AustralieFrV1, PascalFrancis, Curation, bibRecord, 005524

Ammonia-mediated suppression of coke formation in direct-methane solid oxide fuel cells with nickel-based anodes

Identifieur interne : 005524 ( PascalFrancis/Curation ); précédent : 005523; suivant : 005525

Ammonia-mediated suppression of coke formation in direct-methane solid oxide fuel cells with nickel-based anodes

Auteurs : WEI WANG [République populaire de Chine] ; RAN RAN [République populaire de Chine] ; CHAO SU [Australie] ; YOUMIN CUO [France] ; David Farrusseng [France] ; ZONGPING SHAO [République populaire de Chine, Australie]

Source :

Journal of power sources [ 0378-7753 ] ; 2013.

RBID : Pascal:13-0235294

Descripteurs français

Pascal (Inist)
- Coke, Formation, Pile combustible oxyde solide, Anode, Ammoniac, Méthane, Nickel, Matériau électrode, ..
Wicri :
- topic : Coke, Nickel.

English descriptors

KwdEn :
- Ammonia, Anode, Coke, Electrode material, Formation, Methane, Nickel, Solid oxide fuel cell.

Abstract

In this study, we report a novel approach for suppressing coke formation in direct-methane solid oxide fuel cells (SOFCs) with a conventional nickel cermet anode by simply adding ammonia to the fuel gas. Because ammonia preferentially occupies the acidic sites of the anode catalyst materials, a significant decrease in the coke formation rate is realized by introducing ammonia into the methane gas. In addition, hydrogen, a decomposition product of ammonia, also acts as an additional fuel for the SOFCs, resulting in high cell performance. At 700 °C, the coke formation rate over the Ni-YSZ anode is suppressed by 71% after the addition of 33.3% NH₃ into CH₄. Suppressed coke formation is also observed for other Ni catalysts such as Ni/Al₂O₃, a common catalyst for methane reforming that has been successfully used as the anode catalyst layer for SOFCs operating on methane, which suggests that introducing NH₃ as an additive gas is a general method for suppressing the coke formation. The addition of ammonia can also effectively improve the power output and operational stability and offers a novel means for developing new coke-resistant SOFCs operating on widely available hydrocarbons for clean power generation to realize a sustainable future.

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A11	`01`	`1`		`@1 WEI WANG`
A11	`02`	`1`		`@1 RAN RAN`
A11	`03`	`1`		`@1 CHAO SU`
A11	`04`	`1`		`@1 YOUMIN CUO`
A11	`05`	`1`		`@1 FARRUSSENG (David)`
A11	`06`	`1`		`@1 ZONGPING SHAO`
A14	`01`			`@1 State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemistry & Chemical Engineering, Nanjing University of Technology, No. 5 Xin Mofan Road @2 Nanjing 210009 @3 CHN @Z 1 aut. @Z 2 aut. @Z 6 aut.`
A14	`02`			`@1 Department of Chemical Engineering, Curtin University @2 Perth, WA 6845 @3 AUS @Z 3 aut. @Z 6 aut.`
A14	`03`			`@1 Institut de Recherches sur la Catalyse et l'Environnement de Lyon (IRCELYON), UMR5256, CNRS/Université Claude Bernard, Lyon 1, 2 Av. A. Einstein @2 69626 Villeurbanne @3 FRA @Z 4 aut. @Z 5 aut.`
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A44				`@0 0000 @1 © 2013 INIST-CNRS. All rights reserved.`
A45				`@0 35 ref.`
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A64	`01`	`1`		`@0 Journal of power sources`
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C01	`01`		`ENG`	@0 In this study, we report a novel approach for suppressing coke formation in direct-methane solid oxide fuel cells (SOFCs) with a conventional nickel cermet anode by simply adding ammonia to the fuel gas. Because ammonia preferentially occupies the acidic sites of the anode catalyst materials, a significant decrease in the coke formation rate is realized by introducing ammonia into the methane gas. In addition, hydrogen, a decomposition product of ammonia, also acts as an additional fuel for the SOFCs, resulting in high cell performance. At 700 °C, the coke formation rate over the Ni-YSZ anode is suppressed by 71% after the addition of 33.3% NH₃ into CH₄. Suppressed coke formation is also observed for other Ni catalysts such as Ni/Al₂O₃, a common catalyst for methane reforming that has been successfully used as the anode catalyst layer for SOFCs operating on methane, which suggests that introducing NH₃ as an additive gas is a general method for suppressing the coke formation. The addition of ammonia can also effectively improve the power output and operational stability and offers a novel means for developing new coke-resistant SOFCs operating on widely available hydrocarbons for clean power generation to realize a sustainable future.
C02	`01`	`X`		`@0 001D06D03E`
C02	`02`	`X`		`@0 001D05I03E`
C02	`03`	`X`		`@0 001D05C`
C02	`04`	`X`		`@0 230`
C03	`01`	`X`	`FRE`	`@0 Coke @5 01`
C03	`01`	`X`	`ENG`	`@0 Coke @5 01`
C03	`01`	`X`	`SPA`	`@0 Coque @5 01`
C03	`02`	`X`	`FRE`	`@0 Formation @5 02`
C03	`02`	`X`	`ENG`	`@0 Formation @5 02`
C03	`02`	`X`	`SPA`	`@0 Formación @5 02`
C03	`03`	`X`	`FRE`	`@0 Pile combustible oxyde solide @5 03`
C03	`03`	`X`	`ENG`	`@0 Solid oxide fuel cell @5 03`
C03	`03`	`X`	`SPA`	`@0 Pila combustible oxido sólido @5 03`
C03	`04`	`X`	`FRE`	`@0 Anode @5 04`
C03	`04`	`X`	`ENG`	`@0 Anode @5 04`
C03	`04`	`X`	`SPA`	`@0 Anodo @5 04`
C03	`05`	`X`	`FRE`	`@0 Ammoniac @2 NK @2 FX @5 22`
C03	`05`	`X`	`ENG`	`@0 Ammonia @2 NK @2 FX @5 22`
C03	`05`	`X`	`SPA`	`@0 Amoníaco @2 NK @2 FX @5 22`
C03	`06`	`X`	`FRE`	`@0 Méthane @2 NK @2 FX @5 23`
C03	`06`	`X`	`ENG`	`@0 Methane @2 NK @2 FX @5 23`
C03	`06`	`X`	`SPA`	`@0 Metano @2 NK @2 FX @5 23`
C03	`07`	`X`	`FRE`	`@0 Nickel @2 NC @2 FX @5 24`
C03	`07`	`X`	`ENG`	`@0 Nickel @2 NC @2 FX @5 24`
C03	`07`	`X`	`SPA`	`@0 Niquel @2 NC @2 FX @5 24`
C03	`08`	`X`	`FRE`	`@0 Matériau électrode @5 46`
C03	`08`	`X`	`ENG`	`@0 Electrode material @5 46`
C03	`08`	`X`	`SPA`	`@0 Material electrodo @5 46`
C03	`09`	`X`	`FRE`	`@0 . @4 INC @5 82`
C07	`01`	`X`	`FRE`	`@0 Métal transition @2 NC @5 05`
C07	`01`	`X`	`ENG`	`@0 Transition metal @2 NC @5 05`
C07	`01`	`X`	`SPA`	`@0 Metal transición @2 NC @5 05`
N21				`@1 217`
N44	`01`			`@1 OTO`
N82				`@1 OTO`

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Le document en format XML

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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Ammonia-mediated suppression of coke formation in direct-methane solid oxide fuel cells with nickel-based anodes</title>
<author><name sortKey="Wei Wang" sort="Wei Wang" uniqKey="Wei Wang" last="Wei Wang">WEI WANG</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemistry & Chemical Engineering, Nanjing University of Technology, No. 5 Xin Mofan Road</s1>
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<author><name sortKey="Ran Ran" sort="Ran Ran" uniqKey="Ran Ran" last="Ran Ran">RAN RAN</name>
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<author><name sortKey="Chao Su" sort="Chao Su" uniqKey="Chao Su" last="Chao Su">CHAO SU</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Department of Chemical Engineering, Curtin University</s1>
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<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>Institut de Recherches sur la Catalyse et l'Environnement de Lyon (IRCELYON), UMR5256, CNRS/Université Claude Bernard, Lyon 1, 2 Av. A. Einstein</s1>
<s2>69626 Villeurbanne</s2>
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<author><name sortKey="Farrusseng, David" sort="Farrusseng, David" uniqKey="Farrusseng D" first="David" last="Farrusseng">David Farrusseng</name>
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</affiliation>
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<author><name sortKey="Zongping Shao" sort="Zongping Shao" uniqKey="Zongping Shao" last="Zongping Shao">ZONGPING SHAO</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemistry & Chemical Engineering, Nanjing University of Technology, No. 5 Xin Mofan Road</s1>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Ammonia</term>
<term>Anode</term>
<term>Coke</term>
<term>Electrode material</term>
<term>Formation</term>
<term>Methane</term>
<term>Nickel</term>
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<term>Pile combustible oxyde solide</term>
<term>Anode</term>
<term>Ammoniac</term>
<term>Méthane</term>
<term>Nickel</term>
<term>Matériau électrode</term>
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<front><div type="abstract" xml:lang="en">In this study, we report a novel approach for suppressing coke formation in direct-methane solid oxide fuel cells (SOFCs) with a conventional nickel cermet anode by simply adding ammonia to the fuel gas. Because ammonia preferentially occupies the acidic sites of the anode catalyst materials, a significant decrease in the coke formation rate is realized by introducing ammonia into the methane gas. In addition, hydrogen, a decomposition product of ammonia, also acts as an additional fuel for the SOFCs, resulting in high cell performance. At 700 °C, the coke formation rate over the Ni-YSZ anode is suppressed by 71% after the addition of 33.3% NH<sub>3</sub>
 into CH<sub>4</sub>
. Suppressed coke formation is also observed for other Ni catalysts such as Ni/Al<sub>2</sub>
O<sub>3</sub>
, a common catalyst for methane reforming that has been successfully used as the anode catalyst layer for SOFCs operating on methane, which suggests that introducing NH<sub>3</sub>
 as an additive gas is a general method for suppressing the coke formation. The addition of ammonia can also effectively improve the power output and operational stability and offers a novel means for developing new coke-resistant SOFCs operating on widely available hydrocarbons for clean power generation to realize a sustainable future.</div>
</front>
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<fA14 i1="01"><s1>State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemistry & Chemical Engineering, Nanjing University of Technology, No. 5 Xin Mofan Road</s1>
<s2>Nanjing 210009</s2>
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<fA14 i1="02"><s1>Department of Chemical Engineering, Curtin University</s1>
<s2>Perth, WA 6845</s2>
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<fA14 i1="03"><s1>Institut de Recherches sur la Catalyse et l'Environnement de Lyon (IRCELYON), UMR5256, CNRS/Université Claude Bernard, Lyon 1, 2 Av. A. Einstein</s1>
<s2>69626 Villeurbanne</s2>
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<fC01 i1="01" l="ENG"><s0>In this study, we report a novel approach for suppressing coke formation in direct-methane solid oxide fuel cells (SOFCs) with a conventional nickel cermet anode by simply adding ammonia to the fuel gas. Because ammonia preferentially occupies the acidic sites of the anode catalyst materials, a significant decrease in the coke formation rate is realized by introducing ammonia into the methane gas. In addition, hydrogen, a decomposition product of ammonia, also acts as an additional fuel for the SOFCs, resulting in high cell performance. At 700 °C, the coke formation rate over the Ni-YSZ anode is suppressed by 71% after the addition of 33.3% NH<sub>3</sub>
 into CH<sub>4</sub>
. Suppressed coke formation is also observed for other Ni catalysts such as Ni/Al<sub>2</sub>
O<sub>3</sub>
, a common catalyst for methane reforming that has been successfully used as the anode catalyst layer for SOFCs operating on methane, which suggests that introducing NH<sub>3</sub>
 as an additive gas is a general method for suppressing the coke formation. The addition of ammonia can also effectively improve the power output and operational stability and offers a novel means for developing new coke-resistant SOFCs operating on widely available hydrocarbons for clean power generation to realize a sustainable future.</s0>
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<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Solid oxide fuel cell</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA"><s0>Pila combustible oxido sólido</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE"><s0>Anode</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG"><s0>Anode</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA"><s0>Anodo</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE"><s0>Ammoniac</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>22</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG"><s0>Ammonia</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>22</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA"><s0>Amoníaco</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>22</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE"><s0>Méthane</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>23</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Methane</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>23</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Metano</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>23</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Nickel</s0>
<s2>NC</s2>
<s2>FX</s2>
<s5>24</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Nickel</s0>
<s2>NC</s2>
<s2>FX</s2>
<s5>24</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Niquel</s0>
<s2>NC</s2>
<s2>FX</s2>
<s5>24</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Matériau électrode</s0>
<s5>46</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Electrode material</s0>
<s5>46</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Material electrodo</s0>
<s5>46</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>.</s0>
<s4>INC</s4>
<s5>82</s5>
</fC03>
<fC07 i1="01" i2="X" l="FRE"><s0>Métal transition</s0>
<s2>NC</s2>
<s5>05</s5>
</fC07>
<fC07 i1="01" i2="X" l="ENG"><s0>Transition metal</s0>
<s2>NC</s2>
<s5>05</s5>
</fC07>
<fC07 i1="01" i2="X" l="SPA"><s0>Metal transición</s0>
<s2>NC</s2>
<s5>05</s5>
</fC07>
<fN21><s1>217</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
</pA>
</standard>
</inist>
</record>

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   |texte=   Ammonia-mediated suppression of coke formation in direct-methane solid oxide fuel cells with nickel-based anodes
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	Serveur d'exploration sur les relations entre la France et l'Australie
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Ammonia-mediated suppression of coke formation in direct-methane solid oxide fuel cells with nickel-based anodes

Ammonia-mediated suppression of coke formation in direct-methane solid oxide fuel cells with nickel-based anodes

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