ThuliumV1, PubMed, Corpus, bibRecord, 000404

Fluorescence enhancement of rare earth Tb(III) by Tm(III) in benzyl benzoylmethyl sulphoxide complexes.

Identifieur interne : 000404 ( PubMed/Corpus ); précédent : 000403; suivant : 000405

Fluorescence enhancement of rare earth Tb(III) by Tm(III) in benzyl benzoylmethyl sulphoxide complexes.

Auteurs : Wen-Xian Li ; Wen-Juan Chai ; Yu Liu ; Ying-Jie Li ; Tie Ren ; Jing Zhang ; Bo-Yang Ao

Source :

Luminescence : the journal of biological and chemical luminescence [ 1522-7243 ]

RBID : pubmed:22114050

English descriptors

KwdEn :
- Fluorescence, Fluorescent Dyes (chemical synthesis), Fluorescent Dyes (chemistry), Spectrometry, Fluorescence, Sulfoxides (chemistry), Terbium (chemistry), Thulium (chemistry).
MESH :
- chemical , chemical synthesis : Fluorescent Dyes.
- chemical , chemistry : Fluorescent Dyes, Sulfoxides, Terbium, Thulium.
- Fluorescence, Spectrometry, Fluorescence.

Abstract

A series of rare earth complexes [(Tb(x) Tm(y))L5 (ClO4)2](ClO4)·3H(2) O (x:y = 1.000:0.000, 0.999:0.001, 0.995:0.005, 0.990:0.010, 0.950:0.050, 0.900:0.100, 0.800:0.200, 0.700:0.300; L = C(6) H5 CH2 SOCH2 COC6 H5) (Tb(III) luminescence ion; Tm(III) doped inert ion) were synthesized and characterized by elemental analysis, infrared spectra (IR) and (1) H-NMR. The photophysical properties of these complexes were studied in detail using ultraviolet absorption spectra, fluorescent spectra and lifetimes. The fluorescence spectra of complexes indicated that the fluorescence emission intensity was significantly enhanced by Tm(III). The complexes showed the best luminescence properties when the mole ratio Tb(III):Tm(III) was 0.990:0.010. The fluorescence intensity could be increased to 390%. Additionally, phosphorescence spectra and the luminescence mechanisms are discussed.

DOI: 10.1002/bio.1368
PubMed: 22114050

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pubmed:22114050

Le document en format XML

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<author><name sortKey="Li, Wen Xian" sort="Li, Wen Xian" uniqKey="Li W" first="Wen-Xian" last="Li">Wen-Xian Li</name>
<affiliation><nlm:affiliation>College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot, 010021, People's Republic of China.</nlm:affiliation>
</affiliation>
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<author><name sortKey="Chai, Wen Juan" sort="Chai, Wen Juan" uniqKey="Chai W" first="Wen-Juan" last="Chai">Wen-Juan Chai</name>
</author>
<author><name sortKey="Liu, Yu" sort="Liu, Yu" uniqKey="Liu Y" first="Yu" last="Liu">Yu Liu</name>
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<author><name sortKey="Li, Ying Jie" sort="Li, Ying Jie" uniqKey="Li Y" first="Ying-Jie" last="Li">Ying-Jie Li</name>
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<author><name sortKey="Ren, Tie" sort="Ren, Tie" uniqKey="Ren T" first="Tie" last="Ren">Tie Ren</name>
</author>
<author><name sortKey="Zhang, Jing" sort="Zhang, Jing" uniqKey="Zhang J" first="Jing" last="Zhang">Jing Zhang</name>
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<author><name sortKey="Ao, Bo Yang" sort="Ao, Bo Yang" uniqKey="Ao B" first="Bo-Yang" last="Ao">Bo-Yang Ao</name>
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<author><name sortKey="Li, Wen Xian" sort="Li, Wen Xian" uniqKey="Li W" first="Wen-Xian" last="Li">Wen-Xian Li</name>
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<author><name sortKey="Zhang, Jing" sort="Zhang, Jing" uniqKey="Zhang J" first="Jing" last="Zhang">Jing Zhang</name>
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<front><div type="abstract" xml:lang="en">A series of rare earth complexes [(Tb(x) Tm(y))L5 (ClO4)2](ClO4)·3H(2) O (x:y = 1.000:0.000, 0.999:0.001, 0.995:0.005, 0.990:0.010, 0.950:0.050, 0.900:0.100, 0.800:0.200, 0.700:0.300; L = C(6) H5 CH2 SOCH2 COC6 H5) (Tb(III) luminescence ion; Tm(III) doped inert ion) were synthesized and characterized by elemental analysis, infrared spectra (IR) and (1) H-NMR. The photophysical properties of these complexes were studied in detail using ultraviolet absorption spectra, fluorescent spectra and lifetimes. The fluorescence spectra of complexes indicated that the fluorescence emission intensity was significantly enhanced by Tm(III). The complexes showed the best luminescence properties when the mole ratio Tb(III):Tm(III) was 0.990:0.010. The fluorescence intensity could be increased to 390%. Additionally, phosphorescence spectra and the luminescence mechanisms are discussed.</div>
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<Abstract><AbstractText>A series of rare earth complexes [(Tb(x) Tm(y))L5 (ClO4)2](ClO4)·3H(2) O (x:y = 1.000:0.000, 0.999:0.001, 0.995:0.005, 0.990:0.010, 0.950:0.050, 0.900:0.100, 0.800:0.200, 0.700:0.300; L = C(6) H5 CH2 SOCH2 COC6 H5) (Tb(III) luminescence ion; Tm(III) doped inert ion) were synthesized and characterized by elemental analysis, infrared spectra (IR) and (1) H-NMR. The photophysical properties of these complexes were studied in detail using ultraviolet absorption spectra, fluorescent spectra and lifetimes. The fluorescence spectra of complexes indicated that the fluorescence emission intensity was significantly enhanced by Tm(III). The complexes showed the best luminescence properties when the mole ratio Tb(III):Tm(III) was 0.990:0.010. The fluorescence intensity could be increased to 390%. Additionally, phosphorescence spectra and the luminescence mechanisms are discussed.</AbstractText>
<CopyrightInformation>Copyright © 2011 John Wiley & Sons, Ltd.</CopyrightInformation>
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Fluorescence enhancement of rare earth Tb(III) by Tm(III) in benzyl benzoylmethyl sulphoxide complexes.

Fluorescence enhancement of rare earth Tb(III) by Tm(III) in benzyl benzoylmethyl sulphoxide complexes.

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English descriptors

Abstract

Links to Exploration step

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