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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en">Combustion chemistry and flame structure of furan group biofuels using molecular-beam mass spectrometry and gas chromatography – Part II: 2-Methylfuran</title><author><name sortKey="Tran, Luc Sy" sort="Tran, Luc Sy" uniqKey="Tran L" first="Luc-Sy" last="Tran">Luc-Sy Tran</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Togbe, Casimir" sort="Togbe, Casimir" uniqKey="Togbe C" first="Casimir" last="Togbé">Casimir Togbé</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="Liu, Dong" sort="Liu, Dong" uniqKey="Liu D" first="Dong" last="Liu">Dong Liu</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="Felsmann, Daniel" sort="Felsmann, Daniel" uniqKey="Felsmann D" first="Daniel" last="Felsmann">Daniel Felsmann</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="O Wald, Patrick" sort="O Wald, Patrick" uniqKey="O Wald P" first="Patrick" last="O Wald">Patrick O Wald</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Fournet, Rene" sort="Fournet, Rene" uniqKey="Fournet R" first="René" last="Fournet">René Fournet</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Sirjean, Baptiste" sort="Sirjean, Baptiste" uniqKey="Sirjean B" first="Baptiste" last="Sirjean">Baptiste Sirjean</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Kohse Hoinghaus, Katharina" sort="Kohse Hoinghaus, Katharina" uniqKey="Kohse Hoinghaus K" first="Katharina" last="Kohse-Höinghaus">Katharina Kohse-Höinghaus</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">PMC</idno><idno type="pmid">24518895</idno><idno type="pmc">3837210</idno><idno type="url">http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3837210</idno><idno type="RBID">PMC:3837210</idno><idno type="doi">10.1016/j.combustflame.2013.05.027</idno><date when="2014">2014</date><idno type="wicri:Area/Pmc/Corpus">000172</idno><idno type="wicri:explorRef" wicri:stream="Pmc" wicri:step="Corpus" wicri:corpus="PMC">000172</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a" type="main">Combustion chemistry and flame structure of furan group biofuels using molecular-beam mass spectrometry and gas chromatography – Part II: 2-Methylfuran</title><author><name sortKey="Tran, Luc Sy" sort="Tran, Luc Sy" uniqKey="Tran L" first="Luc-Sy" last="Tran">Luc-Sy Tran</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Togbe, Casimir" sort="Togbe, Casimir" uniqKey="Togbe C" first="Casimir" last="Togbé">Casimir Togbé</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="Liu, Dong" sort="Liu, Dong" uniqKey="Liu D" first="Dong" last="Liu">Dong Liu</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="Felsmann, Daniel" sort="Felsmann, Daniel" uniqKey="Felsmann D" first="Daniel" last="Felsmann">Daniel Felsmann</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="O Wald, Patrick" sort="O Wald, Patrick" uniqKey="O Wald P" first="Patrick" last="O Wald">Patrick O Wald</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author><author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Fournet, Rene" sort="Fournet, Rene" uniqKey="Fournet R" first="René" last="Fournet">René Fournet</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Sirjean, Baptiste" sort="Sirjean, Baptiste" uniqKey="Sirjean B" first="Baptiste" last="Sirjean">Baptiste Sirjean</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name><affiliation><nlm:aff id="A1">Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</nlm:aff></affiliation></author><author><name sortKey="Kohse Hoinghaus, Katharina" sort="Kohse Hoinghaus, Katharina" uniqKey="Kohse Hoinghaus K" first="Katharina" last="Kohse-Höinghaus">Katharina Kohse-Höinghaus</name><affiliation><nlm:aff id="A2">Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</nlm:aff></affiliation></author></analytic><series><title level="j">Combustion and flame</title><idno type="ISSN">0010-2180</idno><idno type="eISSN">1556-2921</idno><imprint><date when="2014">2014</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p id="P2">This is Part II of a series of three papers which jointly address the combustion chemistry of furan and its alkylated derivatives 2-methylfuran (MF) and 2,5-dimethylfuran (DMF) under premixed low-pressure flame conditions. Some of them are considered to be promising biofuels. With furan as a common basis studied in Part I of this series, the present paper addresses two laminar premixed low-pressure (20 and 40 mbar) flat argon-diluted (50%) flames of MF which were studied with electron-ionization molecular-beam mass spectrometry (EI-MBMS) and gas chromatography (GC) for equivalence ratios φ=1.0 and 1.7, identical conditions to those for the previously reported furan flames. Mole fractions of reactants, products as well as stable and reactive intermediates were measured as a function of the distance above the burner. Kinetic modeling was performed using a comprehensive reaction mechanism for all three fuels given in Part I and described in the three parts of this series. A comparison of the experimental results and the simulation shows reasonable agreement, as also seen for the furan flames in Part I before. This set of experiments is thus considered to be a valuable additional basis for the validation of the model. The main reaction pathways of MF consumption have been derived from reaction flow analyses, and differences to furan combustion chemistry under the same conditions are discussed.</p></div></front></TEI><pmc article-type="research-article"><pmc-comment>The publisher of this article does not allow downloading of the full text in XML form.</pmc-comment>
<pmc-dir>properties manuscript</pmc-dir>
<front><journal-meta><journal-id journal-id-type="nlm-journal-id">9891739</journal-id><journal-id journal-id-type="pubmed-jr-id">41274</journal-id><journal-id journal-id-type="nlm-ta">Combust Flame</journal-id><journal-id journal-id-type="iso-abbrev">Combust Flame</journal-id><journal-title-group><journal-title>Combustion and flame</journal-title></journal-title-group><issn pub-type="ppub">0010-2180</issn><issn pub-type="epub">1556-2921</issn></journal-meta><article-meta><article-id pub-id-type="pmid">24518895</article-id><article-id pub-id-type="pmc">3837210</article-id><article-id pub-id-type="doi">10.1016/j.combustflame.2013.05.027</article-id><article-id pub-id-type="manuscript">EMS54901</article-id><article-categories><subj-group subj-group-type="heading"><subject>Article</subject></subj-group></article-categories><title-group><article-title>Combustion chemistry and flame structure of furan group biofuels using molecular-beam mass spectrometry and gas chromatography – Part II: 2-Methylfuran</article-title></title-group><contrib-group><contrib contrib-type="author"><name><surname>Tran</surname><given-names>Luc-Sy</given-names></name><xref ref-type="aff" rid="A1">1</xref></contrib><contrib contrib-type="author"><name><surname>Togbé</surname><given-names>Casimir</given-names></name><xref ref-type="aff" rid="A2">2</xref></contrib><contrib contrib-type="author"><name><surname>Liu</surname><given-names>Dong</given-names></name><xref ref-type="aff" rid="A2">2</xref></contrib><contrib contrib-type="author"><name><surname>Felsmann</surname><given-names>Daniel</given-names></name><xref ref-type="aff" rid="A2">2</xref></contrib><contrib contrib-type="author"><name><surname>Oßwald</surname><given-names>Patrick</given-names></name><xref ref-type="aff" rid="A2">2</xref><xref ref-type="author-notes" rid="FN2">#</xref></contrib><contrib contrib-type="author"><name><surname>Glaude</surname><given-names>Pierre-Alexandre</given-names></name><xref ref-type="aff" rid="A1">1</xref></contrib><contrib contrib-type="author"><name><surname>Fournet</surname><given-names>René</given-names></name><xref ref-type="aff" rid="A1">1</xref></contrib><contrib contrib-type="author"><name><surname>Sirjean</surname><given-names>Baptiste</given-names></name><xref ref-type="aff" rid="A1">1</xref></contrib><contrib contrib-type="author"><name><surname>Battin-Leclerc</surname><given-names>Frédérique</given-names></name><xref ref-type="aff" rid="A1">1</xref><xref ref-type="corresp" rid="CR1">*</xref></contrib><contrib contrib-type="author"><name><surname>Kohse-Höinghaus</surname><given-names>Katharina</given-names></name><xref ref-type="aff" rid="A2">2</xref><xref ref-type="corresp" rid="CR1">*</xref></contrib></contrib-group><aff id="A1"><label>1</label>Laboratoire Réactions et Génie des Procédés (LRGP), CNRS, Université de Lorraine, ENSIC, 1 rue Grandville, BP 20451, 54001 Nancy Cedex, France</aff><aff id="A2"><label>2</label>Department of Chemistry, Bielefeld University, Universitätsstraße 25, D-33615 Bielefeld, Germany</aff><author-notes><corresp id="CR1"><label>*</label>Corresponding authors. Katharina Kohse-Höinghaus: <email>kkh@uni-bielefeld.de</email>, Phone: +49 521 106 2052, Fax: +49 521 106 6027 and Frédérique Battin-Leclerc: <email>frederique.battin-leclerc@univ-lorraine.fr</email>, Phone: +33 3 83 17 51 25, Fax: +33 3 83 37 81 20
</corresp><fn fn-type="current-aff" id="FN2"><label>#</label><p id="P1">now at German Aerospace Center (DLR), Institute of Combustion Technology, Pfaffenwaldring 38-40, D-70569 Stuttgart, Germany</p></fn></author-notes><pub-date pub-type="nihms-submitted"><day>26</day><month>9</month><year>2013</year></pub-date><pub-date pub-type="ppub"><day>1</day><month>3</month><year>2014</year></pub-date><pub-date pub-type="pmc-release"><day>01</day><month>9</month><year>2015</year></pub-date><volume>161</volume><issue>3</issue><fpage>766</fpage><lpage>779</lpage><pmc-comment>elocation-id from pubmed: 10.1016/j.combustflame.2013.05.027</pmc-comment>
<self-uri xlink:href="http://www.sciencedirect.com/science/article/pii/S0010218013002204"></self-uri><abstract><p id="P2">This is Part II of a series of three papers which jointly address the combustion chemistry of furan and its alkylated derivatives 2-methylfuran (MF) and 2,5-dimethylfuran (DMF) under premixed low-pressure flame conditions. Some of them are considered to be promising biofuels. With furan as a common basis studied in Part I of this series, the present paper addresses two laminar premixed low-pressure (20 and 40 mbar) flat argon-diluted (50%) flames of MF which were studied with electron-ionization molecular-beam mass spectrometry (EI-MBMS) and gas chromatography (GC) for equivalence ratios φ=1.0 and 1.7, identical conditions to those for the previously reported furan flames. Mole fractions of reactants, products as well as stable and reactive intermediates were measured as a function of the distance above the burner. Kinetic modeling was performed using a comprehensive reaction mechanism for all three fuels given in Part I and described in the three parts of this series. A comparison of the experimental results and the simulation shows reasonable agreement, as also seen for the furan flames in Part I before. This set of experiments is thus considered to be a valuable additional basis for the validation of the model. The main reaction pathways of MF consumption have been derived from reaction flow analyses, and differences to furan combustion chemistry under the same conditions are discussed.</p></abstract><kwd-group><kwd>2-methylfuran</kwd><kwd>low-pressure flame</kwd><kwd>model</kwd><kwd>reaction mechanism</kwd><kwd>reaction flow analysis</kwd><kwd>molecular-beam mass spectrometry</kwd><kwd>gas chromatography</kwd></kwd-group><funding-group><award-group><funding-source country="International">European Research Council : </funding-source><award-id>227669 || ERC_</award-id></award-group></funding-group></article-meta></front></pmc></record>Pour manipuler ce document sous Unix (Dilib)
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