Quasi one-dimensional band dispersion and surface metallization in long-range ordered polymeric wires
Identifieur interne : 002F38 ( Ncbi/Checkpoint ); précédent : 002F37; suivant : 002F39Quasi one-dimensional band dispersion and surface metallization in long-range ordered polymeric wires
Auteurs : Guillaume Vasseur [France] ; Yannick Fagot-Revurat [France] ; Muriel Sicot [France] ; Bertrand Kierren [France] ; Luc Moreau [France] ; Daniel Malterre [France] ; Luis Cardenas [Canada, France] ; Gianluca Galeotti [Canada] ; Josh Lipton-Duffin [Canada, Australie] ; Federico Rosei [Canada, République populaire de Chine] ; Marco Di Giovannantonio [Italie] ; Giorgio Contini [Italie] ; Patrick Le Fèvre [France] ; François Bertran [France] ; Liangbo Liang [États-Unis] ; Vincent Meunier [États-Unis] ; Dmitrii F. Perepichka [Canada]Source :
- Nature Communications [ 2041-1723 ] ; 2016.
Abstract
On-surface covalent self-assembly of organic molecules is a very promising bottom–up approach for producing atomically controlled nanostructures. Due to their highly tuneable properties, these structures may be used as building blocks in electronic carbon-based molecular devices. Following this idea, here we report on the electronic structure of an ordered array of poly(para-phenylene) nanowires produced by surface-catalysed dehalogenative reaction. By scanning tunnelling spectroscopy we follow the quantization of unoccupied molecular states as a function of oligomer length, with Fermi level crossing observed for long chains. Angle-resolved photoelectron spectroscopy reveals a quasi-1D valence band as well as a direct gap of 1.15 eV, as the conduction band is partially filled through adsorption on the surface. Tight-binding modelling and
Url:
DOI: 10.1038/ncomms10235
PubMed: 26725974
PubMed Central: 4725758
Affiliations:
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a" type="main">Quasi one-dimensional band dispersion and surface metallization in long-range ordered polymeric wires</title>
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<author><name sortKey="Fagot Revurat, Yannick" sort="Fagot Revurat, Yannick" uniqKey="Fagot Revurat Y" first="Yannick" last="Fagot-Revurat">Yannick Fagot-Revurat</name>
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, BP 70239, F-54506 Vandoeuvre-les-Nancy,<country>France</country>
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<author><name sortKey="Sicot, Muriel" sort="Sicot, Muriel" uniqKey="Sicot M" first="Muriel" last="Sicot">Muriel Sicot</name>
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<author><name sortKey="Cardenas, Luis" sort="Cardenas, Luis" uniqKey="Cardenas L" first="Luis" last="Cardenas">Luis Cardenas</name>
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<author><name sortKey="Lipton Duffin, Josh" sort="Lipton Duffin, Josh" uniqKey="Lipton Duffin J" first="Josh" last="Lipton-Duffin">Josh Lipton-Duffin</name>
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, 1650 Boulevard Lionel-Boulet, Varennes, Quebec,<country>Canada</country>
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<country xml:lang="fr">Canada</country>
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<affiliation wicri:level="1"><nlm:aff id="a4"><institution>Institute for Future Environments, Queensland University of Technology (QUT)</institution>
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</nlm:aff>
<country xml:lang="fr">Australie</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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<author><name sortKey="Rosei, Federico" sort="Rosei, Federico" uniqKey="Rosei F" first="Federico" last="Rosei">Federico Rosei</name>
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J3X 1S2</nlm:aff>
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<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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<affiliation wicri:level="1"><nlm:aff id="a5"><institution>Institute for Fundamental and Frontier Science, University of Electronic Science and Technology of China</institution>
, Chengdu 610054,<country>China</country>
</nlm:aff>
<country xml:lang="fr">République populaire de Chine</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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<author><name sortKey="Di Giovannantonio, Marco" sort="Di Giovannantonio, Marco" uniqKey="Di Giovannantonio M" first="Marco" last="Di Giovannantonio">Marco Di Giovannantonio</name>
<affiliation wicri:level="1"><nlm:aff id="a6"><institution>Instituto di Struttura della Materia, CNR</institution>
, Via Fosso del Cavaliere 100, 00133 Roma,<country>Italy</country>
</nlm:aff>
<country xml:lang="fr">Italie</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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<author><name sortKey="Contini, Giorgio" sort="Contini, Giorgio" uniqKey="Contini G" first="Giorgio" last="Contini">Giorgio Contini</name>
<affiliation wicri:level="1"><nlm:aff id="a6"><institution>Instituto di Struttura della Materia, CNR</institution>
, Via Fosso del Cavaliere 100, 00133 Roma,<country>Italy</country>
</nlm:aff>
<country xml:lang="fr">Italie</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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<affiliation wicri:level="1"><nlm:aff id="a7"><institution>Physics Department, University of Rome ‘Tor Vergata'</institution>
, Via della Ricerca Scientifica 1, I-00133 Roma,<country>Italy</country>
</nlm:aff>
<country xml:lang="fr">Italie</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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<author><name sortKey="Le Fevre, Patrick" sort="Le Fevre, Patrick" uniqKey="Le Fevre P" first="Patrick" last="Le Fèvre">Patrick Le Fèvre</name>
<affiliation wicri:level="1"><nlm:aff id="a8"><institution>Synchrotron SOLEIL, L'Orme des Merisiers, Saint-Aubin</institution>
, BP 48, F-91192 Gif sur Yvette,<country>France</country>
</nlm:aff>
<country xml:lang="fr">France</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
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</author>
<author><name sortKey="Bertran, Francois" sort="Bertran, Francois" uniqKey="Bertran F" first="François" last="Bertran">François Bertran</name>
<affiliation wicri:level="1"><nlm:aff id="a8"><institution>Synchrotron SOLEIL, L'Orme des Merisiers, Saint-Aubin</institution>
, BP 48, F-91192 Gif sur Yvette,<country>France</country>
</nlm:aff>
<country xml:lang="fr">France</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
</affiliation>
</author>
<author><name sortKey="Liang, Liangbo" sort="Liang, Liangbo" uniqKey="Liang L" first="Liangbo" last="Liang">Liangbo Liang</name>
<affiliation wicri:level="1"><nlm:aff id="a9"><institution>Department of Physics, Applied Physics, and Astronomy, Rensselaer Polytechnic Institute</institution>
, Troy, NY 12180,<country>USA</country>
</nlm:aff>
<country xml:lang="fr">États-Unis</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
</affiliation>
<affiliation wicri:level="1"><nlm:aff id="a10"><institution>Center for Nanophase Materials Sciences, Oak Ridge National Laboratory</institution>
, Oak Ridge, Tennessee 37831,<country>USA</country>
</nlm:aff>
<country xml:lang="fr">États-Unis</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
</affiliation>
</author>
<author><name sortKey="Meunier, Vincent" sort="Meunier, Vincent" uniqKey="Meunier V" first="Vincent" last="Meunier">Vincent Meunier</name>
<affiliation wicri:level="1"><nlm:aff id="a9"><institution>Department of Physics, Applied Physics, and Astronomy, Rensselaer Polytechnic Institute</institution>
, Troy, NY 12180,<country>USA</country>
</nlm:aff>
<country xml:lang="fr">États-Unis</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
</affiliation>
</author>
<author><name sortKey="Perepichka, Dmitrii F" sort="Perepichka, Dmitrii F" uniqKey="Perepichka D" first="Dmitrii F." last="Perepichka">Dmitrii F. Perepichka</name>
<affiliation wicri:level="1"><nlm:aff id="a11"><institution>Department of Chemistry, McGill University</institution>
, 801 Sherbrooke Street West, Montreal, Quebec,<country>Canada</country>
H3A 0B8</nlm:aff>
<country xml:lang="fr">Canada</country>
<wicri:regionArea># see nlm:aff country strict</wicri:regionArea>
</affiliation>
</author>
</analytic>
<series><title level="j">Nature Communications</title>
<idno type="eISSN">2041-1723</idno>
<imprint><date when="2016">2016</date>
</imprint>
</series>
</biblStruct>
</sourceDesc>
</fileDesc>
<profileDesc><textClass></textClass>
</profileDesc>
</teiHeader>
<front><div type="abstract" xml:lang="en"><p>On-surface covalent self-assembly of organic molecules is a very promising bottom–up approach for producing atomically controlled nanostructures. Due to their highly tuneable properties, these structures may be used as building blocks in electronic carbon-based molecular devices. Following this idea, here we report on the electronic structure of an ordered array of poly(para-phenylene) nanowires produced by surface-catalysed dehalogenative reaction. By scanning tunnelling spectroscopy we follow the quantization of unoccupied molecular states as a function of oligomer length, with Fermi level crossing observed for long chains. Angle-resolved photoelectron spectroscopy reveals a quasi-1D valence band as well as a direct gap of 1.15 eV, as the conduction band is partially filled through adsorption on the surface. Tight-binding modelling and <italic>ab initio</italic>
density functional theory calculations lead to a full description of the band structure, including the gap size and charge transfer mechanisms, highlighting a strong substrate–molecule interaction that drives the system into a metallic behaviour.</p>
</div>
</front>
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</biblStruct>
</listBibl>
</div1>
</back>
</TEI>
<affiliations><list><country><li>Australie</li>
<li>Canada</li>
<li>France</li>
<li>Italie</li>
<li>République populaire de Chine</li>
<li>États-Unis</li>
</country>
</list>
<tree><country name="France"><noRegion><name sortKey="Vasseur, Guillaume" sort="Vasseur, Guillaume" uniqKey="Vasseur G" first="Guillaume" last="Vasseur">Guillaume Vasseur</name>
</noRegion>
<name sortKey="Bertran, Francois" sort="Bertran, Francois" uniqKey="Bertran F" first="François" last="Bertran">François Bertran</name>
<name sortKey="Cardenas, Luis" sort="Cardenas, Luis" uniqKey="Cardenas L" first="Luis" last="Cardenas">Luis Cardenas</name>
<name sortKey="Fagot Revurat, Yannick" sort="Fagot Revurat, Yannick" uniqKey="Fagot Revurat Y" first="Yannick" last="Fagot-Revurat">Yannick Fagot-Revurat</name>
<name sortKey="Kierren, Bertrand" sort="Kierren, Bertrand" uniqKey="Kierren B" first="Bertrand" last="Kierren">Bertrand Kierren</name>
<name sortKey="Le Fevre, Patrick" sort="Le Fevre, Patrick" uniqKey="Le Fevre P" first="Patrick" last="Le Fèvre">Patrick Le Fèvre</name>
<name sortKey="Malterre, Daniel" sort="Malterre, Daniel" uniqKey="Malterre D" first="Daniel" last="Malterre">Daniel Malterre</name>
<name sortKey="Moreau, Luc" sort="Moreau, Luc" uniqKey="Moreau L" first="Luc" last="Moreau">Luc Moreau</name>
<name sortKey="Sicot, Muriel" sort="Sicot, Muriel" uniqKey="Sicot M" first="Muriel" last="Sicot">Muriel Sicot</name>
</country>
<country name="Canada"><noRegion><name sortKey="Cardenas, Luis" sort="Cardenas, Luis" uniqKey="Cardenas L" first="Luis" last="Cardenas">Luis Cardenas</name>
</noRegion>
<name sortKey="Galeotti, Gianluca" sort="Galeotti, Gianluca" uniqKey="Galeotti G" first="Gianluca" last="Galeotti">Gianluca Galeotti</name>
<name sortKey="Lipton Duffin, Josh" sort="Lipton Duffin, Josh" uniqKey="Lipton Duffin J" first="Josh" last="Lipton-Duffin">Josh Lipton-Duffin</name>
<name sortKey="Perepichka, Dmitrii F" sort="Perepichka, Dmitrii F" uniqKey="Perepichka D" first="Dmitrii F." last="Perepichka">Dmitrii F. Perepichka</name>
<name sortKey="Rosei, Federico" sort="Rosei, Federico" uniqKey="Rosei F" first="Federico" last="Rosei">Federico Rosei</name>
</country>
<country name="Australie"><noRegion><name sortKey="Lipton Duffin, Josh" sort="Lipton Duffin, Josh" uniqKey="Lipton Duffin J" first="Josh" last="Lipton-Duffin">Josh Lipton-Duffin</name>
</noRegion>
</country>
<country name="République populaire de Chine"><noRegion><name sortKey="Rosei, Federico" sort="Rosei, Federico" uniqKey="Rosei F" first="Federico" last="Rosei">Federico Rosei</name>
</noRegion>
</country>
<country name="Italie"><noRegion><name sortKey="Di Giovannantonio, Marco" sort="Di Giovannantonio, Marco" uniqKey="Di Giovannantonio M" first="Marco" last="Di Giovannantonio">Marco Di Giovannantonio</name>
</noRegion>
<name sortKey="Contini, Giorgio" sort="Contini, Giorgio" uniqKey="Contini G" first="Giorgio" last="Contini">Giorgio Contini</name>
<name sortKey="Contini, Giorgio" sort="Contini, Giorgio" uniqKey="Contini G" first="Giorgio" last="Contini">Giorgio Contini</name>
</country>
<country name="États-Unis"><noRegion><name sortKey="Liang, Liangbo" sort="Liang, Liangbo" uniqKey="Liang L" first="Liangbo" last="Liang">Liangbo Liang</name>
</noRegion>
<name sortKey="Liang, Liangbo" sort="Liang, Liangbo" uniqKey="Liang L" first="Liangbo" last="Liang">Liangbo Liang</name>
<name sortKey="Meunier, Vincent" sort="Meunier, Vincent" uniqKey="Meunier V" first="Vincent" last="Meunier">Vincent Meunier</name>
</country>
</tree>
</affiliations>
</record>
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