2.7 μm Emission from Transparent Er3+,Tm3+ Codoped Yttrium Aluminum Garnet (Y3Al5O12) Nanocrystals-Tellurate Glass Composites by Novel Comelting Technology
Identifieur interne : 000928 ( Main/Exploration ); précédent : 000927; suivant : 0009292.7 μm Emission from Transparent Er3+,Tm3+ Codoped Yttrium Aluminum Garnet (Y3Al5O12) Nanocrystals-Tellurate Glass Composites by Novel Comelting Technology
Auteurs : GUANQI CHAI [République populaire de Chine] ; GUOPING DONG [République populaire de Chine] ; JIANRONG QIU [République populaire de Chine] ; QINYUAN ZHANG [République populaire de Chine] ; ZHONGMIN YANG [République populaire de Chine]Source :
- Journal of physical chemistry. C [ 1932-7447 ] ; 2012.
Descripteurs français
- Pascal (Inist)
- Codopage, Spectrométrie FTIR, Microstructure, Addition erbium, Coprécipitation, Addition thulium, Transition niveau énergie, Etat impureté, Dimension particule, Photoluminescence, Transfert énergie, Conversion fréquence, Grenat aluminium yttrium, Nanocristal, Tellurate, Verre, Matériau composite, Nanocomposite, Matériau laser, Y3Al5O12.
- Wicri :
- topic : Verre, Matériau composite.
English descriptors
- KwdEn :
- Codoping, Composite materials, Coprecipitation, Energy transfer, Energy-level transitions, Erbium additions, Fourier-transformed infrared spectrometry, Frequency conversion, Glass, Impurity states, Laser materials, Microstructure, Nanocomposites, Nanocrystal, Particle size, Photoluminescence, Tellurates, Thulium additions, YAG.
Abstract
Yttrium aluminum garnet Y3Al5O12 (YA-G):Er3+,Tm3+ phosphor powders with preferable luminescent properties and nanocrystals with better morphology were synthesized by the solid-state reaction method and coprecipitation method, respectively. The composition and morphology were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), and transmission electron microscopy (TEM), which showed that the nanocrystals were pseudomonodispersed with the particle size of ∼30 nm. Photoluminescence (PL) spectra indicated the 2.7 μm emission of Er3+ was remarkably enhanced via Tm3+ sensitization, and a novel circulatory energy transfer mechanism was proposed. A novel dehydration method was used to decrease the contents of the hydroxyl group (OH-) confirmed by photoluminescence spectra and Fourier transform infrared spectra (FTIR). YAG crystallites were introduced into tellurate glass and formed to glass composites with good optical performance. These nanocrystals-glass composites open a brand new field for the research of mid-infrared laser materials.
Affiliations:
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Le document en format XML
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,Tm<sup>3+</sup>
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Al<sub>5</sub>
O<sub>12</sub>
) Nanocrystals-Tellurate Glass Composites by Novel Comelting Technology</title>
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<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">2.7 μm Emission from Transparent Er<sup>3+</sup>
,Tm<sup>3+</sup>
Codoped Yttrium Aluminum Garnet (Y<sub>3</sub>
Al<sub>5</sub>
O<sub>12</sub>
) Nanocrystals-Tellurate Glass Composites by Novel Comelting Technology</title>
<author><name sortKey="Guanqi Chai" sort="Guanqi Chai" uniqKey="Guanqi Chai" last="Guanqi Chai">GUANQI CHAI</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Luminescent Materials and Devices, and Institute of Optical Communication Materials, South China University of Technology</s1>
<s2>Guangzhou 510641</s2>
<s3>CHN</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
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<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
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<country>République populaire de Chine</country>
<placeName><settlement type="city">Jiangmen</settlement>
<region type="province">Guangdong</region>
</placeName>
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<author><name sortKey="Guoping Dong" sort="Guoping Dong" uniqKey="Guoping Dong" last="Guoping Dong">GUOPING DONG</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Luminescent Materials and Devices, and Institute of Optical Communication Materials, South China University of Technology</s1>
<s2>Guangzhou 510641</s2>
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<placeName><settlement type="city">Jiangmen</settlement>
<region type="province">Guangdong</region>
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<author><name sortKey="Jianrong Qiu" sort="Jianrong Qiu" uniqKey="Jianrong Qiu" last="Jianrong Qiu">JIANRONG QIU</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Luminescent Materials and Devices, and Institute of Optical Communication Materials, South China University of Technology</s1>
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<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
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<country>République populaire de Chine</country>
<placeName><settlement type="city">Jiangmen</settlement>
<region type="province">Guangdong</region>
</placeName>
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<author><name sortKey="Qinyuan Zhang" sort="Qinyuan Zhang" uniqKey="Qinyuan Zhang" last="Qinyuan Zhang">QINYUAN ZHANG</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Luminescent Materials and Devices, and Institute of Optical Communication Materials, South China University of Technology</s1>
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<author><name sortKey="Zhongmin Yang" sort="Zhongmin Yang" uniqKey="Zhongmin Yang" last="Zhongmin Yang">ZHONGMIN YANG</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>State Key Laboratory of Luminescent Materials and Devices, and Institute of Optical Communication Materials, South China University of Technology</s1>
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<s3>CHN</s3>
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<placeName><settlement type="city">Jiangmen</settlement>
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<series><title level="j" type="main">Journal of physical chemistry. C</title>
<title level="j" type="abbreviated">J. phys. chem., C</title>
<idno type="ISSN">1932-7447</idno>
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<seriesStmt><title level="j" type="main">Journal of physical chemistry. C</title>
<title level="j" type="abbreviated">J. phys. chem., C</title>
<idno type="ISSN">1932-7447</idno>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Codoping</term>
<term>Composite materials</term>
<term>Coprecipitation</term>
<term>Energy transfer</term>
<term>Energy-level transitions</term>
<term>Erbium additions</term>
<term>Fourier-transformed infrared spectrometry</term>
<term>Frequency conversion</term>
<term>Glass</term>
<term>Impurity states</term>
<term>Laser materials</term>
<term>Microstructure</term>
<term>Nanocomposites</term>
<term>Nanocrystal</term>
<term>Particle size</term>
<term>Photoluminescence</term>
<term>Tellurates</term>
<term>Thulium additions</term>
<term>YAG</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Codopage</term>
<term>Spectrométrie FTIR</term>
<term>Microstructure</term>
<term>Addition erbium</term>
<term>Coprécipitation</term>
<term>Addition thulium</term>
<term>Transition niveau énergie</term>
<term>Etat impureté</term>
<term>Dimension particule</term>
<term>Photoluminescence</term>
<term>Transfert énergie</term>
<term>Conversion fréquence</term>
<term>Grenat aluminium yttrium</term>
<term>Nanocristal</term>
<term>Tellurate</term>
<term>Verre</term>
<term>Matériau composite</term>
<term>Nanocomposite</term>
<term>Matériau laser</term>
<term>Y3Al5O12</term>
</keywords>
<keywords scheme="Wicri" type="topic" xml:lang="fr"><term>Verre</term>
<term>Matériau composite</term>
</keywords>
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<front><div type="abstract" xml:lang="en">Yttrium aluminum garnet Y<sub>3</sub>
Al<sub>5</sub>
O<sub>12</sub>
(YA-G):Er<sup>3+</sup>
,Tm<sup>3+</sup>
phosphor powders with preferable luminescent properties and nanocrystals with better morphology were synthesized by the solid-state reaction method and coprecipitation method, respectively. The composition and morphology were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), and transmission electron microscopy (TEM), which showed that the nanocrystals were pseudomonodispersed with the particle size of ∼30 nm. Photoluminescence (PL) spectra indicated the 2.7 μm emission of Er<sup>3+</sup>
was remarkably enhanced via Tm<sup>3+</sup>
sensitization, and a novel circulatory energy transfer mechanism was proposed. A novel dehydration method was used to decrease the contents of the hydroxyl group (OH<sup>-</sup>
) confirmed by photoluminescence spectra and Fourier transform infrared spectra (FTIR). YAG crystallites were introduced into tellurate glass and formed to glass composites with good optical performance. These nanocrystals-glass composites open a brand new field for the research of mid-infrared laser materials.</div>
</front>
</TEI>
<affiliations><list><country><li>République populaire de Chine</li>
</country>
<region><li>Guangdong</li>
</region>
<settlement><li>Jiangmen</li>
</settlement>
</list>
<tree><country name="République populaire de Chine"><region name="Guangdong"><name sortKey="Guanqi Chai" sort="Guanqi Chai" uniqKey="Guanqi Chai" last="Guanqi Chai">GUANQI CHAI</name>
</region>
<name sortKey="Guoping Dong" sort="Guoping Dong" uniqKey="Guoping Dong" last="Guoping Dong">GUOPING DONG</name>
<name sortKey="Jianrong Qiu" sort="Jianrong Qiu" uniqKey="Jianrong Qiu" last="Jianrong Qiu">JIANRONG QIU</name>
<name sortKey="Qinyuan Zhang" sort="Qinyuan Zhang" uniqKey="Qinyuan Zhang" last="Qinyuan Zhang">QINYUAN ZHANG</name>
<name sortKey="Zhongmin Yang" sort="Zhongmin Yang" uniqKey="Zhongmin Yang" last="Zhongmin Yang">ZHONGMIN YANG</name>
</country>
</tree>
</affiliations>
</record>
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