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CHAPTER 3 - Pd–Phosphine Precatalysts for Modern Cross-Coupling Reactions

Identifieur interne : 001759 ( Istex/Corpus ); précédent : 001758; suivant : 001760

CHAPTER 3 - Pd–Phosphine Precatalysts for Modern Cross-Coupling Reactions

Auteurs : Carin C. C. Johansson Seechurn ; Hongbo Li ; Thomas J. Colacot

Source :

RSC Catalysis Series [ 1757-6725 ]

RBID : ISTEX:3395C3848943C1A8AE38C3178AD2A758080CB12D

Abstract

The development and use of well-defined preformed Pd catalysts are reviewed from academic and industrial points of view. The strategies employed for the development of Pd precatalysts resulting in either L2Pd(0) or LPd(0) are discussed with examples from industry and academia on how the properties of the ligand and the nature of the precatalyst itself can precisely affect the efficiency of a number of cross-coupling reactions. The well-defined preformed Pd catalysts often improve the selectivity and activity of selected cross-coupling reactions by reducing the metal loading and the ligand-to-metal ratios. In addition, they are often more practical to handle than the corresponding in situ system containing a Pd precursor such as Pd(dba)x and a pyrophoric ligand such as t-Bu3P.

Url:

https://api.istex.fr/document/3395C3848943C1A8AE38C3178AD2A758080CB12D/fulltext/pdf

DOI: 10.1039/9781782620259-00091

Links to Exploration step

ISTEX:3395C3848943C1A8AE38C3178AD2A758080CB12D

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<abstract><p>The development and use of well-defined preformed Pd catalysts are reviewed from academic and industrial points of view. The strategies employed for the development of Pd precatalysts resulting in either L<sub>2</sub>
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<name type="personal"><namePart type="given">Carin C. C.</namePart>
<namePart type="family">Johansson Seechurn</namePart>
<affiliation>Johnson Matthey Catalysis and Chiral Technologies, Orchard Road, Royston, SG8 5HE, UK</affiliation>
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<name type="personal"><namePart type="given">Hongbo</namePart>
<namePart type="family">Li</namePart>
<affiliation>Johnson Matthey Catalysis and Chiral Technologies, 2001 Nolte Drive, West Deptford, NJ 08066, USA</affiliation>
<affiliation>E-mail: thomas.colacot@jmusa.com</affiliation>
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<name type="personal"><namePart type="given">Thomas J.</namePart>
<namePart type="family">Colacot</namePart>
<affiliation>Johnson Matthey Catalysis and Chiral Technologies, 2001 Nolte Drive, West Deptford, NJ 08066, USA</affiliation>
<affiliation>E-mail: thomas.colacot@jmusa.com</affiliation>
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<abstract>The development and use of well-defined preformed Pd catalysts are reviewed from academic and industrial points of view. The strategies employed for the development of Pd precatalysts resulting in either L2Pd(0) or LPd(0) are discussed with examples from industry and academia on how the properties of the ligand and the nature of the precatalyst itself can precisely affect the efficiency of a number of cross-coupling reactions. The well-defined preformed Pd catalysts often improve the selectivity and activity of selected cross-coupling reactions by reducing the metal loading and the ligand-to-metal ratios. In addition, they are often more practical to handle than the corresponding in situ system containing a Pd precursor such as Pd(dba)x and a pyrophoric ligand such as t-Bu3P.</abstract>
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<identifier type="ISSN">1757-6725</identifier>
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<part><date>2015</date>
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CHAPTER 3 - Pd–Phosphine Precatalysts for Modern Cross-Coupling Reactions

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