Combustion chemistry and flame structure of furan group biofuels using molecular-beam mass spectrometry and gas chromatography - Part II: 2-Methylfuran.
Identifieur interne : 000043 ( PubMed/Curation ); précédent : 000042; suivant : 000044Combustion chemistry and flame structure of furan group biofuels using molecular-beam mass spectrometry and gas chromatography - Part II: 2-Methylfuran.
Auteurs : Luc-Sy Tran [France] ; Casimir Togbé [Allemagne] ; Dong Liu [Allemagne] ; Daniel Felsmann [Allemagne] ; Patrick O Wald [Allemagne] ; Pierre-Alexandre Glaude [France] ; René Fournet [France] ; Baptiste Sirjean [France] ; Frédérique Battin-Leclerc [France] ; Katharina Kohse-Höinghaus [Allemagne]Source :
- Combustion and flame [ 0010-2180 ] ; 2014.
Abstract
This is Part II of a series of three papers which jointly address the combustion chemistry of furan and its alkylated derivatives 2-methylfuran (MF) and 2,5-dimethylfuran (DMF) under premixed low-pressure flame conditions. Some of them are considered to be promising biofuels. With furan as a common basis studied in Part I of this series, the present paper addresses two laminar premixed low-pressure (20 and 40 mbar) flat argon-diluted (50%) flames of MF which were studied with electron-ionization molecular-beam mass spectrometry (EI-MBMS) and gas chromatography (GC) for equivalence ratios φ=1.0 and 1.7, identical conditions to those for the previously reported furan flames. Mole fractions of reactants, products as well as stable and reactive intermediates were measured as a function of the distance above the burner. Kinetic modeling was performed using a comprehensive reaction mechanism for all three fuels given in Part I and described in the three parts of this series. A comparison of the experimental results and the simulation shows reasonable agreement, as also seen for the furan flames in Part I before. This set of experiments is thus considered to be a valuable additional basis for the validation of the model. The main reaction pathways of MF consumption have been derived from reaction flow analyses, and differences to furan combustion chemistry under the same conditions are discussed.
DOI: 10.1016/j.combustflame.2013.05.027
PubMed: 24518895
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BP 20451, 54001 Nancy Cedex, France.</nlm:affiliation><country xml:lang="fr">France</country><wicri:regionArea>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex</wicri:regionArea></affiliation></author><author><name sortKey="Kohse Hoinghaus, Katharina" sort="Kohse Hoinghaus, Katharina" uniqKey="Kohse Hoinghaus K" first="Katharina" last="Kohse-Höinghaus">Katharina Kohse-Höinghaus</name><affiliation wicri:level="1"><nlm:affiliation>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany.</nlm:affiliation><country xml:lang="fr">Allemagne</country><wicri:regionArea>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld</wicri:regionArea></affiliation></author></analytic><series><title level="j">Combustion and flame</title><idno type="ISSN">0010-2180</idno><imprint><date when="2014" type="published">2014</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">This is Part II of a series of three papers which jointly address the combustion chemistry of furan and its alkylated derivatives 2-methylfuran (MF) and 2,5-dimethylfuran (DMF) under premixed low-pressure flame conditions. Some of them are considered to be promising biofuels. With furan as a common basis studied in Part I of this series, the present paper addresses two laminar premixed low-pressure (20 and 40 mbar) flat argon-diluted (50%) flames of MF which were studied with electron-ionization molecular-beam mass spectrometry (EI-MBMS) and gas chromatography (GC) for equivalence ratios φ=1.0 and 1.7, identical conditions to those for the previously reported furan flames. Mole fractions of reactants, products as well as stable and reactive intermediates were measured as a function of the distance above the burner. Kinetic modeling was performed using a comprehensive reaction mechanism for all three fuels given in Part I and described in the three parts of this series. A comparison of the experimental results and the simulation shows reasonable agreement, as also seen for the furan flames in Part I before. This set of experiments is thus considered to be a valuable additional basis for the validation of the model. The main reaction pathways of MF consumption have been derived from reaction flow analyses, and differences to furan combustion chemistry under the same conditions are discussed.</div></front></TEI><pubmed><MedlineCitation Status="Publisher" Owner="NLM"><PMID Version="1">24518895</PMID><DateCreated><Year>2014</Year><Month>2</Month><Day>12</Day></DateCreated><DateRevised><Year>2015</Year><Month>9</Month><Day>1</Day></DateRevised><Article PubModel="Print"><Journal><ISSN IssnType="Print">0010-2180</ISSN><JournalIssue CitedMedium="Print"><Volume>161</Volume><Issue>3</Issue><PubDate><Year>2014</Year><Month>Mar</Month><Day>1</Day></PubDate></JournalIssue><Title>Combustion and flame</Title><ISOAbbreviation>Combust Flame</ISOAbbreviation></Journal><ArticleTitle>Combustion chemistry and flame structure of furan group biofuels using molecular-beam mass spectrometry and gas chromatography - Part II: 2-Methylfuran.</ArticleTitle><Pagination><MedlinePgn>766-779</MedlinePgn></Pagination><Abstract><AbstractText>This is Part II of a series of three papers which jointly address the combustion chemistry of furan and its alkylated derivatives 2-methylfuran (MF) and 2,5-dimethylfuran (DMF) under premixed low-pressure flame conditions. Some of them are considered to be promising biofuels. With furan as a common basis studied in Part I of this series, the present paper addresses two laminar premixed low-pressure (20 and 40 mbar) flat argon-diluted (50%) flames of MF which were studied with electron-ionization molecular-beam mass spectrometry (EI-MBMS) and gas chromatography (GC) for equivalence ratios φ=1.0 and 1.7, identical conditions to those for the previously reported furan flames. Mole fractions of reactants, products as well as stable and reactive intermediates were measured as a function of the distance above the burner. Kinetic modeling was performed using a comprehensive reaction mechanism for all three fuels given in Part I and described in the three parts of this series. A comparison of the experimental results and the simulation shows reasonable agreement, as also seen for the furan flames in Part I before. This set of experiments is thus considered to be a valuable additional basis for the validation of the model. The main reaction pathways of MF consumption have been derived from reaction flow analyses, and differences to furan combustion chemistry under the same conditions are discussed.</AbstractText></Abstract><AuthorList><Author><LastName>Tran</LastName><ForeName>Luc-Sy</ForeName><Initials>LS</Initials><AffiliationInfo><Affiliation>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France.</Affiliation></AffiliationInfo></Author><Author><LastName>Togbé</LastName><ForeName>Casimir</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany.</Affiliation></AffiliationInfo></Author><Author><LastName>Liu</LastName><ForeName>Dong</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany.</Affiliation></AffiliationInfo></Author><Author><LastName>Felsmann</LastName><ForeName>Daniel</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany.</Affiliation></AffiliationInfo></Author><Author><LastName>Oßwald</LastName><ForeName>Patrick</ForeName><Initials>P</Initials><AffiliationInfo><Affiliation>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany.</Affiliation></AffiliationInfo></Author><Author><LastName>Glaude</LastName><ForeName>Pierre-Alexandre</ForeName><Initials>PA</Initials><AffiliationInfo><Affiliation>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France.</Affiliation></AffiliationInfo></Author><Author><LastName>Fournet</LastName><ForeName>René</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France.</Affiliation></AffiliationInfo></Author><Author><LastName>Sirjean</LastName><ForeName>Baptiste</ForeName><Initials>B</Initials><AffiliationInfo><Affiliation>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France.</Affiliation></AffiliationInfo></Author><Author><LastName>Battin-Leclerc</LastName><ForeName>Frédérique</ForeName><Initials>F</Initials><AffiliationInfo><Affiliation>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France.</Affiliation></AffiliationInfo></Author><Author><LastName>Kohse-Höinghaus</LastName><ForeName>Katharina</ForeName><Initials>K</Initials><AffiliationInfo><Affiliation>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany.</Affiliation></AffiliationInfo></Author></AuthorList><Language>ENG</Language><GrantList><Grant><GrantID>227669</GrantID><Agency>European Research Council</Agency><Country>International</Country></Grant></GrantList><PublicationTypeList><PublicationType UI="">JOURNAL ARTICLE</PublicationType></PublicationTypeList></Article><MedlineJournalInfo><MedlineTA>Combust Flame</MedlineTA><NlmUniqueID>9891739</NlmUniqueID><ISSNLinking>0010-2180</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">2-methylfuran</Keyword><Keyword MajorTopicYN="N">gas chromatography</Keyword><Keyword MajorTopicYN="N">low-pressure flame</Keyword><Keyword MajorTopicYN="N">model</Keyword><Keyword MajorTopicYN="N">molecular-beam mass spectrometry</Keyword><Keyword MajorTopicYN="N">reaction flow analysis</Keyword><Keyword MajorTopicYN="N">reaction mechanism</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="entrez"><Year>2014</Year><Month>2</Month><Day>13</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2014</Year><Month>2</Month><Day>13</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2014</Year><Month>2</Month><Day>13</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="doi">10.1016/j.combustflame.2013.05.027</ArticleId><ArticleId IdType="pubmed">24518895</ArticleId><ArticleId IdType="pmc">PMC3837210</ArticleId><ArticleId IdType="mid">EMS54901</ArticleId></ArticleIdList><pmc-dir>nihms</pmc-dir>
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