LrgpV1, Pmc, Corpus, bibRecord, 000155

Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes

Identifieur interne : 000155 ( Pmc/Corpus ); précédent : 000154; suivant : 000156

Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes

Auteurs : Chiheb Bahrini ; Olivier Herbinet ; Pierre-Alexandre Glaude ; Coralie Schoemaecker ; Christa Fittschen ; Frédérique Battin-Leclerc

Source :

Journal of the American Chemical Society [ 0002-7863 ] ; 2012.

RBID : PMC:3586669

Abstract

The first reliable quantification of hydrogen peroxide (H₂O₂) formed during the low temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was n-butane, the smallest alkane which has an oxidation behaviour close to that of the species present in gasoline and diesel fuels.

Url:

http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3586669

DOI: 10.1021/ja305200h
PubMed: 22746212
PubMed Central: 3586669

Links to Exploration step

PMC:3586669

Le document en format XML

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<author><name sortKey="Bahrini, Chiheb" sort="Bahrini, Chiheb" uniqKey="Bahrini C" first="Chiheb" last="Bahrini">Chiheb Bahrini</name>
<affiliation><nlm:aff id="A1">LRGP, Université de Lorraine, CNRS, ENSIC, BP 20451, 1 rue Grandville, 54001 Nancy, France</nlm:aff>
</affiliation>
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<author><name sortKey="Herbinet, Olivier" sort="Herbinet, Olivier" uniqKey="Herbinet O" first="Olivier" last="Herbinet">Olivier Herbinet</name>
<affiliation><nlm:aff id="A1">LRGP, Université de Lorraine, CNRS, ENSIC, BP 20451, 1 rue Grandville, 54001 Nancy, France</nlm:aff>
</affiliation>
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<author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name>
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<author><name sortKey="Schoemaecker, Coralie" sort="Schoemaecker, Coralie" uniqKey="Schoemaecker C" first="Coralie" last="Schoemaecker">Coralie Schoemaecker</name>
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</affiliation>
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<author><name sortKey="Fittschen, Christa" sort="Fittschen, Christa" uniqKey="Fittschen C" first="Christa" last="Fittschen">Christa Fittschen</name>
<affiliation><nlm:aff id="A2">PC2A, University Lille 1, CNRS, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France</nlm:aff>
</affiliation>
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<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
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<author><name sortKey="Glaude, Pierre Alexandre" sort="Glaude, Pierre Alexandre" uniqKey="Glaude P" first="Pierre-Alexandre" last="Glaude">Pierre-Alexandre Glaude</name>
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<author><name sortKey="Schoemaecker, Coralie" sort="Schoemaecker, Coralie" uniqKey="Schoemaecker C" first="Coralie" last="Schoemaecker">Coralie Schoemaecker</name>
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</affiliation>
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<author><name sortKey="Fittschen, Christa" sort="Fittschen, Christa" uniqKey="Fittschen C" first="Christa" last="Fittschen">Christa Fittschen</name>
<affiliation><nlm:aff id="A2">PC2A, University Lille 1, CNRS, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France</nlm:aff>
</affiliation>
</author>
<author><name sortKey="Battin Leclerc, Frederique" sort="Battin Leclerc, Frederique" uniqKey="Battin Leclerc F" first="Frédérique" last="Battin-Leclerc">Frédérique Battin-Leclerc</name>
<affiliation><nlm:aff id="A1">LRGP, Université de Lorraine, CNRS, ENSIC, BP 20451, 1 rue Grandville, 54001 Nancy, France</nlm:aff>
</affiliation>
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<series><title level="j">Journal of the American Chemical Society</title>
<idno type="ISSN">0002-7863</idno>
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<front><div type="abstract" xml:lang="en"><p id="P1">The first reliable quantification of hydrogen peroxide (H<sub>2</sub>
O<sub>2</sub>
) formed during the low temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was <italic>n</italic>
-butane, the smallest alkane which has an oxidation behaviour close to that of the species present in gasoline and diesel fuels.</p>
</div>
</front>
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<pmc article-type="research-article"><pmc-comment>The publisher of this article does not allow downloading of the full text in XML form.</pmc-comment>
  <pmc-dir>properties manuscript</pmc-dir>
  <front><journal-meta><journal-id journal-id-type="nlm-journal-id">7503056</journal-id>
<journal-id journal-id-type="pubmed-jr-id">4435</journal-id>
<journal-id journal-id-type="nlm-ta">J Am Chem Soc</journal-id>
<journal-id journal-id-type="iso-abbrev">J. Am. Chem. Soc.</journal-id>
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<article-categories><subj-group subj-group-type="heading"><subject>Article</subject>
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<title-group><article-title>Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes</article-title>
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<contrib-group><contrib contrib-type="author"><name><surname>Bahrini</surname>
<given-names>Chiheb</given-names>
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<xref ref-type="aff" rid="A1">#</xref>
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<contrib contrib-type="author"><name><surname>Herbinet</surname>
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<contrib contrib-type="author"><name><surname>Glaude</surname>
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<contrib contrib-type="author"><name><surname>Schoemaecker</surname>
<given-names>Coralie</given-names>
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<xref ref-type="aff" rid="A2">$</xref>
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<contrib contrib-type="author"><name><surname>Fittschen</surname>
<given-names>Christa</given-names>
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<xref ref-type="aff" rid="A2">$</xref>
</contrib>
<contrib contrib-type="author"><name><surname>Battin-Leclerc</surname>
<given-names>Frédérique</given-names>
</name>
<xref ref-type="aff" rid="A1">#</xref>
<xref ref-type="corresp" rid="CR1">*</xref>
</contrib>
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<aff id="A1"><label>#</label>
LRGP, Université de Lorraine, CNRS, ENSIC, BP 20451, 1 rue Grandville, 54001 Nancy, France</aff>
<aff id="A2"><label>$</label>
PC2A, University Lille 1, CNRS, Cité Scientifique, Bât. C11, 59655 Villeneuve d’Ascq, France</aff>
<author-notes><corresp id="CR1"><label>*</label>
<bold>Corresponding Author</bold>
: <email>Frederique.Battin-Leclerc@ensic.inpl-nancy.fr</email>
</corresp>
</author-notes>
<pub-date pub-type="nihms-submitted"><day>22</day>
<month>2</month>
<year>2013</year>
</pub-date>
<pub-date pub-type="epub"><day>12</day>
<month>7</month>
<year>2012</year>
</pub-date>
<pub-date pub-type="ppub"><day>25</day>
<month>7</month>
<year>2012</year>
</pub-date>
<pub-date pub-type="pmc-release"><day>04</day>
<month>3</month>
<year>2013</year>
</pub-date>
<volume>134</volume>
<issue>29</issue>
<fpage>11944</fpage>
<lpage>11947</lpage>
<abstract><p id="P1">The first reliable quantification of hydrogen peroxide (H<sub>2</sub>
O<sub>2</sub>
) formed during the low temperature oxidation of an organic compound has been achieved thanks to a new system that couples a jet stirred reactor to a detection by continuous wave cavity ring-down spectroscopy (cw-CRDS) in the near infrared. The quantification of this key compound for hydrocarbon low-temperature oxidation regime has been obtained under conditions close to those actually observed before the autoignition. The studied hydrocarbon was <italic>n</italic>
-butane, the smallest alkane which has an oxidation behaviour close to that of the species present in gasoline and diesel fuels.</p>
</abstract>
<kwd-group><kwd>Hydrogen peroxide</kwd>
<kwd>alkane oxidation</kwd>
<kwd>jet stirred reactor</kwd>
<kwd>cavity ring down spectroscopy</kwd>
</kwd-group>
<funding-group><award-group><funding-source country="International">European Research Council : </funding-source>
<award-id>227669 || ERC_</award-id>
</award-group>
</funding-group>
</article-meta>
</front>
</pmc>
</record>

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Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes

Quantification of hydrogen peroxide during the low-temperature oxidation of alkanes

Source :

Abstract

Links to Exploration step

Le document en format XML

Pour manipuler ce document sous Unix (Dilib)

Pour mettre un lien sur cette page dans le réseau Wicri

Pour générer des pages wiki