Coriolis effects on “intermediate case” of intramolecular vibrational relaxation: Rotational-temperature dependence of energy- resolved fluorescence from jet-cooled perylene with 776–975 cm−1 excess energies
Identifieur interne : 004235 ( Main/Merge ); précédent : 004234; suivant : 004236Coriolis effects on “intermediate case” of intramolecular vibrational relaxation: Rotational-temperature dependence of energy- resolved fluorescence from jet-cooled perylene with 776–975 cm−1 excess energies
Auteurs : B. E. Forch [États-Unis] ; K. T. Chen [États-Unis] ; E. C. Lim [États-Unis]Source :
- Chemical Physics Letters [ 0009-2614 ] ; 1983.
Abstract
The rotational-temperature dependence of the energy-resolved fluorescence, combined with the calculated level density, indicates that the large variations in the rate of the intramolecular vibrational relaxation over a small excess energy in S1 perylene is due to the fluctuations in the density of accessible vibrational levels, resulting from the vibrational selection rules for second-order Coriolis coupling.
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DOI: 10.1016/0009-2614(83)87335-7
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