Thorn-like flexible Ag2C2O4/TiO2 nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.
Identifieur interne : 000206 ( Main/Corpus ); précédent : 000205; suivant : 000207Thorn-like flexible Ag2C2O4/TiO2 nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.
Auteurs : Xiaohui Wu ; Leitao Cao ; Jun Song ; Yang Si ; Jianyong Yu ; Bin DingSource :
- Journal of colloid and interface science [ 1095-7103 ] ; 2020.
English descriptors
- KwdEn :
- Adsorption (MeSH), Anti-Bacterial Agents (chemistry), Anti-Bacterial Agents (pharmacology), Catalysis (MeSH), Disinfection (MeSH), Escherichia coli (drug effects), Escherichia coli (growth & development), Light (MeSH), Metal Nanoparticles (chemistry), Nanofibers (chemistry), Photochemical Processes (MeSH), Silver Compounds (chemistry), Silver Compounds (pharmacology), Titanium (chemistry), Titanium (pharmacology).
- MESH :
- chemical , chemistry : Anti-Bacterial Agents, Silver Compounds, Titanium.
- chemical , pharmacology : Anti-Bacterial Agents, Silver Compounds, Titanium.
- chemistry : Metal Nanoparticles, Nanofibers.
- drug effects : Escherichia coli.
- growth & development : Escherichia coli.
- Adsorption, Catalysis, Disinfection, Light, Photochemical Processes.
Abstract
TiO2-based fibrous membranes as plasmonic heterojunction photocatalysts would hold great promise in the field of water disinfection, however, it still existed a great challenge to design and construct such materials. Here, we presented the fabrication of continuous, hierarchical, and easy-to-recycle flexible Ag2C2O4/TiO2 heterostructured nanofibrous membranes (NMs) that were composed of thorn-like nanofibers through electrospinning technique followed by successive ionic layer adsorption and reaction (SILAR) process. Ag2C2O4 nanoplates were firmly anchored on the surface of TiO2 and the obtained Ag2C2O4/TiO2 heterojunction photocatalysts underwent a silent-to-active transition of visible-light response under light irradiation due to the surface plasmon resonance (SPR) effect of Ag nanoparticles derived from Ag2C2O4, forming a new plasmonic heterojunction photocatalyst. By virtue of the hierarchical structure, enhanced visible light absorption and efficient charge carriers separation, Ag2C2O4/TiO2 NMs possessed high bactericidal efficiency of >99.999% within 30 min, strong reactive oxygen species (ROS) producing capability (1510 μg g-1 and 659 μg g-1 for superoxide radicals and hydroxyl radicals, respectively), and good reusability. This work may offer new insights into the design of antibacterial materials for pathogenic microorganism-contaminated water purification.
DOI: 10.1016/j.jcis.2019.10.119
PubMed: 31706650
Links to Exploration step
pubmed:31706650Le document en format XML
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C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.</title>
<author><name sortKey="Wu, Xiaohui" sort="Wu, Xiaohui" uniqKey="Wu X" first="Xiaohui" last="Wu">Xiaohui Wu</name>
<affiliation><nlm:affiliation>State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Textiles, Donghua University, Shanghai 201620, China.</nlm:affiliation>
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<author><name sortKey="Cao, Leitao" sort="Cao, Leitao" uniqKey="Cao L" first="Leitao" last="Cao">Leitao Cao</name>
<affiliation><nlm:affiliation>State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Textiles, Donghua University, Shanghai 201620, China.</nlm:affiliation>
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<author><name sortKey="Song, Jun" sort="Song, Jun" uniqKey="Song J" first="Jun" last="Song">Jun Song</name>
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<author><name sortKey="Yu, Jianyong" sort="Yu, Jianyong" uniqKey="Yu J" first="Jianyong" last="Yu">Jianyong Yu</name>
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<author><name sortKey="Ding, Bin" sort="Ding, Bin" uniqKey="Ding B" first="Bin" last="Ding">Bin Ding</name>
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<sourceDesc><biblStruct><analytic><title xml:lang="en">Thorn-like flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.</title>
<author><name sortKey="Wu, Xiaohui" sort="Wu, Xiaohui" uniqKey="Wu X" first="Xiaohui" last="Wu">Xiaohui Wu</name>
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<author><name sortKey="Song, Jun" sort="Song, Jun" uniqKey="Song J" first="Jun" last="Song">Jun Song</name>
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<author><name sortKey="Si, Yang" sort="Si, Yang" uniqKey="Si Y" first="Yang" last="Si">Yang Si</name>
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<author><name sortKey="Yu, Jianyong" sort="Yu, Jianyong" uniqKey="Yu J" first="Jianyong" last="Yu">Jianyong Yu</name>
<affiliation><nlm:affiliation>Innovation Center for Textile Science and Technology, Donghua University, Shanghai 200051, China.</nlm:affiliation>
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<author><name sortKey="Ding, Bin" sort="Ding, Bin" uniqKey="Ding B" first="Bin" last="Ding">Bin Ding</name>
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<term>Anti-Bacterial Agents (chemistry)</term>
<term>Anti-Bacterial Agents (pharmacology)</term>
<term>Catalysis (MeSH)</term>
<term>Disinfection (MeSH)</term>
<term>Escherichia coli (drug effects)</term>
<term>Escherichia coli (growth & development)</term>
<term>Light (MeSH)</term>
<term>Metal Nanoparticles (chemistry)</term>
<term>Nanofibers (chemistry)</term>
<term>Photochemical Processes (MeSH)</term>
<term>Silver Compounds (chemistry)</term>
<term>Silver Compounds (pharmacology)</term>
<term>Titanium (chemistry)</term>
<term>Titanium (pharmacology)</term>
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<term>Silver Compounds</term>
<term>Titanium</term>
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<keywords scheme="MESH" type="chemical" qualifier="pharmacology" xml:lang="en"><term>Anti-Bacterial Agents</term>
<term>Silver Compounds</term>
<term>Titanium</term>
</keywords>
<keywords scheme="MESH" qualifier="chemistry" xml:lang="en"><term>Metal Nanoparticles</term>
<term>Nanofibers</term>
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<keywords scheme="MESH" qualifier="drug effects" xml:lang="en"><term>Escherichia coli</term>
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<keywords scheme="MESH" xml:lang="en"><term>Adsorption</term>
<term>Catalysis</term>
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<front><div type="abstract" xml:lang="en">TiO<sub>2</sub>
-based fibrous membranes as plasmonic heterojunction photocatalysts would hold great promise in the field of water disinfection, however, it still existed a great challenge to design and construct such materials. Here, we presented the fabrication of continuous, hierarchical, and easy-to-recycle flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterostructured nanofibrous membranes (NMs) that were composed of thorn-like nanofibers through electrospinning technique followed by successive ionic layer adsorption and reaction (SILAR) process. Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
nanoplates were firmly anchored on the surface of TiO<sub>2</sub>
and the obtained Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterojunction photocatalysts underwent a silent-to-active transition of visible-light response under light irradiation due to the surface plasmon resonance (SPR) effect of Ag nanoparticles derived from Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
, forming a new plasmonic heterojunction photocatalyst. By virtue of the hierarchical structure, enhanced visible light absorption and efficient charge carriers separation, Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
NMs possessed high bactericidal efficiency of >99.999% within 30 min, strong reactive oxygen species (ROS) producing capability (1510 μg g<sup>-1</sup>
and 659 μg g<sup>-1</sup>
for superoxide radicals and hydroxyl radicals, respectively), and good reusability. This work may offer new insights into the design of antibacterial materials for pathogenic microorganism-contaminated water purification.</div>
</front>
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<ArticleTitle>Thorn-like flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
nanofibers as hierarchical heterojunction photocatalysts for efficient visible-light-driven bacteria-killing.</ArticleTitle>
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<Abstract><AbstractText>TiO<sub>2</sub>
-based fibrous membranes as plasmonic heterojunction photocatalysts would hold great promise in the field of water disinfection, however, it still existed a great challenge to design and construct such materials. Here, we presented the fabrication of continuous, hierarchical, and easy-to-recycle flexible Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterostructured nanofibrous membranes (NMs) that were composed of thorn-like nanofibers through electrospinning technique followed by successive ionic layer adsorption and reaction (SILAR) process. Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
nanoplates were firmly anchored on the surface of TiO<sub>2</sub>
and the obtained Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
heterojunction photocatalysts underwent a silent-to-active transition of visible-light response under light irradiation due to the surface plasmon resonance (SPR) effect of Ag nanoparticles derived from Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
, forming a new plasmonic heterojunction photocatalyst. By virtue of the hierarchical structure, enhanced visible light absorption and efficient charge carriers separation, Ag<sub>2</sub>
C<sub>2</sub>
O<sub>4</sub>
/TiO<sub>2</sub>
NMs possessed high bactericidal efficiency of >99.999% within 30 min, strong reactive oxygen species (ROS) producing capability (1510 μg g<sup>-1</sup>
and 659 μg g<sup>-1</sup>
for superoxide radicals and hydroxyl radicals, respectively), and good reusability. This work may offer new insights into the design of antibacterial materials for pathogenic microorganism-contaminated water purification.</AbstractText>
<CopyrightInformation>Copyright © 2019 Elsevier Inc. All rights reserved.</CopyrightInformation>
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<Keyword MajorTopicYN="N">Bacteria-killing</Keyword>
<Keyword MajorTopicYN="N">Heterostructured photocatalysts</Keyword>
<Keyword MajorTopicYN="N">Nanofirous membranes</Keyword>
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