Susceptibility and remanence studies in the quasi-1D mixed ferromagnet CoTAC : Mn
Identifieur interne : 000F17 ( Istex/Corpus ); précédent : 000F16; suivant : 000F18Susceptibility and remanence studies in the quasi-1D mixed ferromagnet CoTAC : Mn
Auteurs : A. Cheikhrouhou ; C. Dupas ; J. P. Renard ; P. VeilletSource :
- Journal of Magnetism and Magnetic Materials [ 0304-8853 ] ; 1985.
Abstract
The ac susceptibility and dc magnetization of CoTAC : Mn ((CH3)3NHCo1−xMnxCl3⋅2H2O) have been studied in the temperature range 1.3–4.2 K on two monocrystalline samples with x = 2.9 and 9.3%. In CoTAC : Mn (9.3%), the variation with the measuring frequency ν of the temperature of the susceptibility maximum Tg(ν) is well described over five decades of frequency by an Arrhenius law Tg-1(ν) = a − b log ν characteristic of superparamagnetic clusters. In CoTAC : Mn (2.9%) Tg(ν) does not differ significantly from that of pure CoTAC. Both compounds exhibit strong remanence effects below Tg. The variations with time, temperature and applied magnetic field of the IRM and TRM are similar to those observed in spin glasses. These experiments confirm the onset of spin-glass-like behaviour or superparamagnetism in quasi-1D insulators with random intrachain exchange at very low impurity concentration. Comparison with the previously studied mixed compound CHAC : Mn evidences the influence of the exchange anisotropy on the static properties of these systems.
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DOI: 10.1016/0304-8853(85)90122-2
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Renard</name><affiliation><mods:affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</mods:affiliation></affiliation></author><author><name sortKey="Veillet, P" sort="Veillet, P" uniqKey="Veillet P" first="P." last="Veillet">P. 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Veillet</name><affiliation><mods:affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</mods:affiliation></affiliation></author></analytic><monogr></monogr><series><title level="j">Journal of Magnetism and Magnetic Materials</title><title level="j" type="abbrev">MAGMA</title><idno type="ISSN">0304-8853</idno><imprint><publisher>ELSEVIER</publisher><date type="published" when="1985">1985</date><biblScope unit="volume">49</biblScope><biblScope unit="issue">1–2</biblScope><biblScope unit="page" from="201">201</biblScope><biblScope unit="page" to="209">209</biblScope></imprint><idno type="ISSN">0304-8853</idno></series><idno type="istex">3AD8F80B6ECAED1068581D37ECE43F0E13D56154</idno><idno type="DOI">10.1016/0304-8853(85)90122-2</idno><idno type="PII">0304-8853(85)90122-2</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">0304-8853</idno></seriesStmt></fileDesc><profileDesc><textClass></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The ac susceptibility and dc magnetization of CoTAC : Mn ((CH3)3NHCo1−xMnxCl3⋅2H2O) have been studied in the temperature range 1.3–4.2 K on two monocrystalline samples with x = 2.9 and 9.3%. In CoTAC : Mn (9.3%), the variation with the measuring frequency ν of the temperature of the susceptibility maximum Tg(ν) is well described over five decades of frequency by an Arrhenius law Tg-1(ν) = a − b log ν characteristic of superparamagnetic clusters. In CoTAC : Mn (2.9%) Tg(ν) does not differ significantly from that of pure CoTAC. Both compounds exhibit strong remanence effects below Tg. The variations with time, temperature and applied magnetic field of the IRM and TRM are similar to those observed in spin glasses. These experiments confirm the onset of spin-glass-like behaviour or superparamagnetism in quasi-1D insulators with random intrachain exchange at very low impurity concentration. Comparison with the previously studied mixed compound CHAC : Mn evidences the influence of the exchange anisotropy on the static properties of these systems.</div></front></TEI><istex><corpusName>elsevier</corpusName><author><json:item><name>A. Cheikhrouhou</name><affiliations><json:string>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</json:string></affiliations></json:item><json:item><name>C. Dupas</name><affiliations><json:string>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</json:string></affiliations></json:item><json:item><name>J.P. Renard</name><affiliations><json:string>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</json:string></affiliations></json:item><json:item><name>P. 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The variations with time, temperature and applied magnetic field of the IRM and TRM are similar to those observed in spin glasses. These experiments confirm the onset of spin-glass-like behaviour or superparamagnetism in quasi-1D insulators with random intrachain exchange at very low impurity concentration. 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W. Sfax, Tunisie.</note><affiliation>Permanent address: Ecole Nationale d'Ingénieurs, B.P. W. Sfax, Tunisie.</affiliation><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation></author><author xml:id="author-2"><persName><forename type="first">C.</forename><surname>Dupas</surname></persName><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation></author><author xml:id="author-3"><persName><forename type="first">J.P.</forename><surname>Renard</surname></persName><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation></author><author xml:id="author-4"><persName><forename type="first">P.</forename><surname>Veillet</surname></persName><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation></author></analytic><monogr><title level="j">Journal of Magnetism and Magnetic Materials</title><title level="j" type="abbrev">MAGMA</title><idno type="pISSN">0304-8853</idno><idno type="PII">S0304-8853(00)X0284-3</idno><imprint><publisher>ELSEVIER</publisher><date type="published" when="1985"></date><biblScope unit="volume">49</biblScope><biblScope unit="issue">1–2</biblScope><biblScope unit="page" from="201">201</biblScope><biblScope unit="page" to="209">209</biblScope></imprint></monogr><idno type="istex">3AD8F80B6ECAED1068581D37ECE43F0E13D56154</idno><idno type="DOI">10.1016/0304-8853(85)90122-2</idno><idno type="PII">0304-8853(85)90122-2</idno></biblStruct></sourceDesc></fileDesc><profileDesc><creation><date>1985</date></creation><langUsage><language ident="en">en</language></langUsage><abstract xml:lang="en"><p>The ac susceptibility and dc magnetization of CoTAC : Mn ((CH3)3NHCo1−xMnxCl3⋅2H2O) have been studied in the temperature range 1.3–4.2 K on two monocrystalline samples with x = 2.9 and 9.3%. In CoTAC : Mn (9.3%), the variation with the measuring frequency ν of the temperature of the susceptibility maximum Tg(ν) is well described over five decades of frequency by an Arrhenius law Tg-1(ν) = a − b log ν characteristic of superparamagnetic clusters. In CoTAC : Mn (2.9%) Tg(ν) does not differ significantly from that of pure CoTAC. Both compounds exhibit strong remanence effects below Tg. The variations with time, temperature and applied magnetic field of the IRM and TRM are similar to those observed in spin glasses. These experiments confirm the onset of spin-glass-like behaviour or superparamagnetism in quasi-1D insulators with random intrachain exchange at very low impurity concentration. Comparison with the previously studied mixed compound CHAC : Mn evidences the influence of the exchange anisotropy on the static properties of these systems.</p></abstract></profileDesc><revisionDesc><change when="1984-10-26">Modified</change><change when="1985">Published</change></revisionDesc></teiHeader></istex:fulltextTEI><json:item><original>false</original><mimetype>text/plain</mimetype><extension>txt</extension><uri>https://api.istex.fr/document/3AD8F80B6ECAED1068581D37ECE43F0E13D56154/fulltext/txt</uri></json:item></fulltext><metadata><istex:metadataXml wicri:clean="Elsevier, elements deleted: tail"><istex:xmlDeclaration>version="1.0" encoding="utf-8"</istex:xmlDeclaration><istex:docType PUBLIC="-//ES//DTD journal article DTD version 4.5.2//EN//XML" URI="art452.dtd" name="istex:docType"></istex:docType><istex:document><converted-article version="4.5.2" docsubtype="fla"><item-info><jid>MAGMA</jid><aid>85901222</aid><ce:pii>0304-8853(85)90122-2</ce:pii><ce:doi>10.1016/0304-8853(85)90122-2</ce:doi><ce:copyright type="unknown" year="1985"></ce:copyright></item-info><head><ce:title>Susceptibility and remanence studies in the quasi-1D mixed ferromagnet CoTAC : Mn</ce:title><ce:author-group><ce:author><ce:given-name>A.</ce:given-name><ce:surname>Cheikhrouhou</ce:surname><ce:cross-ref refid="FN1"><ce:sup>∗</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>C.</ce:given-name><ce:surname>Dupas</ce:surname></ce:author><ce:author><ce:given-name>J.P.</ce:given-name><ce:surname>Renard</ce:surname></ce:author><ce:author><ce:given-name>P.</ce:given-name><ce:surname>Veillet</ce:surname></ce:author><ce:affiliation><ce:textfn>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</ce:textfn></ce:affiliation><ce:footnote id="FN1"><ce:label>∗</ce:label><ce:note-para>Permanent address: Ecole Nationale d'Ingénieurs, B.P. W. Sfax, Tunisie.</ce:note-para></ce:footnote></ce:author-group><ce:date-received day="23" month="7" year="1984"></ce:date-received><ce:date-revised day="26" month="10" year="1984"></ce:date-revised><ce:abstract><ce:section-title>Abstract</ce:section-title><ce:abstract-sec><ce:simple-para>The ac susceptibility and dc magnetization of CoTAC : Mn ((CH<ce:inf>3</ce:inf>)<ce:inf>3</ce:inf>NHCo<ce:inf>1−<ce:italic>x</ce:italic></ce:inf>Mn<ce:inf><ce:italic>x</ce:italic></ce:inf>Cl<ce:inf>3</ce:inf>⋅2H<ce:inf>2</ce:inf>O) have been studied in the temperature range 1.3–4.2 K on two monocrystalline samples with <ce:italic>x</ce:italic> = 2.9 and 9.3%. In CoTAC : Mn (9.3%), the variation with the measuring frequency ν of the temperature of the susceptibility maximum <ce:italic>T</ce:italic><ce:inf>g</ce:inf>(ν) is well described over five decades of frequency by an Arrhenius law <ce:italic>T</ce:italic><ce:inf>g</ce:inf><ce:sup>-1</ce:sup>(ν) = <ce:italic>a − b</ce:italic> log ν characteristic of superparamagnetic clusters. In CoTAC : Mn (2.9%) <ce:italic>T</ce:italic><ce:inf>g</ce:inf>(ν) does not differ significantly from that of pure CoTAC. Both compounds exhibit strong remanence effects below <ce:italic>T</ce:italic><ce:inf>g</ce:inf>. The variations with time, temperature and applied magnetic field of the IRM and TRM are similar to those observed in spin glasses. These experiments confirm the onset of spin-glass-like behaviour or superparamagnetism in quasi-1D insulators with random intrachain exchange at very low impurity concentration. Comparison with the previously studied mixed compound CHAC : Mn evidences the influence of the exchange anisotropy on the static properties of these systems.</ce:simple-para></ce:abstract-sec></ce:abstract></head></converted-article></istex:document></istex:metadataXml><mods version="3.6"><titleInfo><title>Susceptibility and remanence studies in the quasi-1D mixed ferromagnet CoTAC : Mn</title></titleInfo><titleInfo type="alternative" contentType="CDATA"><title>Susceptibility and remanence studies in the quasi-1D mixed ferromagnet CoTAC : Mn</title></titleInfo><name type="personal"><namePart type="given">A.</namePart><namePart type="family">Cheikhrouhou</namePart><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation><description>Permanent address: Ecole Nationale d'Ingénieurs, B.P. W. Sfax, Tunisie.</description><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">C.</namePart><namePart type="family">Dupas</namePart><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">J.P.</namePart><namePart type="family">Renard</namePart><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">P.</namePart><namePart type="family">Veillet</namePart><affiliation>Institut d'Electronique Fondamentale, Laboratoire Associé au CNRS, Université Paris XI, Bât. 220, 91405 Orsay-Cedex, France</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="research-article" displayLabel="Full-length article"></genre><originInfo><publisher>ELSEVIER</publisher><dateIssued encoding="w3cdtf">1985</dateIssued><dateModified encoding="w3cdtf">1984-10-26</dateModified><copyrightDate encoding="w3cdtf">1985</copyrightDate></originInfo><language><languageTerm type="code" authority="iso639-2b">eng</languageTerm><languageTerm type="code" authority="rfc3066">en</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType></physicalDescription><abstract lang="en">The ac susceptibility and dc magnetization of CoTAC : Mn ((CH3)3NHCo1−xMnxCl3⋅2H2O) have been studied in the temperature range 1.3–4.2 K on two monocrystalline samples with x = 2.9 and 9.3%. In CoTAC : Mn (9.3%), the variation with the measuring frequency ν of the temperature of the susceptibility maximum Tg(ν) is well described over five decades of frequency by an Arrhenius law Tg-1(ν) = a − b log ν characteristic of superparamagnetic clusters. In CoTAC : Mn (2.9%) Tg(ν) does not differ significantly from that of pure CoTAC. Both compounds exhibit strong remanence effects below Tg. The variations with time, temperature and applied magnetic field of the IRM and TRM are similar to those observed in spin glasses. These experiments confirm the onset of spin-glass-like behaviour or superparamagnetism in quasi-1D insulators with random intrachain exchange at very low impurity concentration. Comparison with the previously studied mixed compound CHAC : Mn evidences the influence of the exchange anisotropy on the static properties of these systems.</abstract><relatedItem type="host"><titleInfo><title>Journal of Magnetism and Magnetic Materials</title></titleInfo><titleInfo type="abbreviated"><title>MAGMA</title></titleInfo><genre type="journal">journal</genre><originInfo><dateIssued encoding="w3cdtf">198503</dateIssued></originInfo><identifier type="ISSN">0304-8853</identifier><identifier type="PII">S0304-8853(00)X0284-3</identifier><part><date>198503</date><detail type="volume"><number>49</number><caption>vol.</caption></detail><detail type="issue"><number>1–2</number><caption>no.</caption></detail><extent unit="issue pages"><start>1</start><end>218</end></extent><extent unit="pages"><start>201</start><end>209</end></extent></part></relatedItem><identifier type="istex">3AD8F80B6ECAED1068581D37ECE43F0E13D56154</identifier><identifier type="DOI">10.1016/0304-8853(85)90122-2</identifier><identifier type="PII">0304-8853(85)90122-2</identifier><recordInfo><recordContentSource>ELSEVIER</recordContentSource></recordInfo></mods></metadata><serie></serie></istex></record>Pour manipuler ce document sous Unix (Dilib)
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