Thorn-like flexible Ag2C2O4/TiO2 nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.
Identifieur interne : 000029 ( Main/Exploration ); précédent : 000028; suivant : 000030Thorn-like flexible Ag2C2O4/TiO2 nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.
Auteurs : Xiaohui Wu [République populaire de Chine] ; Leitao Cao [République populaire de Chine] ; Jun Song [République populaire de Chine] ; Yang Si [République populaire de Chine] ; Jianyong Yu [République populaire de Chine] ; Bin Ding [République populaire de Chine]Source :
- Journal of colloid and interface science [ 1095-7103 ] ; 2020.
Descripteurs français
- KwdFr :
- Adsorption (MeSH), Antibactériens (composition chimique), Antibactériens (pharmacologie), Catalyse (MeSH), Composés de l'argent (composition chimique), Composés de l'argent (pharmacologie), Désinfection (MeSH), Escherichia coli (croissance et développement), Escherichia coli (effets des médicaments et des substances chimiques), Lumière (MeSH), Nanofibres (composition chimique), Nanoparticules métalliques (composition chimique), Processus photochimiques (MeSH), Titane (composition chimique), Titane (pharmacologie).
- MESH :
- composition chimique : Antibactériens, Composés de l'argent, Nanofibres, Nanoparticules métalliques, Titane.
- croissance et développement : Escherichia coli.
- effets des médicaments et des substances chimiques : Escherichia coli.
- pharmacologie : Antibactériens, Composés de l'argent, Titane.
- Adsorption, Catalyse, Désinfection, Lumière, Processus photochimiques.
English descriptors
- KwdEn :
- Adsorption (MeSH), Anti-Bacterial Agents (chemistry), Anti-Bacterial Agents (pharmacology), Catalysis (MeSH), Disinfection (MeSH), Escherichia coli (drug effects), Escherichia coli (growth & development), Light (MeSH), Metal Nanoparticles (chemistry), Nanofibers (chemistry), Photochemical Processes (MeSH), Silver Compounds (chemistry), Silver Compounds (pharmacology), Titanium (chemistry), Titanium (pharmacology).
- MESH :
- chemical , chemistry : Anti-Bacterial Agents, Silver Compounds, Titanium.
- chemical , pharmacology : Anti-Bacterial Agents, Silver Compounds, Titanium.
- chemistry : Metal Nanoparticles, Nanofibers.
- drug effects : Escherichia coli.
- growth & development : Escherichia coli.
- Adsorption, Catalysis, Disinfection, Light, Photochemical Processes.
Abstract
TiO2-based fibrous membranes as plasmonic heterojunction photocatalysts would hold great promise in the field of water disinfection, however, it still existed a great challenge to design and construct such materials. Here, we presented the fabrication of continuous, hierarchical, and easy-to-recycle flexible Ag2C2O4/TiO2 heterostructured nanofibrous membranes (NMs) that were composed of thorn-like nanofibers through electrospinning technique followed by successive ionic layer adsorption and reaction (SILAR) process. Ag2C2O4 nanoplates were firmly anchored on the surface of TiO2 and the obtained Ag2C2O4/TiO2 heterojunction photocatalysts underwent a silent-to-active transition of visible-light response under light irradiation due to the surface plasmon resonance (SPR) effect of Ag nanoparticles derived from Ag2C2O4, forming a new plasmonic heterojunction photocatalyst. By virtue of the hierarchical structure, enhanced visible light absorption and efficient charge carriers separation, Ag2C2O4/TiO2 NMs possessed high bactericidal efficiency of >99.999% within 30 min, strong reactive oxygen species (ROS) producing capability (1510 μg g-1 and 659 μg g-1 for superoxide radicals and hydroxyl radicals, respectively), and good reusability. This work may offer new insights into the design of antibacterial materials for pathogenic microorganism-contaminated water purification.
DOI: 10.1016/j.jcis.2019.10.119
PubMed: 31706650
Affiliations:
Links toward previous steps (curation, corpus...)
Le document en format XML
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C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.</title>
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C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.</title>
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<term>Anti-Bacterial Agents (chemistry)</term>
<term>Anti-Bacterial Agents (pharmacology)</term>
<term>Catalysis (MeSH)</term>
<term>Disinfection (MeSH)</term>
<term>Escherichia coli (drug effects)</term>
<term>Escherichia coli (growth & development)</term>
<term>Light (MeSH)</term>
<term>Metal Nanoparticles (chemistry)</term>
<term>Nanofibers (chemistry)</term>
<term>Photochemical Processes (MeSH)</term>
<term>Silver Compounds (chemistry)</term>
<term>Silver Compounds (pharmacology)</term>
<term>Titanium (chemistry)</term>
<term>Titanium (pharmacology)</term>
</keywords>
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<term>Antibactériens (composition chimique)</term>
<term>Antibactériens (pharmacologie)</term>
<term>Catalyse (MeSH)</term>
<term>Composés de l'argent (composition chimique)</term>
<term>Composés de l'argent (pharmacologie)</term>
<term>Désinfection (MeSH)</term>
<term>Escherichia coli (croissance et développement)</term>
<term>Escherichia coli (effets des médicaments et des substances chimiques)</term>
<term>Lumière (MeSH)</term>
<term>Nanofibres (composition chimique)</term>
<term>Nanoparticules métalliques (composition chimique)</term>
<term>Processus photochimiques (MeSH)</term>
<term>Titane (composition chimique)</term>
<term>Titane (pharmacologie)</term>
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<term>Silver Compounds</term>
<term>Titanium</term>
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<keywords scheme="MESH" type="chemical" qualifier="pharmacology" xml:lang="en"><term>Anti-Bacterial Agents</term>
<term>Silver Compounds</term>
<term>Titanium</term>
</keywords>
<keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Metal Nanoparticles</term>
<term>Nanofibers</term>
</keywords>
<keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Antibactériens</term>
<term>Composés de l'argent</term>
<term>Nanofibres</term>
<term>Nanoparticules métalliques</term>
<term>Titane</term>
</keywords>
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</keywords>
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<term>Composés de l'argent</term>
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<term>Disinfection</term>
<term>Light</term>
<term>Photochemical Processes</term>
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<term>Catalyse</term>
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<front><div type="abstract" xml:lang="en">TiO<sub>2</sub>
-based fibrous membranes as plasmonic heterojunction photocatalysts would hold great promise in the field of water disinfection, however, it still existed a great challenge to design and construct such materials. Here, we presented the fabrication of continuous, hierarchical, and easy-to-recycle flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterostructured nanofibrous membranes (NMs) that were composed of thorn-like nanofibers through electrospinning technique followed by successive ionic layer adsorption and reaction (SILAR) process. Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
nanoplates were firmly anchored on the surface of TiO<sub>2</sub>
and the obtained Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterojunction photocatalysts underwent a silent-to-active transition of visible-light response under light irradiation due to the surface plasmon resonance (SPR) effect of Ag nanoparticles derived from Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
, forming a new plasmonic heterojunction photocatalyst. By virtue of the hierarchical structure, enhanced visible light absorption and efficient charge carriers separation, Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
NMs possessed high bactericidal efficiency of >99.999% within 30 min, strong reactive oxygen species (ROS) producing capability (1510 μg g<sup>-1</sup>
and 659 μg g<sup>-1</sup>
for superoxide radicals and hydroxyl radicals, respectively), and good reusability. This work may offer new insights into the design of antibacterial materials for pathogenic microorganism-contaminated water purification.</div>
</front>
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<DateCompleted><Year>2020</Year>
<Month>06</Month>
<Day>15</Day>
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<DateRevised><Year>2020</Year>
<Month>06</Month>
<Day>15</Day>
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<JournalIssue CitedMedium="Internet"><Volume>560</Volume>
<PubDate><Year>2020</Year>
<Month>Feb</Month>
<Day>15</Day>
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</JournalIssue>
<Title>Journal of colloid and interface science</Title>
<ISOAbbreviation>J Colloid Interface Sci</ISOAbbreviation>
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<ArticleTitle>Thorn-like flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.</ArticleTitle>
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<Abstract><AbstractText>TiO<sub>2</sub>
-based fibrous membranes as plasmonic heterojunction photocatalysts would hold great promise in the field of water disinfection, however, it still existed a great challenge to design and construct such materials. Here, we presented the fabrication of continuous, hierarchical, and easy-to-recycle flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterostructured nanofibrous membranes (NMs) that were composed of thorn-like nanofibers through electrospinning technique followed by successive ionic layer adsorption and reaction (SILAR) process. Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
nanoplates were firmly anchored on the surface of TiO<sub>2</sub>
and the obtained Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterojunction photocatalysts underwent a silent-to-active transition of visible-light response under light irradiation due to the surface plasmon resonance (SPR) effect of Ag nanoparticles derived from Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
, forming a new plasmonic heterojunction photocatalyst. By virtue of the hierarchical structure, enhanced visible light absorption and efficient charge carriers separation, Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
NMs possessed high bactericidal efficiency of >99.999% within 30 min, strong reactive oxygen species (ROS) producing capability (1510 μg g<sup>-1</sup>
and 659 μg g<sup>-1</sup>
for superoxide radicals and hydroxyl radicals, respectively), and good reusability. This work may offer new insights into the design of antibacterial materials for pathogenic microorganism-contaminated water purification.</AbstractText>
<CopyrightInformation>Copyright © 2019 Elsevier Inc. All rights reserved.</CopyrightInformation>
</Abstract>
<AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Wu</LastName>
<ForeName>Xiaohui</ForeName>
<Initials>X</Initials>
<AffiliationInfo><Affiliation>State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Textiles, Donghua University, Shanghai 201620, China.</Affiliation>
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</AffiliationInfo>
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<AffiliationInfo><Affiliation>Innovation Center for Textile Science and Technology, Donghua University, Shanghai 200051, China.</Affiliation>
</AffiliationInfo>
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<Author ValidYN="Y"><LastName>Si</LastName>
<ForeName>Yang</ForeName>
<Initials>Y</Initials>
<AffiliationInfo><Affiliation>State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Textiles, Donghua University, Shanghai 201620, China; Innovation Center for Textile Science and Technology, Donghua University, Shanghai 200051, China. Electronic address: yangsi@dhu.edu.cn.</Affiliation>
</AffiliationInfo>
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<Author ValidYN="Y"><LastName>Yu</LastName>
<ForeName>Jianyong</ForeName>
<Initials>J</Initials>
<AffiliationInfo><Affiliation>Innovation Center for Textile Science and Technology, Donghua University, Shanghai 200051, China.</Affiliation>
</AffiliationInfo>
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<Author ValidYN="Y"><LastName>Ding</LastName>
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<Initials>B</Initials>
<AffiliationInfo><Affiliation>State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Textiles, Donghua University, Shanghai 201620, China; Innovation Center for Textile Science and Technology, Donghua University, Shanghai 200051, China. Electronic address: binding@dhu.edu.cn.</Affiliation>
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<Month>11</Month>
<Day>02</Day>
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<MeshHeadingList><MeshHeading><DescriptorName UI="D000327" MajorTopicYN="N">Adsorption</DescriptorName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D000900" MajorTopicYN="N">Anti-Bacterial Agents</DescriptorName>
<QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName>
<QualifierName UI="Q000494" MajorTopicYN="Y">pharmacology</QualifierName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D002384" MajorTopicYN="N">Catalysis</DescriptorName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D004203" MajorTopicYN="N">Disinfection</DescriptorName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D004926" MajorTopicYN="N">Escherichia coli</DescriptorName>
<QualifierName UI="Q000187" MajorTopicYN="N">drug effects</QualifierName>
<QualifierName UI="Q000254" MajorTopicYN="Y">growth & development</QualifierName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D008027" MajorTopicYN="N">Light</DescriptorName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D053768" MajorTopicYN="N">Metal Nanoparticles</DescriptorName>
<QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D057139" MajorTopicYN="N">Nanofibers</DescriptorName>
<QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D055668" MajorTopicYN="N">Photochemical Processes</DescriptorName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D018030" MajorTopicYN="N">Silver Compounds</DescriptorName>
<QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName>
<QualifierName UI="Q000494" MajorTopicYN="Y">pharmacology</QualifierName>
</MeshHeading>
<MeshHeading><DescriptorName UI="D014025" MajorTopicYN="N">Titanium</DescriptorName>
<QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName>
<QualifierName UI="Q000494" MajorTopicYN="Y">pharmacology</QualifierName>
</MeshHeading>
</MeshHeadingList>
<KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Ag(2)C(2)O(4)/TiO(2)</Keyword>
<Keyword MajorTopicYN="N">Bacteria-killing</Keyword>
<Keyword MajorTopicYN="N">Heterostructured photocatalysts</Keyword>
<Keyword MajorTopicYN="N">Nanofirous membranes</Keyword>
<Keyword MajorTopicYN="N">Visible light</Keyword>
</KeywordList>
</MedlineCitation>
<PubmedData><History><PubMedPubDate PubStatus="received"><Year>2019</Year>
<Month>10</Month>
<Day>08</Day>
</PubMedPubDate>
<PubMedPubDate PubStatus="revised"><Year>2019</Year>
<Month>10</Month>
<Day>27</Day>
</PubMedPubDate>
<PubMedPubDate PubStatus="accepted"><Year>2019</Year>
<Month>10</Month>
<Day>31</Day>
</PubMedPubDate>
<PubMedPubDate PubStatus="pubmed"><Year>2019</Year>
<Month>11</Month>
<Day>11</Day>
<Hour>6</Hour>
<Minute>0</Minute>
</PubMedPubDate>
<PubMedPubDate PubStatus="medline"><Year>2020</Year>
<Month>6</Month>
<Day>17</Day>
<Hour>6</Hour>
<Minute>0</Minute>
</PubMedPubDate>
<PubMedPubDate PubStatus="entrez"><Year>2019</Year>
<Month>11</Month>
<Day>11</Day>
<Hour>6</Hour>
<Minute>0</Minute>
</PubMedPubDate>
</History>
<PublicationStatus>ppublish</PublicationStatus>
<ArticleIdList><ArticleId IdType="pubmed">31706650</ArticleId>
<ArticleId IdType="pii">S0021-9797(19)31313-X</ArticleId>
<ArticleId IdType="doi">10.1016/j.jcis.2019.10.119</ArticleId>
</ArticleIdList>
</PubmedData>
</pubmed>
<affiliations><list><country><li>République populaire de Chine</li>
</country>
<region><li>Shanghai</li>
</region>
<settlement><li>Shanghai</li>
</settlement>
<orgName><li>Université Donghua</li>
</orgName>
</list>
<tree><country name="République populaire de Chine"><region name="Shanghai"><name sortKey="Wu, Xiaohui" sort="Wu, Xiaohui" uniqKey="Wu X" first="Xiaohui" last="Wu">Xiaohui Wu</name>
</region>
<name sortKey="Cao, Leitao" sort="Cao, Leitao" uniqKey="Cao L" first="Leitao" last="Cao">Leitao Cao</name>
<name sortKey="Ding, Bin" sort="Ding, Bin" uniqKey="Ding B" first="Bin" last="Ding">Bin Ding</name>
<name sortKey="Si, Yang" sort="Si, Yang" uniqKey="Si Y" first="Yang" last="Si">Yang Si</name>
<name sortKey="Song, Jun" sort="Song, Jun" uniqKey="Song J" first="Jun" last="Song">Jun Song</name>
<name sortKey="Yu, Jianyong" sort="Yu, Jianyong" uniqKey="Yu J" first="Jianyong" last="Yu">Jianyong Yu</name>
</country>
</tree>
</affiliations>
</record>
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