Photophysical properties of three hydrofullerenes
Identifieur interne : 000499 ( Istex/Corpus ); précédent : 000498; suivant : 000500Photophysical properties of three hydrofullerenes
Auteurs : R. V. Bensasson ; E. Bienvenue ; J.-M. Janot ; S. Leach ; P. Seta ; D. I. Schuster ; S. R. Wilson ; H. ZhaoSource :
- Chemical Physics Letters [ 0009-2614 ] ; 1995.
Abstract
The ground state and lowest triplet state properties of three hydrofullerenes, C60H2, C60H4 and [1-methylsuccinate-4-methyl-cyclohexadiene-2,3]buckminsterfullerene, have been investigated in toluene at room temperature. Their visible ground state absorption spectra are compared to those of methanofullerenes and methanolfulleroids. The triplet properties, including the absorption spectrum between 300 and 800 nm, molar absorption coefficient, quantum yield of formation and quantum yield for the photosensitized production of O2(1Δg), are compared to those of other C60 derivatives.
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DOI: 10.1016/0009-2614(95)01065-H
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<front><div type="abstract" xml:lang="en">The ground state and lowest triplet state properties of three hydrofullerenes, C60H2, C60H4 and [1-methylsuccinate-4-methyl-cyclohexadiene-2,3]buckminsterfullerene, have been investigated in toluene at room temperature. Their visible ground state absorption spectra are compared to those of methanofullerenes and methanolfulleroids. The triplet properties, including the absorption spectrum between 300 and 800 nm, molar absorption coefficient, quantum yield of formation and quantum yield for the photosensitized production of O2(1Δg), are compared to those of other C60 derivatives.</div>
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<head><ce:title>Photophysical properties of three hydrofullerenes</ce:title>
<ce:author-group><ce:author><ce:given-name>R.V.</ce:given-name>
<ce:surname>Bensasson</ce:surname>
<ce:cross-ref refid="AFF1"><ce:sup loc="post">a</ce:sup>
</ce:cross-ref>
</ce:author>
<ce:author><ce:given-name>E.</ce:given-name>
<ce:surname>Bienvenue</ce:surname>
<ce:cross-ref refid="AFF2"><ce:sup loc="post">b</ce:sup>
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<ce:author><ce:given-name>J.-M.</ce:given-name>
<ce:surname>Janot</ce:surname>
<ce:cross-ref refid="AFF2"><ce:sup loc="post">b</ce:sup>
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</ce:author>
<ce:author><ce:given-name>S.</ce:given-name>
<ce:surname>Leach</ce:surname>
<ce:cross-ref refid="AFF3"><ce:sup loc="post">c</ce:sup>
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<ce:cross-ref refid="AFF4"><ce:sup loc="post">d</ce:sup>
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</ce:author>
<ce:author><ce:given-name>P.</ce:given-name>
<ce:surname>Seta</ce:surname>
<ce:cross-ref refid="AFF2"><ce:sup loc="post">b</ce:sup>
</ce:cross-ref>
</ce:author>
<ce:author><ce:given-name>D.I.</ce:given-name>
<ce:surname>Schuster</ce:surname>
<ce:cross-ref refid="AFF5"><ce:sup loc="post">e</ce:sup>
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<ce:author><ce:given-name>S.R.</ce:given-name>
<ce:surname>Wilson</ce:surname>
<ce:cross-ref refid="AFF5"><ce:sup loc="post">e</ce:sup>
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</ce:author>
<ce:author><ce:given-name>H.</ce:given-name>
<ce:surname>Zhao</ce:surname>
<ce:cross-ref refid="AFF5"><ce:sup loc="post">e</ce:sup>
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<ce:affiliation id="AFF1"><ce:label>a</ce:label>
<ce:textfn>Laboratoire de Biophysique, Muséum National d'Histoire Naturelle, CNRS UA481, INSERM U201, 43 rue Cuvier, 75231 Paris Cedex 05, France</ce:textfn>
</ce:affiliation>
<ce:affiliation id="AFF2"><ce:label>b</ce:label>
<ce:textfn>Laboratoire des Matériaux et Procédés Membranaires, UMR 9987 du CNRS, 1919 Route de Mende, BP 5051, 34033 Montpellier Cedex 01, France</ce:textfn>
</ce:affiliation>
<ce:affiliation id="AFF3"><ce:label>c</ce:label>
<ce:textfn>Laboratoire de Photophysique Moléculaire du CNRS, Université de Paris-Sud, 91405 Orsay, France</ce:textfn>
</ce:affiliation>
<ce:affiliation id="AFF4"><ce:label>d</ce:label>
<ce:textfn>DAMAP, CNRS URA 812, Observatoire de Paris-Meudon, 92195 Meudon, France</ce:textfn>
</ce:affiliation>
<ce:affiliation id="AFF5"><ce:label>e</ce:label>
<ce:textfn>Department of Chemistry, New York University, Washington Square, New York, NY 10003, USA</ce:textfn>
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<ce:date-received day="3" month="7" year="1995"></ce:date-received>
<ce:date-accepted day="25" month="8" year="1995"></ce:date-accepted>
<ce:abstract class="author"><ce:section-title>Abstract</ce:section-title>
<ce:abstract-sec><ce:simple-para view="all" id="simple-para.0010">The ground state and lowest triplet state properties of three hydrofullerenes, C<ce:inf loc="post">60</ce:inf>
H<ce:inf loc="post">2</ce:inf>
, C<ce:inf loc="post">60</ce:inf>
H<ce:inf loc="post">4</ce:inf>
and [1-methylsuccinate-4-methyl-cyclohexadiene-2,3]buckminsterfullerene, have been investigated in toluene at room temperature. Their visible ground state absorption spectra are compared to those of methanofullerenes and methanolfulleroids. The triplet properties, including the absorption spectrum between 300 and 800 nm, molar absorption coefficient, quantum yield of formation and quantum yield for the photosensitized production of <math altimg="si1.gif"><rm>O</rm>
<inf loc="post">2</inf>
(<sup loc="pre">1</sup>
Δ<inf loc="post"><rm>g</rm>
</inf>
)</math>
, are compared to those of other C<ce:inf loc="post">60</ce:inf>
derivatives.</ce:simple-para>
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<affiliation>DAMAP, CNRS URA 812, Observatoire de Paris-Meudon, 92195 Meudon, France</affiliation>
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<abstract lang="en">The ground state and lowest triplet state properties of three hydrofullerenes, C60H2, C60H4 and [1-methylsuccinate-4-methyl-cyclohexadiene-2,3]buckminsterfullerene, have been investigated in toluene at room temperature. Their visible ground state absorption spectra are compared to those of methanofullerenes and methanolfulleroids. The triplet properties, including the absorption spectrum between 300 and 800 nm, molar absorption coefficient, quantum yield of formation and quantum yield for the photosensitized production of O2(1Δg), are compared to those of other C60 derivatives.</abstract>
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