Adsorption Property and Mechanism of Oxytetracycline onto Willow Residues.
Identifieur interne : 000808 ( Main/Corpus ); précédent : 000807; suivant : 000809Adsorption Property and Mechanism of Oxytetracycline onto Willow Residues.
Auteurs : Di Wang ; Haiyang Xu ; Shengke Yang ; Wenke Wang ; Yanhua WangSource :
- International journal of environmental research and public health [ 1660-4601 ] ; 2017.
English descriptors
- KwdEn :
- Adsorption (MeSH), Anti-Bacterial Agents (metabolism), Environmental Restoration and Remediation (methods), Hydrogen-Ion Concentration (MeSH), Kinetics (MeSH), Microscopy, Electron, Scanning (MeSH), Oxytetracycline (metabolism), Plant Leaves (metabolism), Plant Roots (metabolism), Plant Stems (metabolism), Salix (metabolism), Spectroscopy, Fourier Transform Infrared (MeSH), Thermodynamics (MeSH), Water Pollutants, Chemical (metabolism).
- MESH :
- chemical , metabolism : Anti-Bacterial Agents, Oxytetracycline, Water Pollutants, Chemical.
- metabolism : Plant Leaves, Plant Roots, Plant Stems, Salix.
- methods : Environmental Restoration and Remediation.
- Adsorption, Hydrogen-Ion Concentration, Kinetics, Microscopy, Electron, Scanning, Spectroscopy, Fourier Transform Infrared, Thermodynamics.
Abstract
To elucidate the adsorption property and the mechanism of plant residues to reduce oxytetracycline (OTC), the adsorption of OTC onto raw willow roots (WR-R), stems (WS-R), leaves (WL-R), and adsorption onto desugared willow roots (WR-D), stems (WS-D), and leaves (WL-D) were investigated. The structural characterization was analyzed by scanning electron microscopy, Fourier-transform infrared spectra, and an elemental analyzer. OTC adsorption onto the different tissues of willow residues was compared and correlated with their structures. The adsorption kinetics of OTC onto willow residues was found to follow the pseudo-first-order model. The isothermal adsorption process of OTC onto the different tissues of willow residues followed the Langmuir and Freundlich model and the process was also a spontaneous endothermic reaction, which was mainly physical adsorption. After the willow residues were desugared, the polarity decreased and the aromaticity increased, which explained why the adsorption amounts of the desugared willow residues were higher than those of the unmodified residues. These observations suggest that the raw and modified willow residues have great potential as adsorbents to remove organic pollutants.
DOI: 10.3390/ijerph15010008
PubMed: 29271892
PubMed Central: PMC5800108
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Liaoyang 111003, China. 13386793382@163.com.</nlm:affiliation></affiliation></author><author><name sortKey="Yang, Shengke" sort="Yang, Shengke" uniqKey="Yang S" first="Shengke" last="Yang">Shengke Yang</name><affiliation><nlm:affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. ysk110@126.com.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. ysk110@126.com.</nlm:affiliation></affiliation></author><author><name sortKey="Wang, Wenke" sort="Wang, Wenke" uniqKey="Wang W" first="Wenke" last="Wang">Wenke Wang</name><affiliation><nlm:affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. wenkew@chd.edu.cn.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>School of Environmental 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wicri:step="Corpus" wicri:corpus="PubMed">000808</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en">Adsorption Property and Mechanism of Oxytetracycline onto Willow Residues.</title><author><name sortKey="Wang, Di" sort="Wang, Di" uniqKey="Wang D" first="Di" last="Wang">Di Wang</name><affiliation><nlm:affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. wd4591@126.com.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. wd4591@126.com.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>College of Natural Resources and Environment, Northwest A&F University, Yangling 712100, China. wd4591@126.com.</nlm:affiliation></affiliation></author><author><name sortKey="Xu, Haiyang" sort="Xu, Haiyang" uniqKey="Xu H" first="Haiyang" last="Xu">Haiyang Xu</name><affiliation><nlm:affiliation>Liaoning Zhongwang Group Co., Ltd., Liaoyang 111003, China. 13386793382@163.com.</nlm:affiliation></affiliation></author><author><name sortKey="Yang, Shengke" sort="Yang, Shengke" uniqKey="Yang S" first="Shengke" last="Yang">Shengke Yang</name><affiliation><nlm:affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. ysk110@126.com.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. ysk110@126.com.</nlm:affiliation></affiliation></author><author><name sortKey="Wang, Wenke" sort="Wang, Wenke" uniqKey="Wang W" first="Wenke" last="Wang">Wenke Wang</name><affiliation><nlm:affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. wenkew@chd.edu.cn.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. wenkew@chd.edu.cn.</nlm:affiliation></affiliation></author><author><name sortKey="Wang, Yanhua" sort="Wang, Yanhua" uniqKey="Wang Y" first="Yanhua" last="Wang">Yanhua Wang</name><affiliation><nlm:affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. yhwang930@foxmail.com.</nlm:affiliation></affiliation><affiliation><nlm:affiliation>School of Geography and Tourism, Shaanxi Normal University, Xi'an 710054, China. yhwang930@foxmail.com.</nlm:affiliation></affiliation></author></analytic><series><title level="j">International journal of environmental research and public health</title><idno type="eISSN">1660-4601</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Adsorption (MeSH)</term><term>Anti-Bacterial Agents (metabolism)</term><term>Environmental Restoration and Remediation (methods)</term><term>Hydrogen-Ion Concentration (MeSH)</term><term>Kinetics (MeSH)</term><term>Microscopy, Electron, Scanning (MeSH)</term><term>Oxytetracycline (metabolism)</term><term>Plant Leaves (metabolism)</term><term>Plant Roots (metabolism)</term><term>Plant Stems (metabolism)</term><term>Salix (metabolism)</term><term>Spectroscopy, Fourier Transform Infrared (MeSH)</term><term>Thermodynamics (MeSH)</term><term>Water Pollutants, Chemical (metabolism)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="metabolism" xml:lang="en"><term>Anti-Bacterial Agents</term><term>Oxytetracycline</term><term>Water Pollutants, Chemical</term></keywords><keywords scheme="MESH" qualifier="metabolism" xml:lang="en"><term>Plant Leaves</term><term>Plant Roots</term><term>Plant Stems</term><term>Salix</term></keywords><keywords scheme="MESH" qualifier="methods" xml:lang="en"><term>Environmental Restoration and Remediation</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Adsorption</term><term>Hydrogen-Ion Concentration</term><term>Kinetics</term><term>Microscopy, Electron, Scanning</term><term>Spectroscopy, Fourier Transform Infrared</term><term>Thermodynamics</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">To elucidate the adsorption property and the mechanism of plant residues to reduce oxytetracycline (OTC), the adsorption of OTC onto raw willow roots (WR-R), stems (WS-R), leaves (WL-R), and adsorption onto desugared willow roots (WR-D), stems (WS-D), and leaves (WL-D) were investigated. The structural characterization was analyzed by scanning electron microscopy, Fourier-transform infrared spectra, and an elemental analyzer. OTC adsorption onto the different tissues of willow residues was compared and correlated with their structures. The adsorption kinetics of OTC onto willow residues was found to follow the pseudo-first-order model. The isothermal adsorption process of OTC onto the different tissues of willow residues followed the Langmuir and Freundlich model and the process was also a spontaneous endothermic reaction, which was mainly physical adsorption. After the willow residues were desugared, the polarity decreased and the aromaticity increased, which explained why the adsorption amounts of the desugared willow residues were higher than those of the unmodified residues. These observations suggest that the raw and modified willow residues have great potential as adsorbents to remove organic pollutants.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Curated" Owner="NLM"><PMID Version="1">29271892</PMID><DateCompleted><Year>2018</Year><Month>11</Month><Day>26</Day></DateCompleted><DateRevised><Year>2018</Year><Month>11</Month><Day>26</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Electronic">1660-4601</ISSN><JournalIssue CitedMedium="Internet"><Volume>15</Volume><Issue>1</Issue><PubDate><Year>2017</Year><Month>12</Month><Day>22</Day></PubDate></JournalIssue><Title>International journal of environmental research and public health</Title><ISOAbbreviation>Int J Environ Res Public Health</ISOAbbreviation></Journal><ArticleTitle>Adsorption Property and Mechanism of Oxytetracycline onto Willow Residues.</ArticleTitle><ELocationID EIdType="pii" ValidYN="Y">E8</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.3390/ijerph15010008</ELocationID><Abstract><AbstractText>To elucidate the adsorption property and the mechanism of plant residues to reduce oxytetracycline (OTC), the adsorption of OTC onto raw willow roots (WR-R), stems (WS-R), leaves (WL-R), and adsorption onto desugared willow roots (WR-D), stems (WS-D), and leaves (WL-D) were investigated. The structural characterization was analyzed by scanning electron microscopy, Fourier-transform infrared spectra, and an elemental analyzer. OTC adsorption onto the different tissues of willow residues was compared and correlated with their structures. The adsorption kinetics of OTC onto willow residues was found to follow the pseudo-first-order model. The isothermal adsorption process of OTC onto the different tissues of willow residues followed the Langmuir and Freundlich model and the process was also a spontaneous endothermic reaction, which was mainly physical adsorption. After the willow residues were desugared, the polarity decreased and the aromaticity increased, which explained why the adsorption amounts of the desugared willow residues were higher than those of the unmodified residues. These observations suggest that the raw and modified willow residues have great potential as adsorbents to remove organic pollutants.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Di</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. wd4591@126.com.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. wd4591@126.com.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>College of Natural Resources and Environment, Northwest A&F University, Yangling 712100, China. wd4591@126.com.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Xu</LastName><ForeName>Haiyang</ForeName><Initials>H</Initials><AffiliationInfo><Affiliation>Liaoning Zhongwang Group Co., Ltd., Liaoyang 111003, China. 13386793382@163.com.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yang</LastName><ForeName>Shengke</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. ysk110@126.com.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. ysk110@126.com.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Wenke</ForeName><Initials>W</Initials><AffiliationInfo><Affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. wenkew@chd.edu.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China. wenkew@chd.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Yanhua</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region, Ministry of Education, Chang'an University, Xi'an 710054, China. yhwang930@foxmail.com.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>School of Geography and Tourism, Shaanxi Normal University, Xi'an 710054, China. yhwang930@foxmail.com.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType><PublicationType UI="D013485">Research Support, Non-U.S. Gov't</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2017</Year><Month>12</Month><Day>22</Day></ArticleDate></Article><MedlineJournalInfo><Country>Switzerland</Country><MedlineTA>Int J Environ Res Public Health</MedlineTA><NlmUniqueID>101238455</NlmUniqueID><ISSNLinking>1660-4601</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D000900">Anti-Bacterial Agents</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D014874">Water Pollutants, Chemical</NameOfSubstance></Chemical><Chemical><RegistryNumber>X20I9EN955</RegistryNumber><NameOfSubstance UI="D010118">Oxytetracycline</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000327" MajorTopicYN="Y">Adsorption</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D000900" MajorTopicYN="N">Anti-Bacterial Agents</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="Y">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D052918" MajorTopicYN="N">Environmental Restoration and Remediation</DescriptorName><QualifierName UI="Q000379" MajorTopicYN="Y">methods</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D006863" MajorTopicYN="N">Hydrogen-Ion Concentration</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D007700" MajorTopicYN="N">Kinetics</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008855" MajorTopicYN="N">Microscopy, Electron, Scanning</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D010118" MajorTopicYN="N">Oxytetracycline</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="Y">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D018515" MajorTopicYN="N">Plant Leaves</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="N">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D018517" MajorTopicYN="N">Plant Roots</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="N">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D018547" MajorTopicYN="N">Plant Stems</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="N">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D032108" MajorTopicYN="N">Salix</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="Y">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D017550" MajorTopicYN="N">Spectroscopy, Fourier Transform Infrared</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D013816" MajorTopicYN="N">Thermodynamics</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D014874" MajorTopicYN="N">Water Pollutants, Chemical</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="Y">metabolism</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="Y">PPCPs</Keyword><Keyword MajorTopicYN="Y">adsorption</Keyword><Keyword MajorTopicYN="Y">oxytetracycline</Keyword><Keyword MajorTopicYN="Y">willow residues</Keyword></KeywordList><CoiStatement>The authors declare no conflict of interest.</CoiStatement></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2017</Year><Month>11</Month><Day>07</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2017</Year><Month>12</Month><Day>13</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2017</Year><Month>12</Month><Day>20</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2017</Year><Month>12</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2017</Year><Month>12</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2018</Year><Month>11</Month><Day>27</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>epublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">29271892</ArticleId><ArticleId IdType="pii">ijerph15010008</ArticleId><ArticleId IdType="doi">10.3390/ijerph15010008</ArticleId><ArticleId 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