Population redistribution in optically trapped polar molecules
Identifieur interne : 006C29 ( Main/Merge ); précédent : 006C28; suivant : 006C30Population redistribution in optically trapped polar molecules
Auteurs : J. Deiglmayr [Allemagne] ; M. Repp [Allemagne] ; O. Dulieu [France] ; R. Wester [Australie] ; M. Weidemüller [Allemagne]Source :
- The European physical journal. D, Atomic, molecular and optical physics : (Print) [ 1434-6060 ] ; 2011.
Descripteurs français
- Pascal (Inist)
- Piégeage optique, Emission spontanée, Photoassociation, Etude théorique, Calcul ab initio, Courbe potentiel, Etat fondamental, Etat rotationnel, Moment dipolaire électrique, Molécule polaire, Molécule ultrafroide, Rayonnement corps noir, Etude comparative, Collision atome atome, Collision sous rayonnement, 3450R, 3380P, 3115A.
English descriptors
- KwdEn :
- Ab initio calculations, Atom-atom collisions, Blackbody radiation, Comparative study, Electric dipole moments, Ground states, Optical trapping, Photoassociation, Polar molecule, Potential energy curve, Radiation assisted collision, Rotational states, Spontaneous emission, Theoretical study, Ultracold molecules.
Abstract
We investigate the rovibrational population redistribution of polar molecules in the electronic ground state induced by spontaneous emission and blackbody radiation. As a model system we use optically trapped LiCs molecules formed by photoassociation in an ultracold two-species gas. The population dynamics of vibrational and rotational states is modeled using an ab initio electric dipole moment function and experimental potential energy curves. Comparison with the evolution of the v" = 3 electronic ground state yields good qualitative agreement. The analysis provides important input to assess applications of ultracold LiCs molecules in quantum simulation and ultracold chemistry.
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Pascal:12-0019049Le document en format XML
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<term>Optical trapping</term>
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<term>Calcul ab initio</term>
<term>Courbe potentiel</term>
<term>Etat fondamental</term>
<term>Etat rotationnel</term>
<term>Moment dipolaire électrique</term>
<term>Molécule polaire</term>
<term>Molécule ultrafroide</term>
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<term>Etude comparative</term>
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<front><div type="abstract" xml:lang="en">We investigate the rovibrational population redistribution of polar molecules in the electronic ground state induced by spontaneous emission and blackbody radiation. As a model system we use optically trapped LiCs molecules formed by photoassociation in an ultracold two-species gas. The population dynamics of vibrational and rotational states is modeled using an ab initio electric dipole moment function and experimental potential energy curves. Comparison with the evolution of the v" = 3 electronic ground state yields good qualitative agreement. The analysis provides important input to assess applications of ultracold LiCs molecules in quantum simulation and ultracold chemistry.</div>
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