LrgpV1, PubMed, Corpus, bibRecord, 000065

Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes.

Identifieur interne : 000065 ( PubMed/Corpus ); précédent : 000064; suivant : 000066

Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes.

Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-Leclerc

Source :

Journal of the American Chemical Society [ 1520-5126 ] ; 2012.

RBID : pubmed:22746212

Abstract

The first reliable quantification of hydrogen peroxide (H(2)O(2)) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.

DOI: 10.1021/ja305200h
PubMed: 22746212

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pubmed:22746212

Le document en format XML

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<author><name sortKey="Herbinet, Olivier" sort="Herbinet, Olivier" uniqKey="Herbinet O" first="Olivier" last="Herbinet">Olivier Herbinet</name>
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<author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name>
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<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
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<front><div type="abstract" xml:lang="en">The first reliable quantification of hydrogen peroxide (H(2)O(2)) formed during the low-temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near-infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behavior close to that of the species present in gasoline and diesel fuels.</div>
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<CommentsCorrectionsList><CommentsCorrections RefType="Cites"><RefSource>Chem Soc Rev. 2011 Sep;40(9):4762-82</RefSource>
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Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes.

Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes.

Source :

Abstract

Links to Exploration step

Le document en format XML

Pour manipuler ce document sous Unix (Dilib)

Pour mettre un lien sur cette page dans le réseau Wicri

Pour générer des pages wiki