CHEMICAL CHARACTERIZATION OF NORTH SEA AEROSOL PARTICLES
Identifieur interne : 000C47 ( Main/Corpus ); précédent : 000C46; suivant : 000C48CHEMICAL CHARACTERIZATION OF NORTH SEA AEROSOL PARTICLES
Auteurs : M. Ebert ; S. Weinbruch ; P. Hoffmann ; H. M. OrtnerSource :
- Journal of Aerosol Science [ 0021-8502 ] ; 1999.
Abstract
Aerosol particles with diameters between 0.1 and 25μm were collected on the island of Helgoland (Germany) in October of 1996 (NORDEX 96 field campaign). The chemical bulk composition was determined for four different size fractions by total reflection X-ray fluorescence analysis. In addition, size, morphology, and chemical composition of approximately 3000 individual particles were determined by high-resolution scanning electron microscopy and electron probe microanalysis. Due to the use of a field emission source electron microscope the size range studied is extended down to 10nm. The high lateral resolution of this instrument facilitates the detection of biological particles and soot, two components of North Sea aerosols not recognized by previous workers. The chemical bulk composition and the relative abundance of different particle groups depend on the air mass trajectories. Variations of the chemical bulk composition between all samples can be explained by assuming the mixing, in different proportions, of a marine and a continental component. The marine component is characterized by a high abundance of sea-salt, aged sea-salt and a mixture of sea-salt and alumosilicates. Air masses that crossed the continent prior to sampling on Helgoland have higher abundances of alumosilicates, Si-rich particles, Fe-rich particles, calcium sulphates, soot and carbonaceous material. The anthropogenic fraction is about 8–33% (derived from the particle number concentrations) for marine air masses from the North Atlantic, and 14–69% for air masses that crossed the European continent.
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DOI: 10.1016/S0021-8502(99)00549-2
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Ebert</name><affiliation><mods:affiliation>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</mods:affiliation></affiliation></author><author><name sortKey="Weinbruch, S" sort="Weinbruch, S" uniqKey="Weinbruch S" first="S." last="Weinbruch">S. Weinbruch</name><affiliation><mods:affiliation>Institut für Mineralogie, Technische Universität Darmstadt, Schnittspahnstr. 9, D-64287 Darmstadt, Germany</mods:affiliation></affiliation></author><author><name sortKey="Hoffmann, P" sort="Hoffmann, P" uniqKey="Hoffmann P" first="P." last="Hoffmann">P. Hoffmann</name><affiliation><mods:affiliation>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</mods:affiliation></affiliation></author><author><name sortKey="Ortner, H M" sort="Ortner, H M" uniqKey="Ortner H" first="H. M." last="Ortner">H. M. Ortner</name><affiliation><mods:affiliation>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</mods:affiliation></affiliation></author></analytic><monogr></monogr><series><title level="j">Journal of Aerosol Science</title><title level="j" type="abbrev">AS</title><idno type="ISSN">0021-8502</idno><imprint><publisher>ELSEVIER</publisher><date type="published" when="1999">1999</date><biblScope unit="volume">31</biblScope><biblScope unit="issue">5</biblScope><biblScope unit="page" from="613">613</biblScope><biblScope unit="page" to="632">632</biblScope></imprint><idno type="ISSN">0021-8502</idno></series><idno type="istex">576151A090612E42F6367791642ED69F87FDBFE8</idno><idno type="DOI">10.1016/S0021-8502(99)00549-2</idno><idno type="PII">S0021-8502(99)00549-2</idno></biblStruct></sourceDesc><seriesStmt><idno type="ISSN">0021-8502</idno></seriesStmt></fileDesc><profileDesc><textClass></textClass><langUsage><language ident="en">en</language></langUsage></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Aerosol particles with diameters between 0.1 and 25μm were collected on the island of Helgoland (Germany) in October of 1996 (NORDEX 96 field campaign). The chemical bulk composition was determined for four different size fractions by total reflection X-ray fluorescence analysis. In addition, size, morphology, and chemical composition of approximately 3000 individual particles were determined by high-resolution scanning electron microscopy and electron probe microanalysis. Due to the use of a field emission source electron microscope the size range studied is extended down to 10nm. The high lateral resolution of this instrument facilitates the detection of biological particles and soot, two components of North Sea aerosols not recognized by previous workers. The chemical bulk composition and the relative abundance of different particle groups depend on the air mass trajectories. Variations of the chemical bulk composition between all samples can be explained by assuming the mixing, in different proportions, of a marine and a continental component. The marine component is characterized by a high abundance of sea-salt, aged sea-salt and a mixture of sea-salt and alumosilicates. Air masses that crossed the continent prior to sampling on Helgoland have higher abundances of alumosilicates, Si-rich particles, Fe-rich particles, calcium sulphates, soot and carbonaceous material. The anthropogenic fraction is about 8–33% (derived from the particle number concentrations) for marine air masses from the North Atlantic, and 14–69% for air masses that crossed the European continent.</div></front></TEI><istex><corpusName>elsevier</corpusName><author><json:item><name>M. Ebert</name><affiliations><json:string>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</json:string></affiliations></json:item><json:item><name>S. Weinbruch</name><affiliations><json:string>Institut für Mineralogie, Technische Universität Darmstadt, Schnittspahnstr. 9, D-64287 Darmstadt, Germany</json:string></affiliations></json:item><json:item><name>P. Hoffmann</name><affiliations><json:string>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</json:string></affiliations></json:item><json:item><name>H.M. Ortner</name><affiliations><json:string>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</json:string></affiliations></json:item></author><language><json:string>eng</json:string></language><abstract>Aerosol particles with diameters between 0.1 and 25μm were collected on the island of Helgoland (Germany) in October of 1996 (NORDEX 96 field campaign). The chemical bulk composition was determined for four different size fractions by total reflection X-ray fluorescence analysis. In addition, size, morphology, and chemical composition of approximately 3000 individual particles were determined by high-resolution scanning electron microscopy and electron probe microanalysis. Due to the use of a field emission source electron microscope the size range studied is extended down to 10nm. The high lateral resolution of this instrument facilitates the detection of biological particles and soot, two components of North Sea aerosols not recognized by previous workers. The chemical bulk composition and the relative abundance of different particle groups depend on the air mass trajectories. Variations of the chemical bulk composition between all samples can be explained by assuming the mixing, in different proportions, of a marine and a continental component. The marine component is characterized by a high abundance of sea-salt, aged sea-salt and a mixture of sea-salt and alumosilicates. Air masses that crossed the continent prior to sampling on Helgoland have higher abundances of alumosilicates, Si-rich particles, Fe-rich particles, calcium sulphates, soot and carbonaceous material. 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The chemical bulk composition was determined for four different size fractions by total reflection X-ray fluorescence analysis. In addition, size, morphology, and chemical composition of approximately 3000 individual particles were determined by high-resolution scanning electron microscopy and electron probe microanalysis. Due to the use of a field emission source electron microscope the size range studied is extended down to 10nm. The high lateral resolution of this instrument facilitates the detection of biological particles and soot, two components of North Sea aerosols not recognized by previous workers. The chemical bulk composition and the relative abundance of different particle groups depend on the air mass trajectories. Variations of the chemical bulk composition between all samples can be explained by assuming the mixing, in different proportions, of a marine and a continental component. The marine component is characterized by a high abundance of sea-salt, aged sea-salt and a mixture of sea-salt and alumosilicates. Air masses that crossed the continent prior to sampling on Helgoland have higher abundances of alumosilicates, Si-rich particles, Fe-rich particles, calcium sulphates, soot and carbonaceous material. The anthropogenic fraction is about 8–33% (derived from the particle number concentrations) for marine air masses from the North Atlantic, and 14–69% for air masses that crossed the European continent.</p></abstract></profileDesc><revisionDesc><change when="1999-08-27">Registration</change><change when="1999">Published</change><change xml:id="refBibs-istex" who="#ISTEX-API" when="2016-3-5">References added</change></revisionDesc></teiHeader></istex:fulltextTEI><json:item><original>false</original><mimetype>text/plain</mimetype><extension>txt</extension><uri>https://api.istex.fr/document/576151A090612E42F6367791642ED69F87FDBFE8/fulltext/txt</uri></json:item></fulltext><metadata><istex:metadataXml wicri:clean="Elsevier converted-article found"><istex:xmlDeclaration>version="1.0" encoding="utf-8"</istex:xmlDeclaration><istex:docType PUBLIC="-//ES//DTD journal article DTD version 4.5.2//EN//XML" URI="art452.dtd" name="istex:docType"></istex:docType><istex:document><converted-article version="4.5.2" docsubtype="fla"><item-info><jid>AS</jid><aid>3073</aid><ce:pii>S0021-8502(99)00549-2</ce:pii><ce:doi>10.1016/S0021-8502(99)00549-2</ce:doi><ce:copyright type="full-transfer" year="2000">Elsevier Science Ltd</ce:copyright></item-info><head><ce:title>CHEMICAL CHARACTERIZATION OF NORTH SEA AEROSOL PARTICLES</ce:title><ce:author-group><ce:author><ce:given-name>M.</ce:given-name><ce:surname>Ebert</ce:surname><ce:cross-ref refid="ORFA"><ce:sup>a</ce:sup></ce:cross-ref><ce:cross-ref refid="COR1">*</ce:cross-ref></ce:author><ce:author><ce:given-name>S.</ce:given-name><ce:surname>Weinbruch</ce:surname><ce:cross-ref refid="ORFB"><ce:sup>b</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>P.</ce:given-name><ce:surname>Hoffmann</ce:surname><ce:cross-ref refid="ORFA"><ce:sup>a</ce:sup></ce:cross-ref></ce:author><ce:author><ce:given-name>H.M.</ce:given-name><ce:surname>Ortner</ce:surname><ce:cross-ref refid="ORFA"><ce:sup>a</ce:sup></ce:cross-ref></ce:author><ce:affiliation id="ORFA"><ce:label>a</ce:label><ce:textfn>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</ce:textfn></ce:affiliation><ce:affiliation id="ORFB"><ce:label>b</ce:label><ce:textfn>Institut für Mineralogie, Technische Universität Darmstadt, Schnittspahnstr. 9, D-64287 Darmstadt, Germany</ce:textfn></ce:affiliation><ce:correspondence id="COR1"><ce:label>*</ce:label><ce:text>Author to whom correspondence should be addressed.</ce:text></ce:correspondence></ce:author-group><ce:date-received day="19" month="4" year="1999"></ce:date-received><ce:date-accepted day="27" month="8" year="1999"></ce:date-accepted><ce:abstract><ce:section-title>Abstract</ce:section-title><ce:abstract-sec><ce:simple-para>Aerosol particles with diameters between 0.1 and 25<ce:hsp sp="0.25"></ce:hsp><ce:italic>μ</ce:italic>m were collected on the island of Helgoland (Germany) in October of 1996 (NORDEX 96 field campaign). The chemical bulk composition was determined for four different size fractions by total reflection X-ray fluorescence analysis. In addition, size, morphology, and chemical composition of approximately 3000 individual particles were determined by high-resolution scanning electron microscopy and electron probe microanalysis. Due to the use of a field emission source electron microscope the size range studied is extended down to 10<ce:hsp sp="0.25"></ce:hsp>nm. The high lateral resolution of this instrument facilitates the detection of biological particles and soot, two components of North Sea aerosols not recognized by previous workers. The chemical bulk composition and the relative abundance of different particle groups depend on the air mass trajectories. Variations of the chemical bulk composition between all samples can be explained by assuming the mixing, in different proportions, of a marine and a continental component. The marine component is characterized by a high abundance of sea-salt, aged sea-salt and a mixture of sea-salt and alumosilicates. Air masses that crossed the continent prior to sampling on Helgoland have higher abundances of alumosilicates, Si-rich particles, Fe-rich particles, calcium sulphates, soot and carbonaceous material. The anthropogenic fraction is about 8–33% (derived from the particle number concentrations) for marine air masses from the North Atlantic, and 14–69% for air masses that crossed the European continent.</ce:simple-para></ce:abstract-sec></ce:abstract></head></converted-article></istex:document></istex:metadataXml><mods version="3.6"><titleInfo><title>CHEMICAL CHARACTERIZATION OF NORTH SEA AEROSOL PARTICLES</title></titleInfo><titleInfo type="alternative" contentType="CDATA"><title>CHEMICAL CHARACTERIZATION OF NORTH SEA AEROSOL PARTICLES</title></titleInfo><name type="personal"><namePart type="given">M.</namePart><namePart type="family">Ebert</namePart><affiliation>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</affiliation><description>Author to whom correspondence should be addressed.</description><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">S.</namePart><namePart type="family">Weinbruch</namePart><affiliation>Institut für Mineralogie, Technische Universität Darmstadt, Schnittspahnstr. 9, D-64287 Darmstadt, Germany</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">P.</namePart><namePart type="family">Hoffmann</namePart><affiliation>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</affiliation><role><roleTerm type="text">author</roleTerm></role></name><name type="personal"><namePart type="given">H.M.</namePart><namePart type="family">Ortner</namePart><affiliation>Technische Universität Darmstadt, Fachbereich Materialwissenschaft, Fachgebiet Chemische Analytik, Petersenstr. 23, D-64287 Darmstadt, Germany</affiliation><role><roleTerm type="text">author</roleTerm></role></name><typeOfResource>text</typeOfResource><genre type="research-article" displayLabel="Full-length article"></genre><originInfo><publisher>ELSEVIER</publisher><dateIssued encoding="w3cdtf">1999</dateIssued><dateValid encoding="w3cdtf">1999-08-27</dateValid><copyrightDate encoding="w3cdtf">2000</copyrightDate></originInfo><language><languageTerm type="code" authority="iso639-2b">eng</languageTerm><languageTerm type="code" authority="rfc3066">en</languageTerm></language><physicalDescription><internetMediaType>text/html</internetMediaType></physicalDescription><abstract lang="en">Aerosol particles with diameters between 0.1 and 25μm were collected on the island of Helgoland (Germany) in October of 1996 (NORDEX 96 field campaign). The chemical bulk composition was determined for four different size fractions by total reflection X-ray fluorescence analysis. In addition, size, morphology, and chemical composition of approximately 3000 individual particles were determined by high-resolution scanning electron microscopy and electron probe microanalysis. Due to the use of a field emission source electron microscope the size range studied is extended down to 10nm. The high lateral resolution of this instrument facilitates the detection of biological particles and soot, two components of North Sea aerosols not recognized by previous workers. The chemical bulk composition and the relative abundance of different particle groups depend on the air mass trajectories. Variations of the chemical bulk composition between all samples can be explained by assuming the mixing, in different proportions, of a marine and a continental component. The marine component is characterized by a high abundance of sea-salt, aged sea-salt and a mixture of sea-salt and alumosilicates. Air masses that crossed the continent prior to sampling on Helgoland have higher abundances of alumosilicates, Si-rich particles, Fe-rich particles, calcium sulphates, soot and carbonaceous material. The anthropogenic fraction is about 8–33% (derived from the particle number concentrations) for marine air masses from the North Atlantic, and 14–69% for air masses that crossed the European continent.</abstract><relatedItem type="host"><titleInfo><title>Journal of Aerosol Science</title></titleInfo><titleInfo type="abbreviated"><title>AS</title></titleInfo><genre type="Journal">journal</genre><originInfo><dateIssued encoding="w3cdtf">200005</dateIssued></originInfo><identifier type="ISSN">0021-8502</identifier><identifier type="PII">S0021-8502(00)X0044-4</identifier><part><date>200005</date><detail type="volume"><number>31</number><caption>vol.</caption></detail><detail type="issue"><number>5</number><caption>no.</caption></detail><extent unit="issue pages"><start>509</start><end>632</end></extent><extent unit="pages"><start>613</start><end>632</end></extent></part></relatedItem><identifier type="istex">576151A090612E42F6367791642ED69F87FDBFE8</identifier><identifier type="DOI">10.1016/S0021-8502(99)00549-2</identifier><identifier type="PII">S0021-8502(99)00549-2</identifier><accessCondition type="use and reproduction" contentType="">© 2000Elsevier Science Ltd</accessCondition><recordInfo><recordContentSource>ELSEVIER</recordContentSource><recordOrigin>Elsevier Science Ltd, ©2000</recordOrigin></recordInfo></mods></metadata><enrichments><istex:catWosTEI uri="https://api.istex.fr/document/576151A090612E42F6367791642ED69F87FDBFE8/enrichments/catWos"><teiHeader><profileDesc><textClass><classCode scheme="WOS">ENGINEERING, CHEMICAL</classCode><classCode scheme="WOS">ENGINEERING, MECHANICAL</classCode><classCode scheme="WOS">ENVIRONMENTAL SCIENCES</classCode><classCode scheme="WOS">METEOROLOGY & ATMOSPHERIC SCIENCES</classCode></textClass></profileDesc></teiHeader></istex:catWosTEI><istex:refBibTEI uri="https://api.istex.fr/document/576151A090612E42F6367791642ED69F87FDBFE8/enrichments/refBib"><teiHeader></teiHeader><text><front></front><body></body><back><listBibl><biblStruct><analytic><title level="a" type="main">UniversitaK t Frankfurt) for wind data, and the Deutscher Wetterdienst (O!enbach) for calculation of air mass back-trajectories. 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