Codopant ion-induced tunable upconversion emission in β-NaYF4:Yb3+/Tm3+ nanorods.
Identifieur interne : 000327 ( PubMed/Corpus ); précédent : 000326; suivant : 000328Codopant ion-induced tunable upconversion emission in β-NaYF4:Yb3+/Tm3+ nanorods.
Auteurs : Dangli Gao ; Xiangyu Zhang ; Hairong Zheng ; Peng Shi ; Long Li ; Yawen LingSource :
- Dalton transactions (Cambridge, England : 2003) [ 1477-9234 ] ; 2013.
English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Fluorides, Ions, Thulium, Ytterbium, Yttrium.
- chemistry : Nanotubes.
- Spectroscopy, Fourier Transform Infrared, Temperature.
Abstract
An innovative route to tune upconversion (UC) emission in β-NaYF(4):Yb(3+)/Tm(3+) nanorods through codoping a third rare-earth ion upon continuous wave excitation near 976 nm is reported. The dependence of UC emission on codopant concentration and environment temperature shows that tailored local environment and readjustable depopulation of excited-state ions are responsible for the tuning of UC luminescence. Codopant ions introduce a new distribution of active ions and a modified distance between Tm(3+) and Yb(3+) ions, making UC systems more sensitive to impurity ions than downconversion systems.
DOI: 10.1039/c2dt31814h
PubMed: 23165284
Links to Exploration step
pubmed:23165284Le document en format XML
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<author><name sortKey="Zhang, Xiangyu" sort="Zhang, Xiangyu" uniqKey="Zhang X" first="Xiangyu" last="Zhang">Xiangyu Zhang</name>
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<author><name sortKey="Zheng, Hairong" sort="Zheng, Hairong" uniqKey="Zheng H" first="Hairong" last="Zheng">Hairong Zheng</name>
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<author><name sortKey="Shi, Peng" sort="Shi, Peng" uniqKey="Shi P" first="Peng" last="Shi">Peng Shi</name>
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<author><name sortKey="Li, Long" sort="Li, Long" uniqKey="Li L" first="Long" last="Li">Long Li</name>
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<front><div type="abstract" xml:lang="en">An innovative route to tune upconversion (UC) emission in β-NaYF(4):Yb(3+)/Tm(3+) nanorods through codoping a third rare-earth ion upon continuous wave excitation near 976 nm is reported. The dependence of UC emission on codopant concentration and environment temperature shows that tailored local environment and readjustable depopulation of excited-state ions are responsible for the tuning of UC luminescence. Codopant ions introduce a new distribution of active ions and a modified distance between Tm(3+) and Yb(3+) ions, making UC systems more sensitive to impurity ions than downconversion systems.</div>
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<Abstract><AbstractText>An innovative route to tune upconversion (UC) emission in β-NaYF(4):Yb(3+)/Tm(3+) nanorods through codoping a third rare-earth ion upon continuous wave excitation near 976 nm is reported. The dependence of UC emission on codopant concentration and environment temperature shows that tailored local environment and readjustable depopulation of excited-state ions are responsible for the tuning of UC luminescence. Codopant ions introduce a new distribution of active ions and a modified distance between Tm(3+) and Yb(3+) ions, making UC systems more sensitive to impurity ions than downconversion systems.</AbstractText>
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