Nd3+ sensitized up/down converting dual-mode nanomaterials for efficient in-vitro and in-vivo bioimaging excited at 800 nm.
Identifieur interne : 000263 ( PubMed/Checkpoint ); précédent : 000262; suivant : 000264Nd3+ sensitized up/down converting dual-mode nanomaterials for efficient in-vitro and in-vivo bioimaging excited at 800 nm.
Auteurs : Xiaomin Li [République populaire de Chine] ; Rui Wang [République populaire de Chine] ; Fan Zhang [République populaire de Chine] ; Lei Zhou [République populaire de Chine] ; Dengke Shen [République populaire de Chine] ; Chi Yao [République populaire de Chine] ; Dongyuan Zhao [République populaire de Chine]Source :
- Scientific reports [ 2045-2322 ] ; 2013.
Descripteurs français
- KwdFr :
- MESH :
English descriptors
- KwdEn :
- Animals, Chlorides (chemistry), Diagnostic Imaging (instrumentation), Diagnostic Imaging (methods), Erbium (chemistry), Fluorescence, Fluorescent Dyes (chemistry), Gadolinium (chemistry), Lanthanoid Series Elements (chemistry), Mice, Nanoparticles (chemistry), Neodymium (chemistry), Sodium (chemistry), Thulium (chemistry), Ytterbium (chemistry).
- MESH :
- chemical , chemistry : Chlorides, Erbium, Fluorescent Dyes, Gadolinium, Lanthanoid Series Elements, Neodymium, Sodium, Thulium, Ytterbium.
- chemistry : Nanoparticles.
- instrumentation : Diagnostic Imaging.
- methods : Diagnostic Imaging.
- Animals, Fluorescence, Mice.
Abstract
Core/shell1/shell2/shell3 structured NaGdF4:Nd/NaYF4/NaGdF4:Nd,Yb,Er/NaYF4 nanocrystals were well designed and synthesized, each of the parts assume respective role and work together to achieve dual-mode upconverting (UC) and downconverting (DC) luminescence upon the low heat effect 800-nm excitation. Nd(3+), Yb(3+), Er(3+) tri-doped NaGdF4:Nd,Yb,Er UC layer [NIR (800 nm)-to-Visible (540 nm)] with a constitutional efficient 800 nm excitable property were achieved for the in-vitro bioimaging with low auto-fluorescence and photo-damage effects. Moreover, typical NIR (800 nm)-to-NIR (860-895 nm) DC luminescence of Nd(3+) has also been realized with this designed nanostructure. Due to the low heat effect, high penetration depth of the excitation and the high efficiency of the DC luminescence, the in-vivo high contrast DC imaging of a whole body nude mouse was achieved. We believe that such dual-mode luminescence NCs will open the door to engineering the excitation and emission wavelengths of NCs and will provide a new tool for a wide variety of applications in the fields of bioanalysis and biomedical.
DOI: 10.1038/srep03536
PubMed: 24346622
Affiliations:
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pubmed:24346622Le document en format XML
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<front><div type="abstract" xml:lang="en">Core/shell1/shell2/shell3 structured NaGdF4:Nd/NaYF4/NaGdF4:Nd,Yb,Er/NaYF4 nanocrystals were well designed and synthesized, each of the parts assume respective role and work together to achieve dual-mode upconverting (UC) and downconverting (DC) luminescence upon the low heat effect 800-nm excitation. Nd(3+), Yb(3+), Er(3+) tri-doped NaGdF4:Nd,Yb,Er UC layer [NIR (800 nm)-to-Visible (540 nm)] with a constitutional efficient 800 nm excitable property were achieved for the in-vitro bioimaging with low auto-fluorescence and photo-damage effects. Moreover, typical NIR (800 nm)-to-NIR (860-895 nm) DC luminescence of Nd(3+) has also been realized with this designed nanostructure. Due to the low heat effect, high penetration depth of the excitation and the high efficiency of the DC luminescence, the in-vivo high contrast DC imaging of a whole body nude mouse was achieved. We believe that such dual-mode luminescence NCs will open the door to engineering the excitation and emission wavelengths of NCs and will provide a new tool for a wide variety of applications in the fields of bioanalysis and biomedical.</div>
</front>
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<Abstract><AbstractText>Core/shell1/shell2/shell3 structured NaGdF4:Nd/NaYF4/NaGdF4:Nd,Yb,Er/NaYF4 nanocrystals were well designed and synthesized, each of the parts assume respective role and work together to achieve dual-mode upconverting (UC) and downconverting (DC) luminescence upon the low heat effect 800-nm excitation. Nd(3+), Yb(3+), Er(3+) tri-doped NaGdF4:Nd,Yb,Er UC layer [NIR (800 nm)-to-Visible (540 nm)] with a constitutional efficient 800 nm excitable property were achieved for the in-vitro bioimaging with low auto-fluorescence and photo-damage effects. Moreover, typical NIR (800 nm)-to-NIR (860-895 nm) DC luminescence of Nd(3+) has also been realized with this designed nanostructure. Due to the low heat effect, high penetration depth of the excitation and the high efficiency of the DC luminescence, the in-vivo high contrast DC imaging of a whole body nude mouse was achieved. We believe that such dual-mode luminescence NCs will open the door to engineering the excitation and emission wavelengths of NCs and will provide a new tool for a wide variety of applications in the fields of bioanalysis and biomedical.</AbstractText>
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