Ag loaded WO3 nanoplates for efficient photocatalytic degradation of sulfanilamide and their bactericidal effect under visible light irradiation.
Identifieur interne : 000639 ( Main/Corpus ); précédent : 000638; suivant : 000640Ag loaded WO3 nanoplates for efficient photocatalytic degradation of sulfanilamide and their bactericidal effect under visible light irradiation.
Auteurs : Wenyu Zhu ; Jincheng Liu ; Shuyan Yu ; Yan Zhou ; Xiaoli YanSource :
- Journal of hazardous materials [ 1873-3336 ] ; 2016.
English descriptors
- KwdEn :
- Anti-Bacterial Agents (metabolism), Bacillus subtilis (drug effects), Bacteria (drug effects), Bacteria (radiation effects), Biodegradation, Environmental (MeSH), Catalysis (MeSH), Escherichia coli (drug effects), Hydrogen-Ion Concentration (MeSH), Light (MeSH), Nanostructures (MeSH), Oxides (chemistry), Photochemical Processes (MeSH), Photolysis (MeSH), Silver (chemistry), Sulfanilamide (MeSH), Sulfanilamides (chemistry), Sulfanilamides (metabolism), Sulfanilamides (radiation effects), Temperature (MeSH), Tungsten (chemistry).
- MESH :
- chemical , chemistry : Oxides, Silver, Sulfanilamides, Tungsten.
- chemical , metabolism : Anti-Bacterial Agents, Sulfanilamides.
- drug effects : Bacillus subtilis, Bacteria, Escherichia coli.
- radiation effects : Bacteria, Sulfanilamides.
- Biodegradation, Environmental, Catalysis, Hydrogen-Ion Concentration, Light, Nanostructures, Photochemical Processes, Photolysis, Sulfanilamide, Temperature.
Abstract
Sulfonamides (SAs) are extensively used antibiotics and their residues in the water bodies propose potential threat to the public. In this study, degradation efficiency of sulfanilamide (SAM), which is the precursor of SAs, using WO3 nanoplates and their Ag heterogeneous as photocatalysts was investigated. WO3 nanoplates with uniform size were synthesized by a facile one step hydrothermal method. Different amount of Ag nanoparticles (Ag NPs) were loaded onto WO3 nanoplates using a photo-reduction method to generate WO3/Ag composites. The physio-chemical properties of synthesized nanomaterials were systematically characterized. Photodegradation of SAM by WO3 and WO3/Ag composites was conducted under visible light irradiation. The results show that WO3/Ag composites performed much better than pure WO3 where the highest removal rate was 96.2% in 5h. Ag as excellent antibacterial agent also endows certain antibacterial efficiency to WO3, and 100% removal efficiency against Escherichia Coli and Bacillus subtilis could be achieved in 2h under visible light irradiation for all three WO3/Ag composites synthesized. The improved performance in terms of SAM degradation and antibacterial activity of WO3/Ag can be attributed to the improved electron-hole pair separation rate where Ag NPs act as effective electron trapper during the photocatalytic process.
DOI: 10.1016/j.jhazmat.2016.06.066
PubMed: 27450332
Links to Exploration step
pubmed:27450332Le document en format XML
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Electronic address: JCLIU@ntu.edu.sg.</nlm:affiliation></affiliation></author><author><name sortKey="Yu, Shuyan" sort="Yu, Shuyan" uniqKey="Yu S" first="Shuyan" last="Yu">Shuyan Yu</name><affiliation><nlm:affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</nlm:affiliation></affiliation></author><author><name sortKey="Zhou, Yan" sort="Zhou, Yan" uniqKey="Zhou Y" first="Yan" last="Zhou">Yan Zhou</name><affiliation><nlm:affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</nlm:affiliation></affiliation></author><author><name sortKey="Yan, Xiaoli" sort="Yan, Xiaoli" uniqKey="Yan X" first="Xiaoli" last="Yan">Xiaoli Yan</name><affiliation><nlm:affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Current address: Environmental and Water Technology Centre of Innovation, Ngee Ann Polytechnic, 535 Clementi Road, Singapore 599489, Republic of Singapore. 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Electronic address: JCLIU@ntu.edu.sg.</nlm:affiliation></affiliation></author><author><name sortKey="Yu, Shuyan" sort="Yu, Shuyan" uniqKey="Yu S" first="Shuyan" last="Yu">Shuyan Yu</name><affiliation><nlm:affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</nlm:affiliation></affiliation></author><author><name sortKey="Zhou, Yan" sort="Zhou, Yan" uniqKey="Zhou Y" first="Yan" last="Zhou">Yan Zhou</name><affiliation><nlm:affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</nlm:affiliation></affiliation></author><author><name sortKey="Yan, Xiaoli" sort="Yan, Xiaoli" uniqKey="Yan X" first="Xiaoli" last="Yan">Xiaoli Yan</name><affiliation><nlm:affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Current address: Environmental and Water Technology Centre of Innovation, Ngee Ann Polytechnic, 535 Clementi Road, Singapore 599489, Republic of Singapore. Electronic address: XLYAN@ntu.edu.sg.</nlm:affiliation></affiliation></author></analytic><series><title level="j">Journal of hazardous materials</title><idno type="eISSN">1873-3336</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Anti-Bacterial Agents (metabolism)</term><term>Bacillus subtilis (drug effects)</term><term>Bacteria (drug effects)</term><term>Bacteria (radiation effects)</term><term>Biodegradation, Environmental (MeSH)</term><term>Catalysis (MeSH)</term><term>Escherichia coli (drug effects)</term><term>Hydrogen-Ion Concentration (MeSH)</term><term>Light (MeSH)</term><term>Nanostructures (MeSH)</term><term>Oxides (chemistry)</term><term>Photochemical Processes (MeSH)</term><term>Photolysis (MeSH)</term><term>Silver (chemistry)</term><term>Sulfanilamide (MeSH)</term><term>Sulfanilamides (chemistry)</term><term>Sulfanilamides (metabolism)</term><term>Sulfanilamides (radiation effects)</term><term>Temperature (MeSH)</term><term>Tungsten (chemistry)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Oxides</term><term>Silver</term><term>Sulfanilamides</term><term>Tungsten</term></keywords><keywords scheme="MESH" type="chemical" qualifier="metabolism" xml:lang="en"><term>Anti-Bacterial Agents</term><term>Sulfanilamides</term></keywords><keywords scheme="MESH" qualifier="drug effects" xml:lang="en"><term>Bacillus subtilis</term><term>Bacteria</term><term>Escherichia coli</term></keywords><keywords scheme="MESH" qualifier="radiation effects" xml:lang="en"><term>Bacteria</term><term>Sulfanilamides</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Biodegradation, Environmental</term><term>Catalysis</term><term>Hydrogen-Ion Concentration</term><term>Light</term><term>Nanostructures</term><term>Photochemical Processes</term><term>Photolysis</term><term>Sulfanilamide</term><term>Temperature</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Sulfonamides (SAs) are extensively used antibiotics and their residues in the water bodies propose potential threat to the public. In this study, degradation efficiency of sulfanilamide (SAM), which is the precursor of SAs, using WO3 nanoplates and their Ag heterogeneous as photocatalysts was investigated. WO3 nanoplates with uniform size were synthesized by a facile one step hydrothermal method. Different amount of Ag nanoparticles (Ag NPs) were loaded onto WO3 nanoplates using a photo-reduction method to generate WO3/Ag composites. The physio-chemical properties of synthesized nanomaterials were systematically characterized. Photodegradation of SAM by WO3 and WO3/Ag composites was conducted under visible light irradiation. The results show that WO3/Ag composites performed much better than pure WO3 where the highest removal rate was 96.2% in 5h. Ag as excellent antibacterial agent also endows certain antibacterial efficiency to WO3, and 100% removal efficiency against Escherichia Coli and Bacillus subtilis could be achieved in 2h under visible light irradiation for all three WO3/Ag composites synthesized. The improved performance in terms of SAM degradation and antibacterial activity of WO3/Ag can be attributed to the improved electron-hole pair separation rate where Ag NPs act as effective electron trapper during the photocatalytic process. </div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" Owner="NLM"><PMID Version="1">27450332</PMID><DateCompleted><Year>2018</Year><Month>02</Month><Day>26</Day></DateCompleted><DateRevised><Year>2018</Year><Month>12</Month><Day>02</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1873-3336</ISSN><JournalIssue CitedMedium="Internet"><Volume>318</Volume><PubDate><Year>2016</Year><Month>Nov</Month><Day>15</Day></PubDate></JournalIssue><Title>Journal of hazardous materials</Title><ISOAbbreviation>J Hazard Mater</ISOAbbreviation></Journal><ArticleTitle>Ag loaded WO3 nanoplates for efficient photocatalytic degradation of sulfanilamide and their bactericidal effect under visible light irradiation.</ArticleTitle><Pagination><MedlinePgn>407-416</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0304-3894(16)30621-5</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.jhazmat.2016.06.066</ELocationID><Abstract><AbstractText>Sulfonamides (SAs) are extensively used antibiotics and their residues in the water bodies propose potential threat to the public. In this study, degradation efficiency of sulfanilamide (SAM), which is the precursor of SAs, using WO3 nanoplates and their Ag heterogeneous as photocatalysts was investigated. WO3 nanoplates with uniform size were synthesized by a facile one step hydrothermal method. Different amount of Ag nanoparticles (Ag NPs) were loaded onto WO3 nanoplates using a photo-reduction method to generate WO3/Ag composites. The physio-chemical properties of synthesized nanomaterials were systematically characterized. Photodegradation of SAM by WO3 and WO3/Ag composites was conducted under visible light irradiation. The results show that WO3/Ag composites performed much better than pure WO3 where the highest removal rate was 96.2% in 5h. Ag as excellent antibacterial agent also endows certain antibacterial efficiency to WO3, and 100% removal efficiency against Escherichia Coli and Bacillus subtilis could be achieved in 2h under visible light irradiation for all three WO3/Ag composites synthesized. The improved performance in terms of SAM degradation and antibacterial activity of WO3/Ag can be attributed to the improved electron-hole pair separation rate where Ag NPs act as effective electron trapper during the photocatalytic process. </AbstractText><CopyrightInformation>Copyright © 2016 Elsevier B.V. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Zhu</LastName><ForeName>Wenyu</ForeName><Initials>W</Initials><AffiliationInfo><Affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Jincheng</ForeName><Initials>J</Initials><AffiliationInfo><Affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Current address: Faculty of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510009, China. Electronic address: JCLIU@ntu.edu.sg.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yu</LastName><ForeName>Shuyan</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhou</LastName><ForeName>Yan</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Nanyang Environment and Water Research Institute (NEWRI), Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Republic of Singapore.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yan</LastName><ForeName>Xiaoli</ForeName><Initials>X</Initials><AffiliationInfo><Affiliation>School of Civil and Environmental Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798, Republic of Singapore; Current address: Environmental and Water Technology Centre of Innovation, Ngee Ann Polytechnic, 535 Clementi Road, Singapore 599489, Republic of Singapore. Electronic address: XLYAN@ntu.edu.sg.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2016</Year><Month>07</Month><Day>01</Day></ArticleDate></Article><MedlineJournalInfo><Country>Netherlands</Country><MedlineTA>J Hazard Mater</MedlineTA><NlmUniqueID>9422688</NlmUniqueID><ISSNLinking>0304-3894</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D000900">Anti-Bacterial Agents</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D010087">Oxides</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D013424">Sulfanilamides</NameOfSubstance></Chemical><Chemical><RegistryNumber>21240MF57M</RegistryNumber><NameOfSubstance UI="D000077145">Sulfanilamide</NameOfSubstance></Chemical><Chemical><RegistryNumber>3M4G523W1G</RegistryNumber><NameOfSubstance UI="D012834">Silver</NameOfSubstance></Chemical><Chemical><RegistryNumber>940E10M08M</RegistryNumber><NameOfSubstance UI="C511604">tungsten oxide</NameOfSubstance></Chemical><Chemical><RegistryNumber>V9306CXO6G</RegistryNumber><NameOfSubstance UI="D014414">Tungsten</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000900" MajorTopicYN="N">Anti-Bacterial Agents</DescriptorName><QualifierName UI="Q000378" MajorTopicYN="Y">metabolism</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D001412" MajorTopicYN="N">Bacillus subtilis</DescriptorName><QualifierName UI="Q000187" MajorTopicYN="N">drug effects</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D001419" MajorTopicYN="N">Bacteria</DescriptorName><QualifierName UI="Q000187" MajorTopicYN="Y">drug effects</QualifierName><QualifierName UI="Q000528" MajorTopicYN="Y">radiation effects</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D001673" MajorTopicYN="N">Biodegradation, Environmental</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002384" MajorTopicYN="N">Catalysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D004926" MajorTopicYN="N">Escherichia coli</DescriptorName><QualifierName UI="Q000187" MajorTopicYN="N">drug effects</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D006863" MajorTopicYN="N">Hydrogen-Ion Concentration</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008027" MajorTopicYN="N">Light</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D049329" MajorTopicYN="N">Nanostructures</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D010087" MajorTopicYN="N">Oxides</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D055668" MajorTopicYN="N">Photochemical Processes</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D010782" MajorTopicYN="N">Photolysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D012834" MajorTopicYN="N">Silver</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D000077145" MajorTopicYN="N">Sulfanilamide</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D013424" MajorTopicYN="N">Sulfanilamides</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName><QualifierName UI="Q000378" MajorTopicYN="Y">metabolism</QualifierName><QualifierName UI="Q000528" MajorTopicYN="N">radiation effects</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D013696" MajorTopicYN="N">Temperature</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D014414" MajorTopicYN="N">Tungsten</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Bactericidal effect</Keyword><Keyword MajorTopicYN="N">Photocatalysis</Keyword><Keyword MajorTopicYN="N">Sulfanilamide</Keyword><Keyword MajorTopicYN="N">Tungsten trioxide</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2016</Year><Month>03</Month><Day>02</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2016</Year><Month>06</Month><Day>05</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2016</Year><Month>06</Month><Day>30</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2016</Year><Month>7</Month><Day>25</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2016</Year><Month>7</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2018</Year><Month>2</Month><Day>27</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">27450332</ArticleId><ArticleId IdType="pii">S0304-3894(16)30621-5</ArticleId><ArticleId IdType="doi">10.1016/j.jhazmat.2016.06.066</ArticleId></ArticleIdList></PubmedData></pubmed></record>Pour manipuler ce document sous Unix (Dilib)
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