ThuliumV1, Pascal, Curation, bibRecord, 001880

Frequency upconversion and its new mechanism in Tm3+-doped fluoroaluminate glasses

Identifieur interne : 001880 ( Pascal/Curation ); précédent : 001879; suivant : 001881

Frequency upconversion and its new mechanism in Tm3+-doped fluoroaluminate glasses

Auteurs : K. Hirao [Japon] ; K. Tamai [Japon] ; S. Tanabe ; N. Soga [Japon]

Source :

Journal of non-crystalline solids [ 0022-3093 ] ; 1993.

RBID : Pascal:93-0664431

Descripteurs français

Pascal (Inist)
- Fluorescence, Conversion fréquence, Pompage optique, Faisceau laser, Absorption 2 photons, Transition optique, Etat excité, Transfert énergie, Relaxation croisée, Etat amorphe, Verre, Composition chimique, Niveau énergie, Spectre excitation, Transition radiative, Effet Judd Ofelt, Etude expérimentale, Composé minéral, Fluorure, Système aluminium baryum calcium fluor thulium yttrium, Upconverssion.
Wicri :
- topic : Verre, Composé minéral.

English descriptors

KwdEn :
- Amorphous state, Chemical composition, Cross relaxation, Energy level, Energy transfer, Excitation spectrum, Excited state, Experimental study, Fluorescence, Fluorides, Frequency conversion, Glass, Inorganic compound, Judd Ofelt effect, Laser beam, Optical pumping, Optical transition, Radiative transition, Two photon absorption.

Abstract

Upconversion fluorescences have been observed in the UV (363 nm) and the blue region (451 and 476 nm) in Tm³⁺-doped fluoroaluminate glass by pumping with a DCM dye laser. The two-photon absorption process of upconversion fluorescences was confirmed by the quadratic dependence of the emission intensity on incident pumping power. The excitation spectra for upconversion fluorescences show that the mechanism of upconversion is a simple ESA (excited state absorption) process. In addition to ESA, it was found that the energy transfer by cross-relaxation (³H₄, ³H₆→³F₄, ³F₄) is also involved in the mechanism of the 476 nm blue upconversion fluorescence which differs from that of the UV and the 451 nm blue upconversion fluorescence

A01	`01`	`1`		`@0 0022-3093`
A02	`01`			`@0 JNCSBJ`
A03		`1`		`@0 J. non-cryst. solids`
A05				`@2 160`
A06				`@2 3`
A08	`01`	`1`	`ENG`	`@1 Frequency upconversion and its new mechanism in Tm³⁺-doped fluoroaluminate glasses`
A11	`01`	`1`		`@1 HIRAO (K.)`
A11	`02`	`1`		`@1 TAMAI (K.)`
A11	`03`	`1`		`@1 TANABE (S.)`
A11	`04`	`1`		`@1 SOGA (N.)`
A14	`01`			`@1 Kyoto univ., fac. eng., dep. industrial chemistry @2 Sakyo-ku, Kyoto 606-01 @3 JPN @Z 1 aut. @Z 2 aut. @Z 4 aut.`
A20				`@1 261-267`
A21				`@1 1993`
A23	`01`			`@0 ENG`
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A61				`@0 A`
A64		`1`		`@0 Journal of non-crystalline solids`
A66	`01`			`@0 NLD`
C01	`01`		`ENG`	@0 Upconversion fluorescences have been observed in the UV (363 nm) and the blue region (451 and 476 nm) in Tm³⁺-doped fluoroaluminate glass by pumping with a DCM dye laser. The two-photon absorption process of upconversion fluorescences was confirmed by the quadratic dependence of the emission intensity on incident pumping power. The excitation spectra for upconversion fluorescences show that the mechanism of upconversion is a simple ESA (excited state absorption) process. In addition to ESA, it was found that the energy transfer by cross-relaxation (³H₄, ³H₆→³F₄, ³F₄) is also involved in the mechanism of the 476 nm blue upconversion fluorescence which differs from that of the UV and the 451 nm blue upconversion fluorescence
C02	`01`	`X`		`@0 001B11H08`
C03	`01`	`X`	`FRE`	`@0 Fluorescence @5 01`
C03	`01`	`X`	`ENG`	`@0 Fluorescence @5 01`
C03	`01`	`X`	`GER`	`@0 Fluoreszenz @5 01`
C03	`01`	`X`	`SPA`	`@0 Fluorescencia @5 01`
C03	`02`	`X`	`FRE`	`@0 Conversion fréquence @5 02`
C03	`02`	`X`	`ENG`	`@0 Frequency conversion @5 02`
C03	`02`	`X`	`SPA`	`@0 Conversión frecuencia @5 02`
C03	`03`	`X`	`FRE`	`@0 Pompage optique @5 03`
C03	`03`	`X`	`ENG`	`@0 Optical pumping @5 03`
C03	`03`	`X`	`SPA`	`@0 Bombeo óptico @5 03`
C03	`04`	`X`	`FRE`	`@0 Faisceau laser @5 04`
C03	`04`	`X`	`ENG`	`@0 Laser beam @5 04`
C03	`04`	`X`	`GER`	`@0 Laserstrahl @5 04`
C03	`04`	`X`	`SPA`	`@0 Haz láser @5 04`
C03	`05`	`X`	`FRE`	`@0 Absorption 2 photons @5 05`
C03	`05`	`X`	`ENG`	`@0 Two photon absorption @5 05`
C03	`05`	`X`	`SPA`	`@0 Absorción 2 fotones @5 05`
C03	`06`	`X`	`FRE`	`@0 Transition optique @5 06`
C03	`06`	`X`	`ENG`	`@0 Optical transition @5 06`
C03	`06`	`X`	`GER`	`@0 Optischer Uebergang @5 06`
C03	`06`	`X`	`SPA`	`@0 Transición óptica @5 06`
C03	`07`	`X`	`FRE`	`@0 Etat excité @5 07`
C03	`07`	`X`	`ENG`	`@0 Excited state @5 07`
C03	`07`	`X`	`SPA`	`@0 Estado excitado @5 07`
C03	`08`	`X`	`FRE`	`@0 Transfert énergie @5 08`
C03	`08`	`X`	`ENG`	`@0 Energy transfer @5 08`
C03	`08`	`X`	`SPA`	`@0 Transferencia energía @5 08`
C03	`09`	`X`	`FRE`	`@0 Relaxation croisée @5 09`
C03	`09`	`X`	`ENG`	`@0 Cross relaxation @5 09`
C03	`09`	`X`	`SPA`	`@0 Relajación cruzada @5 09`
C03	`10`	`X`	`FRE`	`@0 Etat amorphe @5 10`
C03	`10`	`X`	`ENG`	`@0 Amorphous state @5 10`
C03	`10`	`X`	`GER`	`@0 Amorpher Zustand @5 10`
C03	`10`	`X`	`SPA`	`@0 Estado amorfo @5 10`
C03	`11`	`X`	`FRE`	`@0 Verre @5 11`
C03	`11`	`X`	`ENG`	`@0 Glass @5 11`
C03	`11`	`X`	`GER`	`@0 Glas @5 11`
C03	`11`	`X`	`SPA`	`@0 Vidrio @5 11`
C03	`12`	`X`	`FRE`	`@0 Composition chimique @5 12`
C03	`12`	`X`	`ENG`	`@0 Chemical composition @5 12`
C03	`12`	`X`	`GER`	`@0 Chemische Zusammensetzung @5 12`
C03	`12`	`X`	`SPA`	`@0 Composición química @5 12`
C03	`13`	`X`	`FRE`	`@0 Niveau énergie @5 13`
C03	`13`	`X`	`ENG`	`@0 Energy level @5 13`
C03	`13`	`X`	`GER`	`@0 Energieniveau @5 13`
C03	`13`	`X`	`SPA`	`@0 Nivel energía @5 13`
C03	`14`	`X`	`FRE`	`@0 Spectre excitation @5 14`
C03	`14`	`X`	`ENG`	`@0 Excitation spectrum @5 14`
C03	`14`	`X`	`SPA`	`@0 Espectro excitación @5 14`
C03	`15`	`X`	`FRE`	`@0 Transition radiative @5 15`
C03	`15`	`X`	`ENG`	`@0 Radiative transition @5 15`
C03	`15`	`X`	`SPA`	`@0 Transición radiativa @5 15`
C03	`16`	`X`	`FRE`	`@0 Effet Judd Ofelt @5 16`
C03	`16`	`X`	`ENG`	`@0 Judd Ofelt effect @5 16`
C03	`16`	`X`	`SPA`	`@0 Efecto Judd Ofelt @5 16`
C03	`17`	`X`	`FRE`	`@0 Etude expérimentale @5 17`
C03	`17`	`X`	`ENG`	`@0 Experimental study @5 17`
C03	`17`	`X`	`GER`	`@0 Experimentelle Untersuchung @5 17`
C03	`17`	`X`	`SPA`	`@0 Estudio experimental @5 17`
C03	`18`	`X`	`FRE`	`@0 Composé minéral @5 18`
C03	`18`	`X`	`ENG`	`@0 Inorganic compound @5 18`
C03	`18`	`X`	`SPA`	`@0 Compuesto inorgánico @5 18`
C03	`19`	`X`	`FRE`	`@0 Fluorure @2 NA @2 FX @5 19`
C03	`19`	`X`	`ENG`	`@0 Fluorides @2 NA @2 FX @5 19`
C03	`19`	`X`	`GER`	`@0 Fluorid @2 NA @2 FX @5 19`
C03	`19`	`X`	`SPA`	`@0 Fluoruro @2 NA @2 FX @5 19`
C03	`20`	`X`	`FRE`	`@0 Système aluminium baryum calcium fluor thulium yttrium @2 NK @4 INC @5 92`
C03	`21`	`X`	`FRE`	`@0 Upconverssion @4 INC @5 93`
N21				`@1 333`

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Le document en format XML

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<series><title level="j" type="main">Journal of non-crystalline solids</title>
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<front><div type="abstract" xml:lang="en">Upconversion fluorescences have been observed in the UV (363 nm) and the blue region (451 and 476 nm) in Tm<sup>3+</sup>
-doped fluoroaluminate glass by pumping with a DCM dye laser. The two-photon absorption process of upconversion fluorescences was confirmed by the quadratic dependence of the emission intensity on incident pumping power. The excitation spectra for upconversion fluorescences show that the mechanism of upconversion is a simple ESA (excited state absorption) process. In addition to ESA, it was found that the energy transfer by cross-relaxation (<sup>3</sup>
H<sub>4</sub>
, <sup>3</sup>
H<sub>6</sub>
→<sup>3</sup>
F<sub>4</sub>
, <sup>3</sup>
F<sub>4</sub>
) is also involved in the mechanism of the 476 nm blue upconversion fluorescence which differs from that of the UV and the 451 nm blue upconversion fluorescence</div>
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<fC01 i1="01" l="ENG"><s0>Upconversion fluorescences have been observed in the UV (363 nm) and the blue region (451 and 476 nm) in Tm<sup>3+</sup>
-doped fluoroaluminate glass by pumping with a DCM dye laser. The two-photon absorption process of upconversion fluorescences was confirmed by the quadratic dependence of the emission intensity on incident pumping power. The excitation spectra for upconversion fluorescences show that the mechanism of upconversion is a simple ESA (excited state absorption) process. In addition to ESA, it was found that the energy transfer by cross-relaxation (<sup>3</sup>
H<sub>4</sub>
, <sup>3</sup>
H<sub>6</sub>
→<sup>3</sup>
F<sub>4</sub>
, <sup>3</sup>
F<sub>4</sub>
) is also involved in the mechanism of the 476 nm blue upconversion fluorescence which differs from that of the UV and the 451 nm blue upconversion fluorescence</s0>
</fC01>
<fC02 i1="01" i2="X"><s0>001B11H08</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Fluorescence</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Fluorescence</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="GER"><s0>Fluoreszenz</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Fluorescencia</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE"><s0>Conversion fréquence</s0>
<s5>02</s5>
</fC03>
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<s5>02</s5>
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<s5>02</s5>
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<fC03 i1="03" i2="X" l="FRE"><s0>Pompage optique</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Optical pumping</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA"><s0>Bombeo óptico</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="X" l="FRE"><s0>Faisceau laser</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="ENG"><s0>Laser beam</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="GER"><s0>Laserstrahl</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="X" l="SPA"><s0>Haz láser</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="X" l="FRE"><s0>Absorption 2 photons</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="ENG"><s0>Two photon absorption</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="X" l="SPA"><s0>Absorción 2 fotones</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="X" l="FRE"><s0>Transition optique</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="ENG"><s0>Optical transition</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="GER"><s0>Optischer Uebergang</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="X" l="SPA"><s0>Transición óptica</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="X" l="FRE"><s0>Etat excité</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="ENG"><s0>Excited state</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="X" l="SPA"><s0>Estado excitado</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="X" l="FRE"><s0>Transfert énergie</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="ENG"><s0>Energy transfer</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="X" l="SPA"><s0>Transferencia energía</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Relaxation croisée</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Cross relaxation</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Relajación cruzada</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="X" l="FRE"><s0>Etat amorphe</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="ENG"><s0>Amorphous state</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="GER"><s0>Amorpher Zustand</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="X" l="SPA"><s0>Estado amorfo</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Verre</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Glass</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="GER"><s0>Glas</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Vidrio</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="X" l="FRE"><s0>Composition chimique</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="ENG"><s0>Chemical composition</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="GER"><s0>Chemische Zusammensetzung</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="X" l="SPA"><s0>Composición química</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Niveau énergie</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Energy level</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="GER"><s0>Energieniveau</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Nivel energía</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="X" l="FRE"><s0>Spectre excitation</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="ENG"><s0>Excitation spectrum</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="X" l="SPA"><s0>Espectro excitación</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="X" l="FRE"><s0>Transition radiative</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="ENG"><s0>Radiative transition</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="X" l="SPA"><s0>Transición radiativa</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Effet Judd Ofelt</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Judd Ofelt effect</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Efecto Judd Ofelt</s0>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Etude expérimentale</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Experimental study</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="GER"><s0>Experimentelle Untersuchung</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Estudio experimental</s0>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>Composé minéral</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="ENG"><s0>Inorganic compound</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="SPA"><s0>Compuesto inorgánico</s0>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Fluorure</s0>
<s2>NA</s2>
<s2>FX</s2>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="ENG"><s0>Fluorides</s0>
<s2>NA</s2>
<s2>FX</s2>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="GER"><s0>Fluorid</s0>
<s2>NA</s2>
<s2>FX</s2>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="SPA"><s0>Fluoruro</s0>
<s2>NA</s2>
<s2>FX</s2>
<s5>19</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Système aluminium baryum calcium fluor thulium yttrium</s0>
<s2>NK</s2>
<s4>INC</s4>
<s5>92</s5>
</fC03>
<fC03 i1="21" i2="X" l="FRE"><s0>Upconverssion</s0>
<s4>INC</s4>
<s5>93</s5>
</fC03>
<fN21><s1>333</s1>
</fN21>
</pA>
</standard>
</inist>
</record>

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Frequency upconversion and its new mechanism in Tm3+-doped fluoroaluminate glasses

Frequency upconversion and its new mechanism in Tm3+-doped fluoroaluminate glasses

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