Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes.
Identifieur interne : 000065 ( PubMed/Corpus ); précédent : 000064; suivant : 000066Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes.
Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-LeclercSource :
- Journal of the American Chemical Society [ 1520-5126 ] ; 2012.
Abstract
The first reliable quantification of hydrogen peroxide (H(2)O(2)) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.
DOI: 10.1021/ja305200h
PubMed: 22746212
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pubmed:22746212Le document en format XML
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<front><div type="abstract" xml:lang="en">The first reliable quantification of hydrogen peroxide (H(2)O(2)) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</div>
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<CommentsCorrectionsList><CommentsCorrections RefType="Cites"><RefSource>Chem Soc Rev. 2011 Sep;40(9):4762-82</RefSource>
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