Catalytic activity of some organolanthanoid derivatives in styrene and propene polymerization
Identifieur interne : 002092 ( Main/Exploration ); précédent : 002091; suivant : 002093Catalytic activity of some organolanthanoid derivatives in styrene and propene polymerization
Auteurs : Evgueni N. Kirillov [Russie] ; Elena A. Fedorova [Russie] ; Alexander A. Trifonov [Russie] ; Mikhail N. Bochkarev [Russie]Source :
- Applied Organometallic Chemistry [ 0268-2605 ] ; 2001-03.
Descripteurs français
- Pascal (Inist)
- Wicri :
- topic : Droit d'auteur, Méthanol, Polymère.
English descriptors
- KwdEn :
- Acad, Amide, Appl, Bochkarev, Bulk polymerization, Catalyst activity, Catalytic activity, Chem, Complex catalyst, Complex catalyst polymerization, Conversion rate, Copyright, Derivative, Divalent, Europium, Experimental study, Fedorova, Hydride, John wiley sons, Kirillov, Lanthanide Complexes, Lanthanoid, Methanol, Molecular hydrides, Molecular weights, Naphthalene, Nauk, Organic ligand, Organolanthanoid, Organolanthanoid derivatives, Organolanthanoids, Organomet, Organometal, Organometallic, Organometallic chemistry, Organometallics, Polymer, Propene, Propene polymerization, Propylene polymer, Room temperature, Samarium, Schumann, Solution polymerization, Stilbene, Stilbene complexes, Styrene polymer, Styrene polymerization, Toluene, Trifonov, Ytterbium, Zakharov.
- Teeft :
- Acad, Amide, Appl, Bochkarev, Catalytic activity, Chem, Copyright, Derivative, Divalent, Europium, Fedorova, Hydride, John wiley sons, Kirillov, Lanthanoid, Methanol, Molecular hydrides, Molecular weights, Naphthalene, Nauk, Organolanthanoid, Organolanthanoid derivatives, Organolanthanoids, Organomet, Organometal, Organometallic, Organometallic chemistry, Organometallics, Polymer, Propene, Propene polymerization, Room temperature, Samarium, Schumann, Stilbene, Stilbene complexes, Styrene polymerization, Toluene, Trifonov, Ytterbium, Zakharov.
Abstract
Organolanthanoids of several classes were examined as potential styrene and propene polymerization catalysts. They are: molecular hydrides of divalent lanthanoids (samarium, europium, ytterbium); naphthalene and stilbene complexes of neodymium(III), samarium(II), europium(II), ytterbium(II), lutetium(III); amides and alkoxides (including heterobifunctional derivatives) of praseodymium(III), neodymium(III), samarium(II), europium(II), thulium(III), ytterbium(II, III); thiolate of samarium(III); phenyl and phenylethinyl derivatives of europium(II), thulium(III), ytterbium(II); methylytterbium cluster Yb8 (μ‐CH3)14(μ‐CH2)(THF)6; heterobimetallic samarium(II), ytterbium(II, III) complexes; diazabutadiene ytterbium(III) derivatives; metallic praseodymium and ytterbium, activated by iodine. The highest activity in styrene polymerization revealed hydrides, naphthalene and stilbene complexes of samarium(II), europium(II) and ytterbium(II). In the propene polymerization only [(η5‐C5H4)CH2CH(CH2OBu)(η1‐O)]YbMe(THF) displayed noticeable activity.Copyright © 2001 John Wiley & Sons, Ltd.
Url:
DOI: 10.1002/aoc.123
Affiliations:
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<term>Amide</term>
<term>Appl</term>
<term>Bochkarev</term>
<term>Bulk polymerization</term>
<term>Catalyst activity</term>
<term>Catalytic activity</term>
<term>Chem</term>
<term>Complex catalyst</term>
<term>Complex catalyst polymerization</term>
<term>Conversion rate</term>
<term>Copyright</term>
<term>Derivative</term>
<term>Divalent</term>
<term>Europium</term>
<term>Experimental study</term>
<term>Fedorova</term>
<term>Hydride</term>
<term>John wiley sons</term>
<term>Kirillov</term>
<term>Lanthanide Complexes</term>
<term>Lanthanoid</term>
<term>Methanol</term>
<term>Molecular hydrides</term>
<term>Molecular weights</term>
<term>Naphthalene</term>
<term>Nauk</term>
<term>Organic ligand</term>
<term>Organolanthanoid</term>
<term>Organolanthanoid derivatives</term>
<term>Organolanthanoids</term>
<term>Organomet</term>
<term>Organometal</term>
<term>Organometallic</term>
<term>Organometallic chemistry</term>
<term>Organometallics</term>
<term>Polymer</term>
<term>Propene</term>
<term>Propene polymerization</term>
<term>Propylene polymer</term>
<term>Room temperature</term>
<term>Samarium</term>
<term>Schumann</term>
<term>Solution polymerization</term>
<term>Stilbene</term>
<term>Stilbene complexes</term>
<term>Styrene polymer</term>
<term>Styrene polymerization</term>
<term>Toluene</term>
<term>Trifonov</term>
<term>Ytterbium</term>
<term>Zakharov</term>
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<keywords scheme="Pascal" xml:lang="fr"><term>Activité catalytique</term>
<term>Catalyseur complexe</term>
<term>Coordinat organique</term>
<term>Etude expérimentale</term>
<term>Lanthanide Complexe</term>
<term>Polymérisation catalyseur complexe</term>
<term>Polymérisation masse</term>
<term>Polymérisation solution</term>
<term>Propène polymère</term>
<term>Styrène polymère</term>
<term>Taux conversion</term>
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<term>Copyright</term>
<term>Derivative</term>
<term>Divalent</term>
<term>Europium</term>
<term>Fedorova</term>
<term>Hydride</term>
<term>John wiley sons</term>
<term>Kirillov</term>
<term>Lanthanoid</term>
<term>Methanol</term>
<term>Molecular hydrides</term>
<term>Molecular weights</term>
<term>Naphthalene</term>
<term>Nauk</term>
<term>Organolanthanoid</term>
<term>Organolanthanoid derivatives</term>
<term>Organolanthanoids</term>
<term>Organomet</term>
<term>Organometal</term>
<term>Organometallic</term>
<term>Organometallic chemistry</term>
<term>Organometallics</term>
<term>Polymer</term>
<term>Propene</term>
<term>Propene polymerization</term>
<term>Room temperature</term>
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<term>Trifonov</term>
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<term>Polymère</term>
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<front><div type="abstract" xml:lang="en">Organolanthanoids of several classes were examined as potential styrene and propene polymerization catalysts. They are: molecular hydrides of divalent lanthanoids (samarium, europium, ytterbium); naphthalene and stilbene complexes of neodymium(III), samarium(II), europium(II), ytterbium(II), lutetium(III); amides and alkoxides (including heterobifunctional derivatives) of praseodymium(III), neodymium(III), samarium(II), europium(II), thulium(III), ytterbium(II, III); thiolate of samarium(III); phenyl and phenylethinyl derivatives of europium(II), thulium(III), ytterbium(II); methylytterbium cluster Yb8 (μ‐CH3)14(μ‐CH2)(THF)6; heterobimetallic samarium(II), ytterbium(II, III) complexes; diazabutadiene ytterbium(III) derivatives; metallic praseodymium and ytterbium, activated by iodine. The highest activity in styrene polymerization revealed hydrides, naphthalene and stilbene complexes of samarium(II), europium(II) and ytterbium(II). In the propene polymerization only [(η5‐C5H4)CH2CH(CH2OBu)(η1‐O)]YbMe(THF) displayed noticeable activity.Copyright © 2001 John Wiley & Sons, Ltd.</div>
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