Photocatalytic degradation of gaseous 1-propanol using an annular reactor : Kinetic modelling and pathways
Identifieur interne : 000331 ( PascalFrancis/Corpus ); précédent : 000330; suivant : 000332Photocatalytic degradation of gaseous 1-propanol using an annular reactor : Kinetic modelling and pathways
Auteurs : G. Vincent ; P. M. Marquaire ; O. ZahraaSource :
- Journal of hazardous materials [ 0304-3894 ] ; 2009.
Descripteurs français
- Pascal (Inist)
- Dégradation photochimique, Réacteur photochimique, Modèle cinétique, Photocatalyse, Oxydation, Pollution, Décontamination, Composé organique volatil, Réacteur catalytique, Réacteur parfaitement agité, Paramètre cinétique, Polluant, Teneur eau, Produit réaction, Modélisation, Adsorption, Devenir polluant.
English descriptors
- KwdEn :
- Adsorption, Catalytic reactor, Continuous stirred tank reactor, Decontamination, Kinetic model, Kinetic parameter, Modeling, Oxidation, Photocatalysis, Photochemical degradation, Photochemical reactor, Pollutant, Pollutant behavior, Pollution, Reaction product, Volatile organic compound, Water content.
Abstract
Photocatalytic oxidation of airborne contaminants appears to be a promising process for remediation of air polluted by Volatile Organic Compounds (VOCs). In the present work, the photocatalytic oxidation of gaseous 1-propanol has been investigated by using an annular photoreactor. The annular photocatalytic reactor was modelled by a cascade of heightened elementary continuously stirred tank reactors. The influence of several kinetic parameters such as pollutant concentration, incident light irradiance, contact time and humidity content has been studied. The photocatalytic degradation by-products of 1-propanol has been identified in the gas-phase by GC/MS. Propionaldehyde and acetaldehyde were found to be the main gaseous intermediates. Propionaldehyde and acetaldehyde have been taken into account in a "two-site model" to evaluate the possible competition of adsorption between 1-propanol and its by-products of degradation. A mechanistic pathway is then proposed for the photocatalytic degradation of 1-propanol.
Notice en format standard (ISO 2709)
Pour connaître la documentation sur le format Inist Standard.
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Format Inist (serveur)
NO : | PASCAL 09-0147586 INIST |
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ET : | Photocatalytic degradation of gaseous 1-propanol using an annular reactor : Kinetic modelling and pathways |
AU : | VINCENT (G.); MARQUAIRE (P. M.); ZAHRAA (O.) |
AF : | Département de Chimie Physique des Réactions, UMR 7630 CNRS, Nancy-Université, ENSIC, 1 rue Grandville, BP 20451/54001 Nancy/France (1 aut., 2 aut., 3 aut.) |
DT : | Publication en série; Niveau analytique |
SO : | Journal of hazardous materials; ISSN 0304-3894; Coden JHMAD9; Pays-Bas; Da. 2009; Vol. 161; No. 2-3; Pp. 1173-1181; Bibl. 32 ref. |
LA : | Anglais |
EA : | Photocatalytic oxidation of airborne contaminants appears to be a promising process for remediation of air polluted by Volatile Organic Compounds (VOCs). In the present work, the photocatalytic oxidation of gaseous 1-propanol has been investigated by using an annular photoreactor. The annular photocatalytic reactor was modelled by a cascade of heightened elementary continuously stirred tank reactors. The influence of several kinetic parameters such as pollutant concentration, incident light irradiance, contact time and humidity content has been studied. The photocatalytic degradation by-products of 1-propanol has been identified in the gas-phase by GC/MS. Propionaldehyde and acetaldehyde were found to be the main gaseous intermediates. Propionaldehyde and acetaldehyde have been taken into account in a "two-site model" to evaluate the possible competition of adsorption between 1-propanol and its by-products of degradation. A mechanistic pathway is then proposed for the photocatalytic degradation of 1-propanol. |
CC : | 001D16; 001D07H; 001C01A03B; 001D07K |
FD : | Dégradation photochimique; Réacteur photochimique; Modèle cinétique; Photocatalyse; Oxydation; Pollution; Décontamination; Composé organique volatil; Réacteur catalytique; Réacteur parfaitement agité; Paramètre cinétique; Polluant; Teneur eau; Produit réaction; Modélisation; Adsorption; Devenir polluant |
FG : | Composé organique |
ED : | Photochemical degradation; Photochemical reactor; Kinetic model; Photocatalysis; Oxidation; Pollution; Decontamination; Volatile organic compound; Catalytic reactor; Continuous stirred tank reactor; Kinetic parameter; Pollutant; Water content; Reaction product; Modeling; Adsorption; Pollutant behavior |
EG : | Organic compounds |
SD : | Degradación fotoquímica; Reactor fotoquímico; Modelo cinético; Fotocatálisis; Oxidación; Polución; Descontaminación; Compuesto orgánico volátil; Reactor catalítico; Reactor perfectamente agitado; Parámetro cinético; Contaminante; Dosis agua; Producto reacción; Modelización; Adsorción; Evolución contaminante |
LO : | INIST-15708.354000185548820780 |
ID : | 09-0147586 |
Links to Exploration step
Pascal:09-0147586Le document en format XML
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<front><div type="abstract" xml:lang="en">Photocatalytic oxidation of airborne contaminants appears to be a promising process for remediation of air polluted by Volatile Organic Compounds (VOCs). In the present work, the photocatalytic oxidation of gaseous 1-propanol has been investigated by using an annular photoreactor. The annular photocatalytic reactor was modelled by a cascade of heightened elementary continuously stirred tank reactors. The influence of several kinetic parameters such as pollutant concentration, incident light irradiance, contact time and humidity content has been studied. The photocatalytic degradation by-products of 1-propanol has been identified in the gas-phase by GC/MS. Propionaldehyde and acetaldehyde were found to be the main gaseous intermediates. Propionaldehyde and acetaldehyde have been taken into account in a "two-site model" to evaluate the possible competition of adsorption between 1-propanol and its by-products of degradation. A mechanistic pathway is then proposed for the photocatalytic degradation of 1-propanol.</div>
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<server><NO>PASCAL 09-0147586 INIST</NO>
<ET>Photocatalytic degradation of gaseous 1-propanol using an annular reactor : Kinetic modelling and pathways</ET>
<AU>VINCENT (G.); MARQUAIRE (P. M.); ZAHRAA (O.)</AU>
<AF>Département de Chimie Physique des Réactions, UMR 7630 CNRS, Nancy-Université, ENSIC, 1 rue Grandville, BP 20451/54001 Nancy/France (1 aut., 2 aut., 3 aut.)</AF>
<DT>Publication en série; Niveau analytique</DT>
<SO>Journal of hazardous materials; ISSN 0304-3894; Coden JHMAD9; Pays-Bas; Da. 2009; Vol. 161; No. 2-3; Pp. 1173-1181; Bibl. 32 ref.</SO>
<LA>Anglais</LA>
<EA>Photocatalytic oxidation of airborne contaminants appears to be a promising process for remediation of air polluted by Volatile Organic Compounds (VOCs). In the present work, the photocatalytic oxidation of gaseous 1-propanol has been investigated by using an annular photoreactor. The annular photocatalytic reactor was modelled by a cascade of heightened elementary continuously stirred tank reactors. The influence of several kinetic parameters such as pollutant concentration, incident light irradiance, contact time and humidity content has been studied. The photocatalytic degradation by-products of 1-propanol has been identified in the gas-phase by GC/MS. Propionaldehyde and acetaldehyde were found to be the main gaseous intermediates. Propionaldehyde and acetaldehyde have been taken into account in a "two-site model" to evaluate the possible competition of adsorption between 1-propanol and its by-products of degradation. A mechanistic pathway is then proposed for the photocatalytic degradation of 1-propanol.</EA>
<CC>001D16; 001D07H; 001C01A03B; 001D07K</CC>
<FD>Dégradation photochimique; Réacteur photochimique; Modèle cinétique; Photocatalyse; Oxydation; Pollution; Décontamination; Composé organique volatil; Réacteur catalytique; Réacteur parfaitement agité; Paramètre cinétique; Polluant; Teneur eau; Produit réaction; Modélisation; Adsorption; Devenir polluant</FD>
<FG>Composé organique</FG>
<ED>Photochemical degradation; Photochemical reactor; Kinetic model; Photocatalysis; Oxidation; Pollution; Decontamination; Volatile organic compound; Catalytic reactor; Continuous stirred tank reactor; Kinetic parameter; Pollutant; Water content; Reaction product; Modeling; Adsorption; Pollutant behavior</ED>
<EG>Organic compounds</EG>
<SD>Degradación fotoquímica; Reactor fotoquímico; Modelo cinético; Fotocatálisis; Oxidación; Polución; Descontaminación; Compuesto orgánico volátil; Reactor catalítico; Reactor perfectamente agitado; Parámetro cinético; Contaminante; Dosis agua; Producto reacción; Modelización; Adsorción; Evolución contaminante</SD>
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