ThuliumV1, Pascal, Curation, bibRecord, 000D96

Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium

Identifieur interne : 000D96 ( Pascal/Curation ); précédent : 000D95; suivant : 000D97

Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium

Auteurs : W. Ryba-Romanowski [Pologne] ; S. Golłab [Pologne] ; G. Dominiak-Dzik [Pologne] ; M. Zelechower [Pologne] ; J. Gabrys-Pisarska [Pologne]

Source :

Journal of alloys and compounds [ 0925-8388 ] ; 2001.

RBID : Pascal:01-0352918

Descripteurs français

Pascal (Inist)
- Photoluminescence, Codopage, Dopage, Addition thulium, Addition terbium, Transfert énergie, Transfert radiatif, Etat impureté, Déclin luminescence, Transition niveau énergie, Extinction luminescence, Dipôle électrique, Interaction dipôle dipôle, Verre fluorure, Indium composé, Système multiple, Etude expérimentale, Système BaF2 GaF3 InF3 NaF SrF2 ZnF2, Ba F Ga In Na Sr Zn, 7855H, 7155J.
Wicri :
- topic : Dopage.

English descriptors

KwdEn :
- Codoping, Dipole dipole interaction, Doping, Electric dipoles, Energy transfer, Energy-level transitions, Experimental study, Fluoride glass, Impurity states, Indium compounds, Luminescence decay, Luminescence quenching, Multiple system, Photoluminescence, Radiative transfer, Terbium additions, Thulium additions.

Abstract

Effect of activator concentration on luminescence spectra and luminescence decay of excited states of Tm³⁺ in indium-based fluoride glass has been investigated. Self-quenching of luminescence originating in the ¹D₂, ¹G₄ and the ³H₄ levels is found to be significant at doping levels as low as 0.5%. Luminescence decay curves are consistent with the Inokuti-Hirayama model for the non-radiative energy transfer involving an electric dipole-electric dipole interaction. Critical distance R₀=12.3 Å, derived from an analysis of the ¹G₄ decay, is relatively high and indicates that the glass matrix favours the ion-ion interaction. Relaxation dynamics for glass samples doubly doped with thulium and terbium provides evidence that terbium ions are able to shorten the ³F₄ lifetime with extremely high efficiency. However, the Tm³⁺→Tb³⁺ energy transfer contributes adversely to relaxation of the ³H₄ level. Critical distance for this interaction is nearly the same as that for the self-quenching of Tm³⁺ luminescence.

A01	`01`	`1`		`@0 0925-8388`
A03		`1`		`@0 J. alloys compd.`
A05				`@2 325`
A06				`@2 1-2`
A08	`01`	`1`	`ENG`	`@1 Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium`
A11	`01`	`1`		`@1 RYBA-ROMANOWSKI (W.)`
A11	`02`	`1`		`@1 GOLŁAB (S.)`
A11	`03`	`1`		`@1 DOMINIAK-DZIK (G.)`
A11	`04`	`1`		`@1 ZELECHOWER (M.)`
A11	`05`	`1`		`@1 GABRYS-PISARSKA (J.)`
A14	`01`			`@1 Institute of Low Temperature and Structure Research, Polish Academy of Sciences, 2 Okolna Street @2 50-422 Wroclaw @3 POL @Z 1 aut. @Z 2 aut. @Z 3 aut.`
A14	`02`			`@1 Silesian University of Technology, Department of Materials Science, 8 Krasinskiego Street @2 40-019 Katowice @3 POL @Z 4 aut. @Z 5 aut.`
A20				`@1 215-222`
A21				`@1 2001`
A23	`01`			`@0 ENG`
A43	`01`			`@1 INIST @2 1151 @5 354000096660340340`
A44				`@0 0000 @1 © 2001 INIST-CNRS. All rights reserved.`
A45				`@0 19 ref.`
A47	`01`	`1`		`@0 01-0352918`
A60				`@1 P`
A61				`@0 A`
A64	`01`	`1`		`@0 Journal of alloys and compounds`
A66	`01`			`@0 CHE`
C01	`01`		`ENG`	@0 Effect of activator concentration on luminescence spectra and luminescence decay of excited states of Tm³⁺ in indium-based fluoride glass has been investigated. Self-quenching of luminescence originating in the ¹D₂, ¹G₄ and the ³H₄ levels is found to be significant at doping levels as low as 0.5%. Luminescence decay curves are consistent with the Inokuti-Hirayama model for the non-radiative energy transfer involving an electric dipole-electric dipole interaction. Critical distance R₀=12.3 Å, derived from an analysis of the ¹G₄ decay, is relatively high and indicates that the glass matrix favours the ion-ion interaction. Relaxation dynamics for glass samples doubly doped with thulium and terbium provides evidence that terbium ions are able to shorten the ³F₄ lifetime with extremely high efficiency. However, the Tm³⁺→Tb³⁺ energy transfer contributes adversely to relaxation of the ³H₄ level. Critical distance for this interaction is nearly the same as that for the self-quenching of Tm³⁺ luminescence.
C02	`01`	`3`		`@0 001B70H55H`
C02	`02`	`3`		`@0 001B70A55J`
C03	`01`	`3`	`FRE`	`@0 Photoluminescence @5 01`
C03	`01`	`3`	`ENG`	`@0 Photoluminescence @5 01`
C03	`02`	`X`	`FRE`	`@0 Codopage @5 02`
C03	`02`	`X`	`ENG`	`@0 Codoping @5 02`
C03	`02`	`X`	`SPA`	`@0 Codrogado @5 02`
C03	`03`	`X`	`FRE`	`@0 Dopage @5 03`
C03	`03`	`X`	`ENG`	`@0 Doping @5 03`
C03	`03`	`X`	`SPA`	`@0 Doping @5 03`
C03	`04`	`3`	`FRE`	`@0 Addition thulium @5 04`
C03	`04`	`3`	`ENG`	`@0 Thulium additions @5 04`
C03	`05`	`3`	`FRE`	`@0 Addition terbium @5 05`
C03	`05`	`3`	`ENG`	`@0 Terbium additions @5 05`
C03	`06`	`3`	`FRE`	`@0 Transfert énergie @5 06`
C03	`06`	`3`	`ENG`	`@0 Energy transfer @5 06`
C03	`07`	`3`	`FRE`	`@0 Transfert radiatif @5 07`
C03	`07`	`3`	`ENG`	`@0 Radiative transfer @5 07`
C03	`08`	`3`	`FRE`	`@0 Etat impureté @5 08`
C03	`08`	`3`	`ENG`	`@0 Impurity states @5 08`
C03	`09`	`X`	`FRE`	`@0 Déclin luminescence @5 09`
C03	`09`	`X`	`ENG`	`@0 Luminescence decay @5 09`
C03	`09`	`X`	`SPA`	`@0 Decadencia luminiscencia @5 09`
C03	`10`	`3`	`FRE`	`@0 Transition niveau énergie @5 10`
C03	`10`	`3`	`ENG`	`@0 Energy-level transitions @5 10`
C03	`11`	`X`	`FRE`	`@0 Extinction luminescence @5 11`
C03	`11`	`X`	`ENG`	`@0 Luminescence quenching @5 11`
C03	`11`	`X`	`SPA`	`@0 Extinción luminiscencia @5 11`
C03	`12`	`3`	`FRE`	`@0 Dipôle électrique @5 13`
C03	`12`	`3`	`ENG`	`@0 Electric dipoles @5 13`
C03	`13`	`X`	`FRE`	`@0 Interaction dipôle dipôle @5 14`
C03	`13`	`X`	`ENG`	`@0 Dipole dipole interaction @5 14`
C03	`13`	`X`	`SPA`	`@0 Interacción dipolo dipolo @5 14`
C03	`14`	`3`	`FRE`	`@0 Verre fluorure @5 15`
C03	`14`	`3`	`ENG`	`@0 Fluoride glass @5 15`
C03	`15`	`3`	`FRE`	`@0 Indium composé @5 16`
C03	`15`	`3`	`ENG`	`@0 Indium compounds @5 16`
C03	`16`	`X`	`FRE`	`@0 Système multiple @5 17`
C03	`16`	`X`	`ENG`	`@0 Multiple system @5 17`
C03	`16`	`X`	`SPA`	`@0 Sistema múltiple @5 17`
C03	`17`	`3`	`FRE`	`@0 Etude expérimentale @5 18`
C03	`17`	`3`	`ENG`	`@0 Experimental study @5 18`
C03	`18`	`3`	`FRE`	`@0 Système BaF2 GaF3 InF3 NaF SrF2 ZnF2 @4 INC @5 52`
C03	`19`	`3`	`FRE`	`@0 Ba F Ga In Na Sr Zn @4 INC @5 53`
C03	`20`	`3`	`FRE`	`@0 7855H @2 PAC @4 INC @5 56`
C03	`21`	`3`	`FRE`	`@0 7155J @2 PAC @4 INC @5 57`
N21				`@1 246`

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Le document en format XML

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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium</title>
<author><name sortKey="Ryba Romanowski, W" sort="Ryba Romanowski, W" uniqKey="Ryba Romanowski W" first="W." last="Ryba-Romanowski">W. Ryba-Romanowski</name>
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<author><name sortKey="Gollab, S" sort="Gollab, S" uniqKey="Gollab S" first="S." last="Golłab">S. Golłab</name>
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<author><name sortKey="Dominiak Dzik, G" sort="Dominiak Dzik, G" uniqKey="Dominiak Dzik G" first="G." last="Dominiak-Dzik">G. Dominiak-Dzik</name>
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<author><name sortKey="Gabrys Pisarska, J" sort="Gabrys Pisarska, J" uniqKey="Gabrys Pisarska J" first="J." last="Gabrys-Pisarska">J. Gabrys-Pisarska</name>
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<series><title level="j" type="main">Journal of alloys and compounds</title>
<title level="j" type="abbreviated">J. alloys compd.</title>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Codoping</term>
<term>Dipole dipole interaction</term>
<term>Doping</term>
<term>Electric dipoles</term>
<term>Energy transfer</term>
<term>Energy-level transitions</term>
<term>Experimental study</term>
<term>Fluoride glass</term>
<term>Impurity states</term>
<term>Indium compounds</term>
<term>Luminescence decay</term>
<term>Luminescence quenching</term>
<term>Multiple system</term>
<term>Photoluminescence</term>
<term>Radiative transfer</term>
<term>Terbium additions</term>
<term>Thulium additions</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Photoluminescence</term>
<term>Codopage</term>
<term>Dopage</term>
<term>Addition thulium</term>
<term>Addition terbium</term>
<term>Transfert énergie</term>
<term>Transfert radiatif</term>
<term>Etat impureté</term>
<term>Déclin luminescence</term>
<term>Transition niveau énergie</term>
<term>Extinction luminescence</term>
<term>Dipôle électrique</term>
<term>Interaction dipôle dipôle</term>
<term>Verre fluorure</term>
<term>Indium composé</term>
<term>Système multiple</term>
<term>Etude expérimentale</term>
<term>Système BaF2 GaF3 InF3 NaF SrF2 ZnF2</term>
<term>Ba F Ga In Na Sr Zn</term>
<term>7855H</term>
<term>7155J</term>
</keywords>
<keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Dopage</term>
</keywords>
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</teiHeader>
<front><div type="abstract" xml:lang="en">Effect of activator concentration on luminescence spectra and luminescence decay of excited states of Tm<sup>3+</sup>
 in indium-based fluoride glass has been investigated. Self-quenching of luminescence originating in the <sup>1</sup>
D<sub>2</sub>
, <sup>1</sup>
G<sub>4</sub>
 and the <sup>3</sup>
H<sub>4</sub>
 levels is found to be significant at doping levels as low as 0.5%. Luminescence decay curves are consistent with the Inokuti-Hirayama model for the non-radiative energy transfer involving an electric dipole-electric dipole interaction. Critical distance R<sub>0</sub>
=12.3 Å, derived from an analysis of the <sup>1</sup>
G<sub>4</sub>
 decay, is relatively high and indicates that the glass matrix favours the ion-ion interaction. Relaxation dynamics for glass samples doubly doped with thulium and terbium provides evidence that terbium ions are able to shorten the <sup>3</sup>
F<sub>4</sub>
 lifetime with extremely high efficiency. However, the Tm<sup>3+</sup>
→Tb<sup>3+</sup>
 energy transfer contributes adversely to relaxation of the <sup>3</sup>
H<sub>4</sub>
 level. Critical distance for this interaction is nearly the same as that for the self-quenching of Tm<sup>3+</sup>
 luminescence.</div>
</front>
</TEI>
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<fA03 i2="1"><s0>J. alloys compd.</s0>
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<fA05><s2>325</s2>
</fA05>
<fA06><s2>1-2</s2>
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<fA08 i1="01" i2="1" l="ENG"><s1>Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium</s1>
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<fA11 i1="01" i2="1"><s1>RYBA-ROMANOWSKI (W.)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>GOLŁAB (S.)</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>DOMINIAK-DZIK (G.)</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>ZELECHOWER (M.)</s1>
</fA11>
<fA11 i1="05" i2="1"><s1>GABRYS-PISARSKA (J.)</s1>
</fA11>
<fA14 i1="01"><s1>Institute of Low Temperature and Structure Research, Polish Academy of Sciences, 2 Okolna Street</s1>
<s2>50-422 Wroclaw</s2>
<s3>POL</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>Silesian University of Technology, Department of Materials Science, 8 Krasinskiego Street</s1>
<s2>40-019 Katowice</s2>
<s3>POL</s3>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
</fA14>
<fA20><s1>215-222</s1>
</fA20>
<fA21><s1>2001</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>1151</s2>
<s5>354000096660340340</s5>
</fA43>
<fA44><s0>0000</s0>
<s1>© 2001 INIST-CNRS. All rights reserved.</s1>
</fA44>
<fA45><s0>19 ref.</s0>
</fA45>
<fA47 i1="01" i2="1"><s0>01-0352918</s0>
</fA47>
<fA60><s1>P</s1>
</fA60>
<fA61><s0>A</s0>
</fA61>
<fA64 i1="01" i2="1"><s0>Journal of alloys and compounds</s0>
</fA64>
<fA66 i1="01"><s0>CHE</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>Effect of activator concentration on luminescence spectra and luminescence decay of excited states of Tm<sup>3+</sup>
 in indium-based fluoride glass has been investigated. Self-quenching of luminescence originating in the <sup>1</sup>
D<sub>2</sub>
, <sup>1</sup>
G<sub>4</sub>
 and the <sup>3</sup>
H<sub>4</sub>
 levels is found to be significant at doping levels as low as 0.5%. Luminescence decay curves are consistent with the Inokuti-Hirayama model for the non-radiative energy transfer involving an electric dipole-electric dipole interaction. Critical distance R<sub>0</sub>
=12.3 Å, derived from an analysis of the <sup>1</sup>
G<sub>4</sub>
 decay, is relatively high and indicates that the glass matrix favours the ion-ion interaction. Relaxation dynamics for glass samples doubly doped with thulium and terbium provides evidence that terbium ions are able to shorten the <sup>3</sup>
F<sub>4</sub>
 lifetime with extremely high efficiency. However, the Tm<sup>3+</sup>
→Tb<sup>3+</sup>
 energy transfer contributes adversely to relaxation of the <sup>3</sup>
H<sub>4</sub>
 level. Critical distance for this interaction is nearly the same as that for the self-quenching of Tm<sup>3+</sup>
 luminescence.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001B70H55H</s0>
</fC02>
<fC02 i1="02" i2="3"><s0>001B70A55J</s0>
</fC02>
<fC03 i1="01" i2="3" l="FRE"><s0>Photoluminescence</s0>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="3" l="ENG"><s0>Photoluminescence</s0>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="X" l="FRE"><s0>Codopage</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="ENG"><s0>Codoping</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="X" l="SPA"><s0>Codrogado</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="X" l="FRE"><s0>Dopage</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="ENG"><s0>Doping</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="X" l="SPA"><s0>Doping</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Addition thulium</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Thulium additions</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="3" l="FRE"><s0>Addition terbium</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="3" l="ENG"><s0>Terbium additions</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="3" l="FRE"><s0>Transfert énergie</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="3" l="ENG"><s0>Energy transfer</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="3" l="FRE"><s0>Transfert radiatif</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="3" l="ENG"><s0>Radiative transfer</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="3" l="FRE"><s0>Etat impureté</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="3" l="ENG"><s0>Impurity states</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="X" l="FRE"><s0>Déclin luminescence</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="ENG"><s0>Luminescence decay</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="X" l="SPA"><s0>Decadencia luminiscencia</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="3" l="FRE"><s0>Transition niveau énergie</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="3" l="ENG"><s0>Energy-level transitions</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="X" l="FRE"><s0>Extinction luminescence</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="ENG"><s0>Luminescence quenching</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="X" l="SPA"><s0>Extinción luminiscencia</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="3" l="FRE"><s0>Dipôle électrique</s0>
<s5>13</s5>
</fC03>
<fC03 i1="12" i2="3" l="ENG"><s0>Electric dipoles</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Interaction dipôle dipôle</s0>
<s5>14</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Dipole dipole interaction</s0>
<s5>14</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Interacción dipolo dipolo</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="3" l="FRE"><s0>Verre fluorure</s0>
<s5>15</s5>
</fC03>
<fC03 i1="14" i2="3" l="ENG"><s0>Fluoride glass</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>Indium composé</s0>
<s5>16</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>Indium compounds</s0>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Système multiple</s0>
<s5>17</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Multiple system</s0>
<s5>17</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Sistema múltiple</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="3" l="FRE"><s0>Etude expérimentale</s0>
<s5>18</s5>
</fC03>
<fC03 i1="17" i2="3" l="ENG"><s0>Experimental study</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>Système BaF2 GaF3 InF3 NaF SrF2 ZnF2</s0>
<s4>INC</s4>
<s5>52</s5>
</fC03>
<fC03 i1="19" i2="3" l="FRE"><s0>Ba F Ga In Na Sr Zn</s0>
<s4>INC</s4>
<s5>53</s5>
</fC03>
<fC03 i1="20" i2="3" l="FRE"><s0>7855H</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>56</s5>
</fC03>
<fC03 i1="21" i2="3" l="FRE"><s0>7155J</s0>
<s2>PAC</s2>
<s4>INC</s4>
<s5>57</s5>
</fC03>
<fN21><s1>246</s1>
</fN21>
</pA>
</standard>
</inist>
</record>

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Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium

Excited state relaxation dynamics and non-radiative energy transfer in fluoroindate glass singly doped with thulium and doubly doped with thulium and terbium

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