An experimental and kinetic investigation of premixed furan/oxygen/argon flames
Identifieur interne : 000C57 ( Main/Merge ); précédent : 000C56; suivant : 000C58An experimental and kinetic investigation of premixed furan/oxygen/argon flames
Auteurs : Zhenyu Tian [France, République populaire de Chine] ; Tao Yuan [République populaire de Chine] ; Rene Fournet [France] ; Pierre-Alexandre Glaude [France] ; Baptiste Sirjean [France] ; Frédérique Battin-Leclerc [France] ; Kuiwen Zhang [République populaire de Chine] ; Fei Qi [République populaire de Chine]Source :
- Combustion and flame [ 0010-2180 ] ; 2011.
English descriptors
Abstract
The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt-6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.
Url:
- http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3695461
- https://hal.archives-ouvertes.fr/hal-00576339
- https://hal.archives-ouvertes.fr/hal-00602362
DOI: 10.1016/j.combustflame.2010.12.022
PubMed: 23814311
PubMed Central: 3695461
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PMC:3695461Le document en format XML
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R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Yuan, Tao" sort="Yuan, Tao" uniqKey="Yuan T" first="Tao" last="Yuan">Tao Yuan</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Fournet, Rene" sort="Fournet, Rene" uniqKey="Fournet R" first="Rene" last="Fournet">Rene Fournet</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Sirjean, Baptiste" sort="Sirjean, Baptiste" uniqKey="Sirjean B" first="Baptiste" last="Sirjean">Baptiste Sirjean</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName><placeName><settlement type="city">Nancy</settlement><region type="region" nuts="2">Grand Est</region><region type="region" nuts="2">Lorraine (région)</region></placeName><orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName><orgName type="university">Université de Lorraine</orgName><orgName type="institution">Centre national de la recherche scientifique</orgName></affiliation></author><author><name sortKey="Zhang, Kuiwen" sort="Zhang, Kuiwen" uniqKey="Zhang K" first="Kuiwen" last="Zhang">Kuiwen Zhang</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Qi, Fei" sort="Qi, Fei" uniqKey="Qi F" first="Fei" last="Qi">Fei Qi</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author></analytic><series><title level="j">Combustion and flame</title><idno type="ISSN">0010-2180</idno><idno type="eISSN">1556-2921</idno><imprint><date when="2011">2011</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="mix" xml:lang="en"><term>Premixed laminar flame Kinetic modeling Furan Tunable synchrotron VUV photoionization Molecular-beam mass spectrometry</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p id="P2">The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt-6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.</p></div></front></TEI><double doi="10.1016/j.combustflame.2010.12.022"><HAL><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">An experimental and kinetic investigation of premixed furan/oxygen/argon flames</title><author><name sortKey="Tian, Z" sort="Tian, Z" uniqKey="Tian Z" first="Z." last="Tian">Z. 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Sirjean</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName></affiliation></author><author><name sortKey="Battin Leclerc, F" sort="Battin Leclerc, F" uniqKey="Battin Leclerc F" first="F." last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName><placeName><settlement type="city">Nancy</settlement><region type="region" nuts="2">Grand Est</region><region type="region" nuts="2">Lorraine (région)</region></placeName><orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName><orgName type="university">Université de Lorraine</orgName><orgName type="institution">Centre national de la recherche scientifique</orgName></affiliation></author><author><name sortKey="Zhang, K" sort="Zhang, K" uniqKey="Zhang K" first="K." last="Zhang">K. Zhang</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-139461" status="INCOMING"><orgName>National Synchrotron Radiation Laboratory</orgName><desc><address><addrLine>Hefei, Anhui 230029, PR China</addrLine><country key="CN"></country></address></desc><listRelation><relation active="#struct-364765" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-364765" type="direct"><org type="institution" xml:id="struct-364765" status="INCOMING"><orgName>UNIVERSITY OF SCIENCE AND TECHNOLOGY OF CHINA</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle></tutelles></hal:affiliation><country>République populaire de Chine</country></affiliation></author><author><name sortKey="Qi, F" sort="Qi, F" uniqKey="Qi F" first="F." last="Qi">F. Qi</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-139461" status="INCOMING"><orgName>National Synchrotron Radiation Laboratory</orgName><desc><address><addrLine>Hefei, Anhui 230029, PR China</addrLine><country key="CN"></country></address></desc><listRelation><relation active="#struct-364765" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-364765" type="direct"><org type="institution" xml:id="struct-364765" status="INCOMING"><orgName>UNIVERSITY OF SCIENCE AND TECHNOLOGY OF CHINA</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle></tutelles></hal:affiliation><country>République populaire de Chine</country></affiliation></author></analytic><idno type="DOI">10.1016/j.combustflame.2010.12.022</idno><series><title level="j">Combustion and Flame</title><idno type="ISSN">0010-2180</idno><imprint><date type="datePub">2011</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="mix" xml:lang="en"><term>Premixed laminar flame Kinetic modeling Furan Tunable synchrotron VUV photoionization Molecular-beam mass spectrometry</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt- 6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.</div></front></TEI></HAL><HAL><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">An experimental and kinetic investigation of premixed furan/oxygen/argon flames</title><author><name sortKey="Tian, Z" sort="Tian, Z" uniqKey="Tian Z" first="Z." last="Tian">Z. Tian</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName></affiliation></author><author><name sortKey="Yuan, T" sort="Yuan, T" uniqKey="Yuan T" first="T." last="Yuan">T. 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Fournet</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName></affiliation></author><author><name sortKey="Glaude, P A" sort="Glaude, P A" uniqKey="Glaude P" first="P. A." last="Glaude">P. A. 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Sirjean</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName></affiliation></author><author><name sortKey="Battin Leclerc, F" sort="Battin Leclerc, F" uniqKey="Battin Leclerc F" first="F." last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName><placeName><settlement type="city">Nancy</settlement><region type="region" nuts="2">Grand Est</region><region type="region" nuts="2">Lorraine (région)</region></placeName><orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName><orgName type="university">Université de Lorraine</orgName><orgName type="institution">Centre national de la recherche scientifique</orgName></affiliation></author><author><name sortKey="Zhang, K" sort="Zhang, K" uniqKey="Zhang K" first="K." last="Zhang">K. Zhang</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-139461" status="INCOMING"><orgName>National Synchrotron Radiation Laboratory</orgName><desc><address><addrLine>Hefei, Anhui 230029, PR China</addrLine><country key="CN"></country></address></desc><listRelation><relation active="#struct-364765" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-364765" type="direct"><org type="institution" xml:id="struct-364765" status="INCOMING"><orgName>UNIVERSITY OF SCIENCE AND TECHNOLOGY OF CHINA</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle></tutelles></hal:affiliation><country>République populaire de Chine</country></affiliation></author><author><name sortKey="Qi, F" sort="Qi, F" uniqKey="Qi F" first="F." last="Qi">F. Qi</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-139461" status="INCOMING"><orgName>National Synchrotron Radiation Laboratory</orgName><desc><address><addrLine>Hefei, Anhui 230029, PR China</addrLine><country key="CN"></country></address></desc><listRelation><relation active="#struct-364765" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-364765" type="direct"><org type="institution" xml:id="struct-364765" status="INCOMING"><orgName>UNIVERSITY OF SCIENCE AND TECHNOLOGY OF CHINA</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle></tutelles></hal:affiliation><country>République populaire de Chine</country></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">HAL</idno><idno type="RBID">Hal:hal-00602362</idno><idno type="halId">hal-00602362</idno><idno type="halUri">https://hal.archives-ouvertes.fr/hal-00602362</idno><idno type="url">https://hal.archives-ouvertes.fr/hal-00602362</idno><idno type="doi">10.1016/j.combustflame.2010.12.022</idno><date when="2011">2011</date><idno type="wicri:Area/Hal/Corpus">000092</idno><idno type="wicri:Area/Hal/Curation">000092</idno><idno type="wicri:Area/Hal/Checkpoint">000A42</idno><idno type="wicri:explorRef" wicri:stream="Hal" wicri:step="Checkpoint">000A42</idno><idno type="wicri:doubleKey">0010-2180:2011:Tian Z:an:experimental:and</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">An experimental and kinetic investigation of premixed furan/oxygen/argon flames</title><author><name sortKey="Tian, Z" sort="Tian, Z" uniqKey="Tian Z" first="Z." last="Tian">Z. 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Fournet</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName></affiliation></author><author><name sortKey="Glaude, P A" sort="Glaude, P A" uniqKey="Glaude P" first="P. A." last="Glaude">P. A. Glaude</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-211875" status="VALID"><idno type="IdRef">153068876</idno><idno type="RNSR">201320573K</idno><idno type="IdUnivLorraine">[UL]RQC--</idno><orgName>Laboratoire Réactions et Génie des Procédés</orgName><orgName type="acronym">LRGP</orgName><date type="start">2013-01-01</date><desc><address><addrLine>Université de Lorraine - ENSIC, 1 rue de Grandville BP 20451, 54001 Nancy Cedex</addrLine><country key="FR"></country></address><ref type="url">http://lrgp.univ-lorraine.fr/</ref></desc><listRelation><relation active="#struct-413289" type="direct"></relation><relation name="UMR7274" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-413289" type="direct"><org type="institution" xml:id="struct-413289" status="VALID"><idno type="IdRef">157040569</idno><idno type="IdUnivLorraine">[UL]100--</idno><orgName>Université de Lorraine</orgName><orgName type="acronym">UL</orgName><date type="start">2012-01-01</date><desc><address><addrLine>34 cours Léopold - CS 25233 - 54052 Nancy cedex</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-lorraine.fr/</ref></desc></org></tutelle><tutelle name="UMR7274" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"><idno type="ISNI">0000000122597504</idno><idno type="IdRef">02636817X</idno><orgName>Centre National de la Recherche Scientifique</orgName><orgName type="acronym">CNRS</orgName><date type="start">1939-10-19</date><desc><address><country key="FR"></country></address><ref type="url">http://www.cnrs.fr/</ref></desc></org></tutelle></tutelles></hal:affiliation><country>France</country><placeName><settlement type="city">Nancy</settlement><settlement type="city">Metz</settlement><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region></placeName><orgName type="university">Université de Lorraine</orgName></affiliation></author><author><name sortKey="Sirjean, B" sort="Sirjean, B" uniqKey="Sirjean B" first="B." last="Sirjean">B. 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Zhang</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-139461" status="INCOMING"><orgName>National Synchrotron Radiation Laboratory</orgName><desc><address><addrLine>Hefei, Anhui 230029, PR China</addrLine><country key="CN"></country></address></desc><listRelation><relation active="#struct-364765" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-364765" type="direct"><org type="institution" xml:id="struct-364765" status="INCOMING"><orgName>UNIVERSITY OF SCIENCE AND TECHNOLOGY OF CHINA</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle></tutelles></hal:affiliation><country>République populaire de Chine</country></affiliation></author><author><name sortKey="Qi, F" sort="Qi, F" uniqKey="Qi F" first="F." last="Qi">F. Qi</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-139461" status="INCOMING"><orgName>National Synchrotron Radiation Laboratory</orgName><desc><address><addrLine>Hefei, Anhui 230029, PR China</addrLine><country key="CN"></country></address></desc><listRelation><relation active="#struct-364765" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-364765" type="direct"><org type="institution" xml:id="struct-364765" status="INCOMING"><orgName>UNIVERSITY OF SCIENCE AND TECHNOLOGY OF CHINA</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle></tutelles></hal:affiliation><country>République populaire de Chine</country></affiliation></author></analytic><idno type="DOI">10.1016/j.combustflame.2010.12.022</idno><series><title level="j">Combustion and Flame</title><idno type="ISSN">0010-2180</idno><imprint><date type="datePub">2011</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="mix" xml:lang="en"><term>Premixed laminar flame Kinetic modeling Furan Tunable synchrotron VUV photoionization Molecular-beam mass spectrometry</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt- 6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.</div></front></TEI></HAL><PMC><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">An experimental and kinetic investigation of premixed furan/oxygen/argon flames</title><author><name sortKey="Tian, Zhenyu" sort="Tian, Zhenyu" uniqKey="Tian Z" first="Zhenyu" last="Tian">Zhenyu Tian</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Yuan, Tao" sort="Yuan, Tao" uniqKey="Yuan T" first="Tao" last="Yuan">Tao Yuan</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Fournet, Rene" sort="Fournet, Rene" uniqKey="Fournet R" first="Rene" last="Fournet">Rene Fournet</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Sirjean, Baptiste" sort="Sirjean, Baptiste" uniqKey="Sirjean B" first="Baptiste" last="Sirjean">Baptiste Sirjean</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName><placeName><settlement type="city">Nancy</settlement><region type="region" nuts="2">Grand Est</region><region type="region" nuts="2">Lorraine (région)</region></placeName><orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName><orgName type="university">Université de Lorraine</orgName><orgName type="institution">Centre national de la recherche scientifique</orgName></affiliation></author><author><name sortKey="Zhang, Kuiwen" sort="Zhang, Kuiwen" uniqKey="Zhang K" first="Kuiwen" last="Zhang">Kuiwen Zhang</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Qi, Fei" sort="Qi, Fei" uniqKey="Qi F" first="Fei" last="Qi">Fei Qi</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PMC</idno><idno type="pmid">23814311</idno><idno type="pmc">3695461</idno><idno type="url">http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3695461</idno><idno type="RBID">PMC:3695461</idno><idno type="doi">10.1016/j.combustflame.2010.12.022</idno><date when="2011">2011</date><idno type="wicri:Area/Pmc/Corpus">000169</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Corpus" wicri:corpus="PMC">000169</idno><idno type="wicri:Area/Pmc/Curation">000169</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Curation">000169</idno><idno type="wicri:Area/Pmc/Checkpoint">000078</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Checkpoint">000078</idno><idno type="wicri:source">PubMed</idno><idno type="wicri:Area/PubMed/Corpus">000090</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Corpus" wicri:corpus="PubMed">000090</idno><idno type="wicri:Area/PubMed/Curation">000090</idno><idno type="wicri:explorRef" wicri:stream="PubMed" wicri:step="Curation">000090</idno><idno type="wicri:Area/PubMed/Checkpoint">000090</idno><idno type="wicri:explorRef" wicri:stream="Checkpoint" wicri:step="PubMed">000090</idno><idno type="wicri:Area/Ncbi/Merge">000275</idno><idno type="wicri:Area/Ncbi/Curation">000275</idno><idno type="wicri:Area/Ncbi/Checkpoint">000275</idno><idno type="wicri:doubleKey">0010-2180:2011:Tian Z:an:experimental:and</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a" type="main">An experimental and kinetic investigation of premixed furan/oxygen/argon flames</title><author><name sortKey="Tian, Zhenyu" sort="Tian, Zhenyu" uniqKey="Tian Z" first="Zhenyu" last="Tian">Zhenyu Tian</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Yuan, Tao" sort="Yuan, Tao" uniqKey="Yuan T" first="Tao" last="Yuan">Tao Yuan</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Fournet, Rene" sort="Fournet, Rene" uniqKey="Fournet R" first="Rene" last="Fournet">Rene Fournet</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Sirjean, Baptiste" sort="Sirjean, Baptiste" uniqKey="Sirjean B" first="Baptiste" last="Sirjean">Baptiste Sirjean</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName></affiliation></author><author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation wicri:level="4"><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex, France</nlm:aff><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés, CNRS, Nancy Université, ENSIC, 1, rue Grandville, BP 451, 54001 Nancy Cedex</wicri:regionArea><placeName><region type="region" nuts="2">Grand Est</region><region type="old region" nuts="2">Lorraine (région)</region><settlement type="city">Nancy</settlement></placeName><orgName type="university">Nancy-Université</orgName><placeName><settlement type="city">Nancy</settlement><region type="region" nuts="2">Grand Est</region><region type="region" nuts="2">Lorraine (région)</region></placeName><orgName type="laboratoire" n="5">Laboratoire réactions et génie des procédés</orgName><orgName type="university">Université de Lorraine</orgName><orgName type="institution">Centre national de la recherche scientifique</orgName></affiliation></author><author><name sortKey="Zhang, Kuiwen" sort="Zhang, Kuiwen" uniqKey="Zhang K" first="Kuiwen" last="Zhang">Kuiwen Zhang</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author><author><name sortKey="Qi, Fei" sort="Qi, Fei" uniqKey="Qi F" first="Fei" last="Qi">Fei Qi</name><affiliation wicri:level="1"><nlm:aff id="A2">National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029, P. R. China</nlm:aff><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>National Synchrotron Radiation Laboratory, University of Science and Technology of China, Hefei, Anhui 230029</wicri:regionArea><wicri:noRegion>Anhui 230029</wicri:noRegion></affiliation></author></analytic><series><title level="j">Combustion and flame</title><idno type="ISSN">0010-2180</idno><idno type="eISSN">1556-2921</idno><imprint><date when="2011">2011</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p id="P2">The detailed chemical structures of three low-pressure (35 Torr) premixed laminar furan/oxygen/argon flames with equivalence ratios of 1.4, 1.8 and 2.2 have been investigated by using tunable synchrotron vacuum ultraviolet (VUV) photoionization and molecular-beam mass spectrometry. About 40 combustion species including hydrocarbons and oxygenated intermediates have been identified by measurements of photoionization efficiency spectra. Mole fraction profiles of the flame species including reactants, intermediates and products have been determined by scanning burner position with some selected photon energies near ionization thresholds. Flame temperatures have been measured by a Pt-6%Rh/Pt-30%Rh thermocouple. A new mechanism involving 206 species and 1368 reactions has been proposed whose predictions are in reasonable agreement with measured species profiles for the three investigated flames. Rate-of-production and sensitivity analyses have been performed to track the key reaction paths governing furan consumption for different equivalence ratios. Both experimental and modeling results indicate that few aromatics could be formed in these flames. Furthermore, the current model has been validated against previous pyrolysis results of the literature obtained behind shock waves and the agreement is reasonable as well.</p></div></front></TEI></PMC></double></record>Pour manipuler ce document sous Unix (Dilib)
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