MersV1, Istex, Corpus, bibRecord, 002446

Catalytic Isomerization of Biomass‐Derived Aldoses: A Review

Identifieur interne : 002446 ( Istex/Corpus ); précédent : 002445; suivant : 002447

Catalytic Isomerization of Biomass‐Derived Aldoses: A Review

Auteurs : Irina Delidovich ; Regina Palkovits

Source :

ChemSusChem [ 1864-5631 ] ; 2016-03-21.

RBID : ISTEX:77598358A20A9EEC34CBC16286DA46CEBADD975B

Abstract

Selected aldohexoses (d‐glucose, d‐mannose, and d‐galactose) and aldopentoses (d‐xylose, l‐arabinose, and d‐ribose) are readily available components of biopolymers. Isomerization reactions of these substances are very attractive as carbon‐efficient processes to broaden the portfolio of abundant monosaccharides. This review focuses on the chemocatalytic isomerization of aldoses into the corresponding ketoses as well as epimerization of aldoses at C2. Recent advances in the fields of catalysis by bases and Lewis acids are considered. The emphasis is laid on newly uncovered catalytic systems and mechanisms of carbohydrate transformations.

Sweet on you: Chemocatalytic isomerization of biobased aldoses gives rise to ketoses and C2 epimeric aldoses. Bases and Lewis acids exhibit high catalytic performance for the isomerization processes. Recently uncovered catalytic systems are reviewed, focusing on structure–performance relations, isomerization mechanisms, and catalyst stability under reaction conditions.

Url:

https://api.istex.fr/ark:/67375/WNG-DZ7TBTX8-M/fulltext.pdf

DOI: 10.1002/cssc.201501577

Links to Exploration step

ISTEX:77598358A20A9EEC34CBC16286DA46CEBADD975B

Le document en format XML

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<titleInfo type="alternative" contentType="CDATA" lang="en"><title>Catalytic Isomerization of Biomass‐Derived Aldoses: A Review</title>
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<name type="personal"><namePart type="termsOfAddress">Dr.</namePart>
<namePart type="given">Irina</namePart>
<namePart type="family">Delidovich</namePart>
<affiliation>Chair of Heterogeneous Catalysis and Chemical Technology, RWTH Aachen University, Worringerweg 2, 52074, Aachen, Germany</affiliation>
<role><roleTerm type="text">author</roleTerm>
</role>
</name>
<name type="personal"><namePart type="termsOfAddress">Prof. Dr.</namePart>
<namePart type="given">Regina</namePart>
<namePart type="family">Palkovits</namePart>
<affiliation>Chair of Heterogeneous Catalysis and Chemical Technology, RWTH Aachen University, Worringerweg 2, 52074, Aachen, Germany</affiliation>
<affiliation>E-mail: Palkovits@itmc.rwth-aachen.de</affiliation>
<role><roleTerm type="text">author</roleTerm>
</role>
</name>
<typeOfResource>text</typeOfResource>
<genre type="review-article" displayLabel="reviewArticle" authority="ISTEX" authorityURI="https://content-type.data.istex.fr" valueURI="https://content-type.data.istex.fr/ark:/67375/XTP-L5L7X3NF-P">review-article</genre>
<originInfo><publisher>Blackwell Publishing Ltd</publisher>
<dateIssued encoding="w3cdtf">2016-03-21</dateIssued>
<dateCaptured encoding="w3cdtf">2015-11-25</dateCaptured>
<edition>I. Delidovich, R. Palkovits, ChemSusChem 2016, 9, 547.</edition>
<copyrightDate encoding="w3cdtf">2016</copyrightDate>
</originInfo>
<language><languageTerm type="code" authority="rfc3066">en</languageTerm>
<languageTerm type="code" authority="iso639-2b">eng</languageTerm>
</language>
<physicalDescription><extent unit="figures">13</extent>
<extent unit="tables">4</extent>
<extent unit="references">177</extent>
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<abstract lang="en">Selected aldohexoses (d‐glucose, d‐mannose, and d‐galactose) and aldopentoses (d‐xylose, l‐arabinose, and d‐ribose) are readily available components of biopolymers. Isomerization reactions of these substances are very attractive as carbon‐efficient processes to broaden the portfolio of abundant monosaccharides. This review focuses on the chemocatalytic isomerization of aldoses into the corresponding ketoses as well as epimerization of aldoses at C2. Recent advances in the fields of catalysis by bases and Lewis acids are considered. The emphasis is laid on newly uncovered catalytic systems and mechanisms of carbohydrate transformations.</abstract>
<abstract type="graphical" lang="en">Sweet on you: Chemocatalytic isomerization of biobased aldoses gives rise to ketoses and C2 epimeric aldoses. Bases and Lewis acids exhibit high catalytic performance for the isomerization processes. Recently uncovered catalytic systems are reviewed, focusing on structure–performance relations, isomerization mechanisms, and catalyst stability under reaction conditions.</abstract>
<note type="funding">Alexander von Humboldt Foundation</note>
<note type="funding">Bayer Foundation</note>
<subject lang="en"><genre>keywords</genre>
<topic>biomass</topic>
<topic>chemocatalysis</topic>
<topic>isomerization</topic>
<topic>Lewis acids</topic>
<topic>saccharides</topic>
</subject>
<relatedItem type="host"><titleInfo><title>ChemSusChem</title>
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<titleInfo type="abbreviated"><title>ChemSusChem</title>
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<identifier type="ISSN">1864-5631</identifier>
<identifier type="eISSN">1864-564X</identifier>
<identifier type="DOI">10.1002/(ISSN)1864-564X</identifier>
<identifier type="PublisherID">CSSC</identifier>
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Catalytic Isomerization of Biomass‐Derived Aldoses: A Review

Catalytic Isomerization of Biomass‐Derived Aldoses: A Review

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