon, Nj" uniqKey="Condon N">NJ Condon</name></author><author><name sortKey="O Connor, S" uniqKey="O Connor S">S O'Connor</name></author><author><name sortKey="Bowman, Sr" uniqKey="Bowman S">SR Bowman</name></author><author><name sortKey="Logie, M" uniqKey="Logie M">M Logie</name></author><author><name sortKey="Ganem, J" uniqKey="Ganem J">J Ganem</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Murdoch, Km" uniqKey="Murdoch K">KM Murdoch</name></author><author><name sortKey="Cockroft, Nj" uniqKey="Cockroft N">NJ Cockroft</name></author></analytic></biblStruct></listBibl></div1></back></TEI></record>Pour manipuler ce document sous 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