Laser-induced, Er3+ trace-sensitized red-to-blue photon-avalanche up-conversion in Tm3+:KY3F10
Identifieur interne : 000050 ( Hal/Checkpoint ); précédent : 000049; suivant : 000051Laser-induced, Er3+ trace-sensitized red-to-blue photon-avalanche up-conversion in Tm3+:KY3F10
Auteurs : E. Boulma [France] ; Jean Pierre Jouart [France] ; Michel Bouffard [France] ; Madjid Diaf [Algérie] ; Jean-Louis Doualan [France] ; Richard Moncorgé [France]Source :
- Optical Materials [ 0925-3467 ] ; 2008.
English descriptors
Abstract
We report here the first results of a spectroscopic study of anti-Stokes emissions from a Tm3+-doped KY3F10 crystal demonstrating the sensitization effect of Er3+ ions, present as trace impurities, on the ESA (3F4 → 1G4) lines of Tm3+.We have also detected Ho3+ traces in Tm3+:KY3F10. Contrary to the Er3+ ion, the Ho3+ ion does not increase the possibilities of resonant transfer with the Tm3+ ion. The Tm3+ →Ho3+ →Tm3+ transfers are much less probable than the Tm3+ → Er3+ → Tm3+ transfers. The majority of the Tm3+ ions excited by sensitized photon-avalanche absorption are exclusively located in the immediate neighbourhood of Er3+ ions. Red-to-green up-conversion mechanism is, for Er3+ either a two-step absorption process or a photon-avalanche absorption process, depending on whether the excitation wavelength is tuned on the 4I13/2 → 4F5/2 or 3F4→ 1G4 transitions.
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<front><div type="abstract" xml:lang="en">We report here the first results of a spectroscopic study of anti-Stokes emissions from a Tm3+-doped KY3F10 crystal demonstrating the sensitization effect of Er3+ ions, present as trace impurities, on the ESA (3F4 → 1G4) lines of Tm3+.We have also detected Ho3+ traces in Tm3+:KY3F10. Contrary to the Er3+ ion, the Ho3+ ion does not increase the possibilities of resonant transfer with the Tm3+ ion. The Tm3+ →Ho3+ →Tm3+ transfers are much less probable than the Tm3+ → Er3+ → Tm3+ transfers. The majority of the Tm3+ ions excited by sensitized photon-avalanche absorption are exclusively located in the immediate neighbourhood of Er3+ ions. Red-to-green up-conversion mechanism is, for Er3+ either a two-step absorption process or a photon-avalanche absorption process, depending on whether the excitation wavelength is tuned on the 4I13/2 → 4F5/2 or 3F4→ 1G4 transitions.</div>
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<idno type="stamp" n="ENSI-CAEN">Ecole Nationale Supérieure d'Ingénieurs de Caen</idno>
<idno type="stamp" n="CEA">CEA - Commissariat à l'énergie atomique</idno>
<idno type="stamp" n="DSM-IRAMIS">IRAMIS</idno>
<idno type="stamp" n="COMUE-NORMANDIE">Normandie Université</idno>
<idno type="stamp" n="IRAMIS-CIMAP" p="DSM-IRAMIS">CIMAP</idno>
</seriesStmt>
<notesStmt><note type="audience" n="2">International</note>
<note type="popular" n="0">No</note>
<note type="peer" n="1">Yes</note>
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<sourceDesc><biblStruct><analytic><title xml:lang="en">Laser-induced, Er3+ trace-sensitized red-to-blue photon-avalanche up-conversion in Tm3+:KY3F10</title>
<author role="aut"><persName><forename type="first">E.</forename>
<surname>Boulma</surname>
</persName>
<idno type="halAuthorId">371584</idno>
<affiliation ref="#struct-7569"></affiliation>
<affiliation ref="#struct-53650"></affiliation>
</author>
<author role="aut"><persName><forename type="first">Jean Pierre</forename>
<surname>Jouart</surname>
</persName>
<email>jean-pierre.jouart@univ-reims.fr</email>
<idno type="halAuthorId">371585</idno>
<affiliation ref="#struct-7569"></affiliation>
</author>
<author role="aut"><persName><forename type="first">Michel</forename>
<surname>Bouffard</surname>
</persName>
<idno type="halAuthorId">371586</idno>
<affiliation ref="#struct-7569"></affiliation>
</author>
<author role="aut"><persName><forename type="first">Madjid</forename>
<surname>Diaf</surname>
</persName>
<idno type="halAuthorId">371587</idno>
<affiliation ref="#struct-53650"></affiliation>
</author>
<author role="aut"><persName><forename type="first">Jean-Louis</forename>
<surname>Doualan</surname>
</persName>
<idno type="halAuthorId">195925</idno>
<affiliation ref="#struct-56527"></affiliation>
</author>
<author role="aut"><persName><forename type="first">Richard</forename>
<surname>Moncorgé</surname>
</persName>
<idno type="halAuthorId">81103</idno>
<affiliation ref="#struct-56527"></affiliation>
</author>
</analytic>
<monogr><idno type="halJournalId" status="VALID">17649</idno>
<idno type="issn">0925-3467</idno>
<title level="j">Optical Materials</title>
<imprint><publisher>Elsevier</publisher>
<biblScope unit="volume">30</biblScope>
<biblScope unit="pp">1028-1032</biblScope>
<date type="datePub">2008</date>
</imprint>
</monogr>
</biblStruct>
</sourceDesc>
<profileDesc><langUsage><language ident="en">English</language>
</langUsage>
<textClass><keywords scheme="author"><term xml:lang="en">Keywords: Fluoride crystals</term>
<term xml:lang="en">Optical spectroscopy</term>
<term xml:lang="en">Up-conversion</term>
<term xml:lang="en">Thulium</term>
<term xml:lang="en">Erbium</term>
<term xml:lang="en">Holmium</term>
</keywords>
<classCode scheme="classification">PACS: 78.55.-m; 42.62.Fi; 42.70.Hj</classCode>
<classCode scheme="halDomain" n="phys.phys.phys-optics">Physics [physics]/Physics [physics]/Optics [physics.optics]</classCode>
<classCode scheme="halTypology" n="ART">Journal articles</classCode>
</textClass>
<abstract xml:lang="en">We report here the first results of a spectroscopic study of anti-Stokes emissions from a Tm3+-doped KY3F10 crystal demonstrating the sensitization effect of Er3+ ions, present as trace impurities, on the ESA (3F4 → 1G4) lines of Tm3+.We have also detected Ho3+ traces in Tm3+:KY3F10. Contrary to the Er3+ ion, the Ho3+ ion does not increase the possibilities of resonant transfer with the Tm3+ ion. The Tm3+ →Ho3+ →Tm3+ transfers are much less probable than the Tm3+ → Er3+ → Tm3+ transfers. The majority of the Tm3+ ions excited by sensitized photon-avalanche absorption are exclusively located in the immediate neighbourhood of Er3+ ions. Red-to-green up-conversion mechanism is, for Er3+ either a two-step absorption process or a photon-avalanche absorption process, depending on whether the excitation wavelength is tuned on the 4I13/2 → 4F5/2 or 3F4→ 1G4 transitions.</abstract>
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