Development of High-Antifouling PPSU Ultrafiltration Membrane by Using Compound Additives: Preparation, Morphologies, and Filtration Resistant Properties
Identifieur interne : 000256 ( Main/Exploration ); précédent : 000255; suivant : 000257Development of High-Antifouling PPSU Ultrafiltration Membrane by Using Compound Additives: Preparation, Morphologies, and Filtration Resistant Properties
Auteurs : Jie Liu ; Zhencheng Zhong ; Rui Ma ; Weichen Zhang ; Jiding LiSource :
- Membranes [ 2077-0375 ] ; 2016.
Abstract
In this study, flat sheet asymmetric polyphenylsulfone (PPSU) ultrafiltration membranes with enhanced antifouling properties were prepared with a non-solvent induced phase separation (NIPS) method through compound additives containing a polymeric pore-forming agent, a small molecular non-solvent and a surfactant. The formation processes of the porous asymmetric membranes with different kinds of additives were studied in detail, and the microstructure controllable preparation of membrane was achieved by establishing a bridge between the membrane preparation parameters and separation performances. All prepared membranes were characterized by using a scanning electron microscope (SEM), contact angle analysis, porosity, maximum pore size, water and BSA solution permeability studies. The performance efficiency of the membrane was evaluated by using BSA as a model foulant in terms of permeability, solute rejection (
Url:
DOI: 10.3390/membranes6020035
PubMed: 27338487
PubMed Central: 4931530
Affiliations:
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">Development of High-Antifouling PPSU Ultrafiltration Membrane by Using Compound Additives: Preparation, Morphologies, and Filtration Resistant Properties</title><author><name sortKey="Liu, Jie" sort="Liu, Jie" uniqKey="Liu J" first="Jie" last="Liu">Jie Liu</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-membranes-06-00035">The State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China;<email>lijiding@mail.tsinghua.edu.cn</email></nlm:aff></affiliation></author><author><name sortKey="Zhong, Zhencheng" sort="Zhong, Zhencheng" uniqKey="Zhong Z" first="Zhencheng" last="Zhong">Zhencheng Zhong</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation></author><author><name sortKey="Ma, Rui" sort="Ma, Rui" uniqKey="Ma R" first="Rui" last="Ma">Rui Ma</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation></author><author><name sortKey="Zhang, Weichen" sort="Zhang, Weichen" uniqKey="Zhang W" first="Weichen" last="Zhang">Weichen Zhang</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation></author><author><name sortKey="Li, Jiding" sort="Li, Jiding" uniqKey="Li J" first="Jiding" last="Li">Jiding Li</name><affiliation><nlm:aff id="af2-membranes-06-00035">The State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China;<email>lijiding@mail.tsinghua.edu.cn</email></nlm:aff></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PMC</idno><idno type="pmid">27338487</idno><idno type="pmc">4931530</idno><idno type="url">http://www.ncbi.nlm.nih.gov/pmc/articles/PMC4931530</idno><idno type="RBID">PMC:4931530</idno><idno type="doi">10.3390/membranes6020035</idno><date when="2016">2016</date><idno type="wicri:Area/Pmc/Corpus">000360</idno><idno type="wicri:Area/Pmc/Curation">000359</idno><idno type="wicri:Area/Pmc/Checkpoint">000211</idno><idno type="wicri:Area/Ncbi/Merge">002083</idno><idno type="wicri:Area/Ncbi/Curation">002083</idno><idno type="wicri:Area/Ncbi/Checkpoint">002083</idno><idno type="wicri:Area/Main/Merge">000256</idno><idno type="wicri:Area/Main/Curation">000256</idno><idno type="wicri:Area/Main/Exploration">000256</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a" type="main">Development of High-Antifouling PPSU Ultrafiltration Membrane by Using Compound Additives: Preparation, Morphologies, and Filtration Resistant Properties</title><author><name sortKey="Liu, Jie" sort="Liu, Jie" uniqKey="Liu J" first="Jie" last="Liu">Jie Liu</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation><affiliation><nlm:aff id="af2-membranes-06-00035">The State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China;<email>lijiding@mail.tsinghua.edu.cn</email></nlm:aff></affiliation></author><author><name sortKey="Zhong, Zhencheng" sort="Zhong, Zhencheng" uniqKey="Zhong Z" first="Zhencheng" last="Zhong">Zhencheng Zhong</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation></author><author><name sortKey="Ma, Rui" sort="Ma, Rui" uniqKey="Ma R" first="Rui" last="Ma">Rui Ma</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation></author><author><name sortKey="Zhang, Weichen" sort="Zhang, Weichen" uniqKey="Zhang W" first="Weichen" last="Zhang">Weichen Zhang</name><affiliation><nlm:aff id="af1-membranes-06-00035">National Institute of Clean and Low Carbon Energy, Beijing 102209, China;<email>zhongzhencheng@nicenergy.com</email> (Z.Z.);<email>marui@nicenergy.com</email> (R.M.);<email>zhangweichen@nicenergy.com</email> (W.Z.)</nlm:aff></affiliation></author><author><name sortKey="Li, Jiding" sort="Li, Jiding" uniqKey="Li J" first="Jiding" last="Li">Jiding Li</name><affiliation><nlm:aff id="af2-membranes-06-00035">The State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China;<email>lijiding@mail.tsinghua.edu.cn</email></nlm:aff></affiliation></author></analytic><series><title level="j">Membranes</title><idno type="eISSN">2077-0375</idno><imprint><date when="2016">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>In this study, flat sheet asymmetric polyphenylsulfone (PPSU) ultrafiltration membranes with enhanced antifouling properties were prepared with a non-solvent induced phase separation (NIPS) method through compound additives containing a polymeric pore-forming agent, a small molecular non-solvent and a surfactant. The formation processes of the porous asymmetric membranes with different kinds of additives were studied in detail, and the microstructure controllable preparation of membrane was achieved by establishing a bridge between the membrane preparation parameters and separation performances. All prepared membranes were characterized by using a scanning electron microscope (SEM), contact angle analysis, porosity, maximum pore size, water and BSA solution permeability studies. The performance efficiency of the membrane was evaluated by using BSA as a model foulant in terms of permeability, solute rejection (<italic>R</italic>), <italic>R<sub>m</sub></italic> (membrane inherent resistance), <italic>R<sub>c</sub></italic> (cake layer resistance), and <italic>R<sub>p</sub></italic> (pore plugging resistance). The results showed that when the compound additives were used, the inter-connected pores were observed, maximum pore size, contact angle and membrane filtration resistance decreased, while the porosity increased. When PVP compound additives were added, the water flux increased from 80.4 to 148.1 L/(m<sup>2</sup>·h), the BSA rejection increased from 53.2% to 81.5%. A similar trend was observed for membranes with added PEG compound additives; the water flux and BSA rejection simultaneously increased. The filtration resistance decreased as a result of compound additives. The uniformity of membrane and the number of effective pores could be enhanced by adding compound additives through the cooperation of different additives.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Aghigh, A" uniqKey="Aghigh A">A. Aghigh</name></author><author><name sortKey="Alizadeh, V" uniqKey="Alizadeh V">V. 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